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Virtually imaged phased array (VIPA) spectrometers provide high resolution and fast acquisition in a compact design, but their performance as dispersive instruments is sensitive to fabrication tolerances, component dimensions, and…

We present and characterize a 2-D imaging spectrometer based on a virtually-imaged phased array (VIPA) disperser for rapid, high-resolution molecular detection using mid-infrared (MIR) frequency combs at 3.1 and 3.8 \mu m. We demonstrate…

Time-resolved spectroscopic temperature measurements of a sealed carbon dioxide sample cell were realized with an optical frequency comb combined with a two-dimensional dispersive spectrometer. A supercontinuum laser source based on an…

An increasing number of applications in exoplanetary science require spectrographs with high resolution and high throughput without the need for a broad spectral range. Examples include the search for biosignatures through the detection of…

Optical frequency-comb-based-high-resolution spectrometers offer enormous potential for spectroscopic applications. Although various implementations have been demonstrated, the lack of suitable mid-infrared comb sources has impeded…

We present gapless, high-resolution absorption and dispersion spectra obtained with quantum cascade laser frequency combs covering 55 cm$^{-1}$. Using phase-sensitive dual comb design, the comb lines are gradually swept over 10 GHz,…

High-resolution spectroscopy is a key element for present and future astronomical instrumentation. In particular, coupled to high contrast imagers and coronagraphs, high spectral resolution enables higher contrast and has been identified as…

We demonstrate a high-accuracy dual-comb spectrometer centered at 3.4 \mu m. The amplitude and phase spectra of the P, Q, and partial R-branch of the methane {\nu}3 band are measured at 25 MHz to 100 MHz point spacing with ~kHz resolution…

A mid-Infrared frequency comb is produced via an optical parametric oscillator (OPO) pumped by an amplified 100 MHz Yb:fiber mode-locked laser. We use this source to make measurements of the concentration of the atmospherically-relevant…

Optics · Physics 2015-05-20 Lora Nugent-Glandorf , Fabrizio Giorgetta , Scott A. Diddams

The analysis of optical spectra - emission or absorption -- has been arguably the most powerful approach for discovering and understanding matters. The invention and development of many kinds of spectrometers have equipped us with versatile…

Optical spectroscopy is a fundamental tool in numerous areas of science and technology. Much effort has focused on miniaturizing spectrometers, but thus far at the cost of high spectral resolution and broad operating range. Here, we…

We have recently introduced the Vernier-based Direct Frequency Comb Cavity-Enhanced Spectroscopy technique and we present the corresponding formalism for quantitative broadband spectroscopy. We achieve high sensitivity and broadband…

Optics · Physics 2016-11-23 Lucile Rutkowski , Jérôme Morville

Chip-scale optical frequency combs can provide broadband spectroscopy for diagnosing complex organic molecules. They are also promising as miniaturized laser spectrometers in applications ranging from atmospheric chemistry to geological…

We demonstrate the usefulness of a nanosecond pulsed single-mode mid-infrared (MIR) optical parametric oscillator (OPO) for Photoacoustic (PA) spectroscopic measurements. The maximum wavelength ranges for the signal and idler are 1.4 um to…

Applied Physics · Physics 2019-01-30 Laurent Lamard , David Balslev-Harder , Andre Peremans , Jan C. Petersen , Mikael Lassen

Quantitative phase imaging (QPI) quantifies the sample-specific optical-phase-delay enabling objective studies of optically-transparent specimens such as biological samples, but lacks chemical sensitivity limiting its application to…

Optics · Physics 2019-09-04 Miu Tamamitsu , Keiichiro Toda , Ryoichi Horisaki , Takuro Ideguchi

We report a photoacoustic spectroscopy setup with a high-power mid-infrared frequency comb as the light source. The setup is used in broadband spectroscopy of radiocarbon methane. Due to the high sensitivity of a cantilever-enhanced…

We have developed a hyperspectral imaging scheme that involves a combination of dual-comb spectroscopy and Hadamard-transform-based single-pixel imaging. The scheme enables us to obtain 12,000 hyperspectral images of amplitude and phase at…

A femtosecond frequency comb provides a vast number of equidistantly spaced narrow band laser modes that can be simultaneously tuned and frequency calibrated with 15 digits accuracy. Our Vernier spectrometer utilizes all of theses modes in…

Optical emission spectroscopy from a small-volume, 5 uL, atmospheric pressure RF-driven helium plasma was used in conjunction with Partial Least Squares Discriminant Analysis (PLS-DA) for the detection of trace concentrations of methane…

Plasma Physics · Physics 2022-07-12 Tahereh Shah Mansouri , Hui Wang , Davide Mariotti , Paul Maguire

We perform femtosecond frequency comb vernier spectroscopy in the near infrared with a femtosecond Er doped fiber laser, a scanning high-finesse cavity and an InGaAs camera. By utilizing the properties of a frequency comb and a scanning…

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