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We used resonant inelastic x-ray scattering to reveal the nature of magnetic interactions in Sr2IrO4, a 5d transition-metal oxide with a spin-orbit entangled ground state and Jeff=1/2 magnetic momemts, referred to as 'isospins'. The magnon…

We report a high-field electron spin resonance study in the sub-THz frequency domain of a single crystal of Sr$_2$IrO$_4$ that has been recently proposed as a prototypical spin-orbital Mott insulator. In the antiferromagnetically (AFM)…

Strongly Correlated Electrons · Physics 2015-06-18 S. Bahr , A. Alfonsov , G. Jackeli , G. Khaliullin , A. Matsumoto , T. Takayama , H. Takagi , B. Büchner , V. Kataev

Sr2IrO4 is one of the prime candidates for realizing exotic quantum spin orders owing to the subtle combination of spin-orbit coupling and electron correlation. Sensitive local magnetization measurement can serve as a powerful tool to study…

Materials Science · Physics 2025-03-26 Hyeokjun Heo , Jeongha An , Junyoung Kwon , Kwangrae Kim , Youngoh Son , B. J. Kim , Joonho Jang

Protected by the interplay of on-site Coulomb interactions and spin-orbit coupling, Sr$_2$IrO$_4$ at high pressure is a rare example of a Mott insulator with a paramagnetic ground state. Here, using optical Raman scattering, we measure both…

Strongly Correlated Electrons · Physics 2021-11-29 Xiang Li , S. E. Cooper , A. Krishnadas , A. de la Torre , R. S. Perry , F. Baumberger , D. M. Silevitch , D. Hsieh , T. F. Rosenbaum , Yejun Feng

Antiferromagnetic materials feature intrinsic ultrafast spin dynamics, making them ideal candidates for future magnonic devices operating at THz frequencies. A major focus of current research is the investigation of optical methods for the…

We study the evolution of magnetic excitations in the disordered two-dimensional antiferromagnet Sr2Ir1-xRuxO4. A gigantic magnetic gap greater than 40 meV opens at x = 0.27 and increases with Ru concentration, rendering the dispersive…

Sr$_2$IrO$_4$ is a weak ferromagnet where the spin arrangement is canted anti-ferromagnetic (AF). Moreover, the spin-structure coupling plays and important role in magnetic behavior of Sr$_2$IrO$_4$. In this concern the magnetization under…

Strongly Correlated Electrons · Physics 2019-04-19 Imtiaz Noor Bhatti , A. K. Pramanik

Antiferromagnet is a promising candidate for the next generation spintronic devices, benefiting from its ultrafast dynamics and spontaneous zero stray field. However, the understanding of their ultrafast spin behaviors is lacking due to the…

We study the interaction of a (classical) light field with the magnetic degrees of freedom in the two-dimensional antiferromagnet Sr$_2$IrO$_4$. The reduced space group symmetry of the crystal allows for several channels for spin-operator…

Strongly Correlated Electrons · Physics 2019-10-14 Urban F. P. Seifert , Leon Balents

The novel electronic state of the canted antiferromagnetic (AFM) insulator, strontium iridate (Sr2IrO4) has been well described by the spin-orbit-entangled isospin Jeff = 1/2, but the role of isospin in transport phenomena remains poorly…

Strongly Correlated Electrons · Physics 2019-05-03 Nara Lee , Eunjung Ko , Hwan Young Choi , Yun Jeong Hong , Muhammad Nauman , Woun Kang , Hyoung Joon Choi , Young Jai Choi , Younjung Jo

Antiferromagnetic spintronics actively introduces new principles of magnetic memory, in which the most fundamental spin-dependent phenomena, i.e. anisotropic magnetoresistance effects, are governed by an antiferromagnet instead of a…

Materials Science · Physics 2018-05-08 Chengliang Lu , Bin Gao , Haowen Wang , Wei Wang , Songliu Yuan , Shuai Dong , Jun-Ming Liu

The collective magnetic excitations in the spin-orbit Mott insulator (Sr$_{1-x}$La$_x$)$_2$IrO$_4$ ($x=0,\,0.01,\,0.04,\, 0.1$) were investigated by means of resonant inelastic x-ray scattering. We report significant magnon energy gaps at…

Metamagnetism in antiferromagnets exhibits distinct critical behaviors and dynamics when invoking spin reversal and rotation. Here we show a 0.05% anisotropic strain suffices to in-situ modulate the metamagnetic critical field of the Mott…

Strongly Correlated Electrons · Physics 2020-07-24 H. Zhang , L. Hao , J. Yang , J. Mutch , Z. Liu , Q. Huang , K. Noordhoek , A. F. May , J. -H. Chu , J. W. Kim , P. J. Ryan , H. D. Zhou , Jian Liu

We show that, contrary to previous belief, the transition to the antiferromagnetic state of Sr$_2$IrO$_4$ in zero magnetic field does show up in the transverse resistivity. We attribute this to a change in transverse integrals associated to…

Strongly Correlated Electrons · Physics 2015-07-01 L. Fruchter , G. Collin , D. Colson , V. Brouet

Ferrimagnets containing several partially compensated magnetic sublattices are considered the most promising materials for all-optical data storage and for ultrafast communications based on spin waves. There are two magnetic phases of the…

Sr$_2$IrO$_4$ has attracted a lot of attention due to its structural and electronic similarities to La$_2$CuO$_4$ which is the parent compound of high-T$_c$ superconducting cuprates. It was proposed to be a strong spin-orbit coupled…

The effect of compression on the magnetic ground state of Sr$_2$IrO$_4$ is studied with x-ray resonant techniques in the diamond anvil cell. The weak interlayer exchange coupling between square-planar 2D IrO$_2$ layers is readily modified…

We investigated the low-energy incommensurate (IC) magnetic fluctuations in Sr$_2$RuO$_4$ by the high-resolution inelastic neutron scattering measurements and random phase approximation (RPA) calculations. We observed a spin resonance with…

The temperature-dependent behavior of magnetic domains plays an essential role in the magnetic properties of materials, leading to widespread applications. However, experimental methods to access the three-dimensional (3D) magnetic domain…

We report on high-field electron spin resonance (ESR) studies of magnetic excitations in the spin-1/2 triangular-lattice antiferromagnet Cs$_2$CuBr$_4$. Frequency-field diagrams of ESR excitations are measured for different orientations of…

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