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Quantum spin liquids represent exotic states of spin systems characterized by long-range entanglement and emergent fractionalized quasiparticles. It is generally believed that disorder is hostile to quantum spin liquids. In our study, we…

Strongly Correlated Electrons · Physics 2024-08-30 Aini Xu , Qinxin Shen , Bo Liu , Zhenyuan Zeng , Lankun Han , Liqin Yan , Jun Luo , Jie Yang , Rui Zhou , Shiliang Li

One of the key questions concerning frustrated lattices that has lately emerged is the role of disorder in inducing spin-liquid-like properties. In this context, the quantum kagome antiferromagnets YCu$_3$(OH)$_6$Cl$_3$, which has been…

Strongly Correlated Electrons · Physics 2019-07-02 A. Zorko , M. Pregelj , M. Klanjšek , M. Gomilšek , Z. Jagličić , J. S. Lord , J. A. T. Verezhak , T. Shang , W. Sun , J. -X. Mi

Kagome lattice decorated with S=1/2 spins is one of the most discussed ways to realize a quantum spin liquid. However, all previous material realizations of this model have suffered from additional complications, ranging from additional…

Experimental studies of high-purity kagome-lattice antiferromagnets (KAFM) are of great importance in attempting to better understand the predicted enigmatic quantum spin-liquid ground state of the KAFM model. However, realizations of this…

Strongly Correlated Electrons · Physics 2021-06-02 W. Sun , T. Arh , M. Gomilšek , P. Koželj , S. Vrtnik , M. Herak , J. -X. Mi , A. Zorko

Finding distinct signatures of a quantum spin liquid (QSL) is an ongoing quest in condensed matter physics, invariably complicated by the presence of disorder in real materials. In this regard the 2D Kagome system…

Strongly Correlated Electrons · Physics 2024-01-22 B. S. Shivaram , J. Prestigiacomo , Aini Xu , Zhenyuan Zeng , Trevor D. Ford , Itamar Kimchi , Shiliang Li , Patrick A. Lee

Spin-1/2 kagome antiferromagnet (AFM) is one of the most studied models in frustrated magnetism since it is a promising candidate to host exotic spin liquid states. However, despite numerous studies using both analytical and numerical…

Strongly Correlated Electrons · Physics 2025-03-11 Tanja Duric , Jia Hui Chung , Bo Yang , Pinaki Sengupta

Kagome-lattice materials have attracted tremendous interest due to the broad prospect for seeking superconductivity, quantum spin liquid states, and topological electronic structures. Among them, the transition-metal kagome lattices are…

Strongly Correlated Electrons · Physics 2023-01-02 Tao Xie , Qiangwei Yin , Qi Wang , A. I. Kolesnikov , G. E. Granroth , D. L. Abernathy , Dongliang Gong , Zhiping Yin , Hechang Lei , A. Podlesnyak

Geometric frustration of magnetic ions can lead to a quantum spin liquid ground state where long range magnetic order is avoided despite strong exchange interactions. The physical realization of quantum spin liquids comprises a major…

Strongly Correlated Electrons · Physics 2023-06-07 Alex Hallett , Catalina Avarvarei , John W. Harter

General conditions in which disordered, spin liquid, and valence-bond ordered phases occur in quantum Ising antiferromagnets are studied using the prototype Kagome lattice spin models. A range of quantum dynamical processes in the Ising…

Strongly Correlated Electrons · Physics 2010-07-16 Predrag Nikolic

The kagome lattice sits at the crossroad of present research efforts in quantum spin liquids, chiral phases, emergent skyrmion excitations and anomalous Hall effects to name but a few. In light of this diversity, our goal in this paper is…

Strongly Correlated Electrons · Physics 2016-02-17 K. Essafi , Owen Benton , Ludovic D. C. Jaubert

The emergent behavior of spin liquids that are born out of geometrical frustration makes them an intriguing state of matter. We show that in the quantum kagome antiferromagnet ZnCu$_3$(OH)$_6$SO$_4$ several different correlated, yet…

Strongly Correlated Electrons · Physics 2016-03-02 M. Gomilsek , M. Klanjsek , M. Pregelj , F. C. Coomer , H. Luetkens , O. Zaharko , T. Fennell , Y. Li , Q. M. Zhang , A. Zorko

Geometrical frustration among interacting spins combined with strong quantum fluctuations destabilize long-range magnetic order in favour of more exotic states such as spin liquids. By following this guiding principle, a number of spin…

Novel magnetic phases are expected to occur in highly frustrated spin systems. Here we study the structurally perfect kagom\'e antiferromagnet CdCu$_3$(OH)$_6$(NO$_3$)$_2\cdot$H$_2$O by magnetization, magnetic torque, and heat capacity…

Strongly Correlated Electrons · Physics 2017-03-29 Ryutaro Okuma , Takeshi Yajima , Daisuke Nishio-Hamane , Tsuyoshi Okubo , Zenji Hiroi

Temperature-dependent dynamical spin correlations, which can be readily accessed via a variety of experimental techniques, hold the potential of offering a unique fingerprint of quantum spin liquids and other intriguing dynamical states. In…

Strongly Correlated Electrons · Physics 2021-01-21 P. Prelovšek , M. Gomilšek , T. Arh , A. Zorko

The interplay between geometric frustration (GF) and bond disorder is studied in the Ising kagome lattice within a cluster approach. The model considers antiferromagnetic (AF) short-range couplings and long-range intercluster disordered…

Strongly Correlated Electrons · Physics 2017-03-23 M. Schmidt , F. M. Zimmer , S. G. Magalhaes

Motivated by the recent experiments on the new spin half Kagome compound ZnCu3(OH)6Cl2, we study a phenomenological model of a frustrated quantum magnet. The model has a spin liquid groundstate and is constructed so as to mimic the…

Strongly Correlated Electrons · Physics 2009-11-13 R. Chitra , M. J. Rozenberg

The Kagome-lattice-based material, Volborthite, $\mathrm{Cu_3 V_2 O_7 (OH)_2 \cdot 2 H_2 O}$, has been considered as a promising platform for discovery of unusual quantum ground states due to the frustrated nature of spin interactions. Here…

Strongly Correlated Electrons · Physics 2017-07-19 Li Ern Chern , Kyusung Hwang , Tomonari Mizoguchi , Yejin Huh , Yong Baek Kim

We present the results of first-principle calculations using the Vienna Ab-initio Simulation Package (VASP) for a new class of organometallics labeled TM3C6O6 (TM =Sc, Ti, V, Cr, Fe, Co, Ni and Cu) in the form of planar, two-dimensional,…

Materials Science · Physics 2023-02-22 Adam Hassan Denawi , Xavier Bouju , Mathieu Abel , Johannes Richter , Roland Hayn

A three-dimensional system of interacting spins typically develops static long-range order when it is cooled. If the spins are quantum (S = 1/2), however, novel quantum paramagnetic states may appear. The most highly sought state among them…

Strongly Correlated Electrons · Physics 2015-05-13 S. -H. Lee , H. Kikuchi , Y. Qiu , B. Lake , Q. Huang , K. Habicht , K. Kiefer

Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…

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