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Present theories of irreversible energy losses and heat generation within Li-ion cells are unsatisfactory because they are not compatible with energy conservation. This work aims to provide a consistent theoretical treatment of energy…

Applied Physics · Physics 2021-08-20 G. Richardson , I. Korotkin

Ion exchange processes between an ion reservoir and a solid matrix are modeled under the assumption that near interface volumes reach equilibrium in a much faster time than the overall ion exchange process time while, in the bulk of the…

Materials Science · Physics 2024-05-09 Guglielmo Macrelli

By using a first-principles approach, monolayer PbI$_2$ is found to have great potential in thermoelectric applications. The linear Boltzmann transport equation is applied to obtain the perturbation to the electron distribution by different…

Materials Science · Physics 2021-05-24 Bo Peng , Haodong Mei , Hao Zhang , Hezhu Shao , Ke Xu , Gang Ni , Qingyuan Jin , Costas M. Soukoulis , Heyuan Zhu

A data-driven solution is provided for the fast-charging problem of lithium-ion batteries with multiple safety and aging constraints. The proposed method optimizes the charging current based on the observed history of measurable battery…

Systems and Control · Electrical Eng. & Systems 2024-05-20 Hamed Taghavian , Malin Andersson , Mikael Johansson

Harvesting waste heat with temperatures lower than 100 oC can improve system efficiency and reduce greenhouse gas emissions, yet it has been a longstanding and challenging task. Electrochemical methods for harvesting low-grade heat have…

Applied Physics · Physics 2021-11-03 Xin Qian , Jungwoo Shin , Yaodong Tu , James Han Zhang , Gang Chen

We analyse the correlated back and forth dynamics and dynamic heterogeneities, i.e. the presence of fast and slow ions, for a lithium metasilicate system via computer simulations. For this purpose we define, in analogy to previous work in…

Disordered Systems and Neural Networks · Physics 2009-11-07 Andreas Heuer , Magnus Kunow , Michael Vogel , Radha D. Banhatti

Lithium-salt-based deep eutectic solvents, where the only cation is Li+, are promising candidates as electrolytes in electrochemical energy-storage devices like batteries. We have performed broadband dielectric spectroscopy on three such…

Soft Condensed Matter · Physics 2022-06-13 A. Schulz , P. Lunkenheimer , A. Loidl

In the linear regime, Onsager's response matrix provides the coupling between heat and charge currents crossing a section of thermoelectric materials of infinitesimal thickness. Integrating this response over the finite thickness of a…

Statistical Mechanics · Physics 2024-12-20 Paul Raux , Christophe Goupil , Gatien Verley

The structure of lithium ion battery components, such as electrodes and separators, are commonly characterised in terms of their porosity and tortuosity. The ratio of these values gives the effective transport of lithium ions in the…

Applied Physics · Physics 2018-06-04 Marie Francine Lagadec , Raphael Zahn , Simon Müller , Vanessa Wood

This paper presents an integrated control strategy for optimal fast charging and active thermal management of Lithium-ion batteries in extreme ambient temperatures, striking a balance between charging speed and battery health. A…

Systems and Control · Electrical Eng. & Systems 2024-10-08 Zehui Lu , Hao Tu , Huazhen Fang , Yebin Wang , Shaoshuai Mou

A Thermally Chargeable Capacitor containing a binary solution of 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)-imide (EMIMTFSI) in acetonitrile is electrically charged by applying a tempera- ture gradient to two ideally…

Soft Condensed Matter · Physics 2015-06-23 Marco Bonetti , Sawako Nakamae , Bo Tao Huang , Thomas J. Salez , Cecile Wiertel-Gasquet , Michel Roger

Aqueous electrolyte solutions under the influence of a temperature gradient can generate thermoelectric fields, which arise from different responses of the positive and negative charges. This is related to the thermo diffusion effect which…

Soft Condensed Matter · Physics 2022-06-23 André Luiz Sehnem , Antônio Martins Figueiredo Neto

Lithium ion batteries are attracting significant and growing interest, because their high energy and high power density render them an excellent option for energy storage, particularly in hybrid and electric vehicles. In this brief, a…

Systems and Control · Computer Science 2018-05-18 Rishi Relan , Yousef Firouz , Jean-Marc Timmermans , Johan Schoukens

We consider equilibrium statistical mechanics of a simplified model for the ideal conductor electrode in an interface contact with a classical semi-infinite electrolyte, modeled by the two-dimensional Coulomb gas of pointlike $\pm$ unit…

Statistical Mechanics · Physics 2009-11-11 L. Samaj , Z. Bajnok

Accurate modeling of charge transport and both thermal and luminescent radiation is crucial to the understanding and design of radiative thermal energy converters. Charge carrier dynamics in semiconductors are well-described by the…

Mesoscale and Nanoscale Physics · Physics 2021-07-13 William A. Callahan , Dudong Feng , Zhuomin M. Zhang , Eric S. Toberer , Andrew J. Ferguson , Eric J. Tervo

In this study, we address the challenge of electrolyte degradation in all-solid-state humidified Li-$O_2$ batteries, which offer high theoretical energy density and potential cost advantages over conventional lithium-ion batteries.…

Thermophoresis is the process of particles moving along a temperature gradient in thermodynamic systems. Even though it has been studied for over 150 years, there is neither a complete theoretical description of thermophoresis in liquids…

Soft Condensed Matter · Physics 2020-01-17 Benjamin F. Maier

Lithium-ion battery (Li-ion) is becoming the dominant energy storage solution in many applications such as hybrid electric and electric vehicles, due to its higher energy density and longer life cycle. For these applications, the battery…

Systems and Control · Electrical Eng. & Systems 2024-12-20 Jeongeun Son , Yuncheng Du

A statistical-type model is developed to describe the ion production and electron emission in collisions of (molecular) ions with atoms. The model is based on the Boltzmann population of the bound electronic energy levels of the quasi…

Atomic Physics · Physics 2016-08-19 Zoltán Juhász

Accurately measuring the cycle lifetime of commercial lithium-ion batteries is crucial for performance and technology development. We introduce a novel hybrid approach combining a physics-based equation with a self-attention model to…

Machine Learning · Computer Science 2025-05-07 Constantin-Daniel Nicolae , Sara Sameer , Nathan Sun , Karena Yan