Related papers: Simulating Nonadiabatic Dynamics in Benzophenone: …
We investigate the Fano-Anderson model coupled to a large ensemble of spins under the influence of an external magnetic field. The interaction between the two spin systems is treated within a meanfield-approach and we assume an anisotropic…
Singlet fission, the molecular process through which photons are effectively converted into pairs of lower energy triplet excitons, holds promise as a means of boosting photovoltaic device efficiencies. In the preceding article of this…
Internal conversion from the photoexcited state to a correlated singlet triplet-pair state is believed to be the precursor of singlet fission in carotenoids. We present numerical simulations of this process using a pi-electron model that…
We study, experimentally and theoretically, the controlled transfer of harmonically trapped ultracold gases between different quantum states. In particular we experimentally demonstrate a fast decompression and displacement of both a…
We present a theoretical study of recent laser-alignment and mixed-field-orientation experiments of asymmetric top molecules. In these experiments, pendular states were created using linearly polarized strong ac electric fields from pulsed…
We develop a computationally inexpensive model to examine the dynamics of boson-assisted electron relaxation in solids, studying nonequilibrium dynamics in a metal, in a nodal superconductor with a stationary density of states, and in a…
A dynamical many body theory of single color photoassociation in a Bose-Einstein condensate is presented. The theory describes the time evolution of a condensed atomic ensemble under the influence of an arbitrarily varying near resonant…
In trapped Bose-Einstein condensates (BECs), \emph{condensate growth} refers to the process in which an increasing number of quasi-particles are immediately transferred from the non-condensate state (the thermal cloud) into the condensate…
In condensed-matter systems, competition between ground states at phase boundaries can lead to significant changes in material properties under external stimuli, particularly when these ground states have different crystal symmetries. A key…
We study the nonequilibrium dynamics of photoexcited electrons in the narrow-gap Mott insulator VO$_2$. The initial stages of relaxation are treated using a quantum Boltzmann equation methodology, which reveals a rapid ($\sim$ femtosecond…
Identifying dynamical signatures of excited state quantum phase transitions (ESQPTs) in experimentally realizable quantum many-body systems is helpful for understanding the dynamical effects of ESQPTs. In such systems, the highly…
Modeling linear absorption spectra of solvated chromophores is highly challenging as contributions are present both from coupling of the electronic states to nuclear vibrations and solute-solvent interactions. In systems where excited…
Photoinduced charge-transfer excitations are key to understand the primary processes of natural photosynthesis and for designing photovoltaic and photocatalytic devices. In this paper, we use Bacteriochlorophyll dimers extracted from the…
We study spectroscopy of artificial solid-state four-level quantum system. This system is formed by two coupled superconducting flux qubits. When multiple driving frequency of the applied microwaves matches the energy difference between any…
Bare-state population inversion is demonstrated in a two-level system with all dipole matrix elements nonzero. A laser field is resonantly driving the sample whereas a second weaker and lower frequency coherent field additionally pumps it…
Magneto photoluminescence and excitation spectroscopy are used to probe the excited state spectrum of negatively charged trions in a InGaAs quantum dot. A single dot optical charging device allows us to selectively prepare specific few (1e,…
In conventional Bardeen-Cooper-Schrieffer (BCS) superconductors, electrons with opposite momenta bind into Cooper pairs due to an attractive interaction mediated by phonons in the material. While superconductivity naturally emerges at…
Excited-state nonadiabatic simulations with quantum mechanics/molecular mechanics (QM/MM) are essential to understand photoinduced processes in explicit environments. However, the high computational cost of the underlying quantum chemical…
We investigate the mutiphoton process between different Bloch states in an amplitude modulated optical lattice. In the experiment, we perform the modulation with more than one frequency components, which includes a high degree of freedom…
Statistical mechanics is founded on the assumption that a system can reach thermal equilibrium, regardless of the starting state. Interactions between particles facilitate thermalization, but, can interacting systems always equilibrate…