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We present a novel method for improving the quantum simulation of the ground state energy of molecules. We perform a pre-processing step classically, which reduces the dimensionality of the problem by generating a custom mapping which…

Quantum Physics · Physics 2023-03-03 Kaur Kristjuhan , Mark Nicholas Jones

Density matrix embedding theory (DMET) is a fully quantum-mechanical embedding method which shows great promise as a method of defeating the inherent exponential cost scaling of multiconfigurational wave function-based calculations by…

Chemical Physics · Physics 2019-02-07 Matthew R. Hermes , Laura Gagliardi

Dynamic mode decomposition (DMD) is an emerging methodology that has recently attracted computational scientists working on nonintrusive reduced order modeling. One of the major strengths that DMD possesses is having ground theoretical…

Numerical Analysis · Mathematics 2022-01-12 Shady E. Ahmed , Omer San , Diana A. Bistrian , Ionel M. Navon

Quantum embedding theories are promising approaches to investigate strongly-correlated electronic states of active regions of large-scale molecular or condensed systems. Notable examples are spin defects in semiconductors and insulators. We…

Materials Science · Physics 2021-12-14 He Ma , Nan Sheng , Marco Govoni , Giulia Galli

We provide practical simulation methods for scalar field theories on a quantum computer that yield improved asymptotics as well as concrete gate estimates for the simulation and physical qubit estimates using the surface code. We achieve…

We investigate fully self-consistent multiscale quantum-classical algorithms on current generation superconducting quantum computers, in a unified approach to tackle the correlated electronic structure of large systems in both quantum…

We present a novel framework for simulating matrix models on a quantum computer. Supersymmetric matrix models have natural applications to superstring/M-theory and gravitational physics, in an appropriate limit of parameters. Furthermore,…

High Energy Physics - Theory · Physics 2021-07-23 Hrant Gharibyan , Masanori Hanada , Masazumi Honda , Junyu Liu

We present a hardware-efficient optimization scheme for quantum chemistry calculations, utilizing the Sampled Quantum Diagonalization (SQD) method. Our algorithm, optimized SQD (SQDOpt), combines the classical Davidson method technique with…

Quantum Physics · Physics 2025-03-05 Nora Bauer , Kübra Yeter-Aydeniz , George Siopsis

We extend density matrix embedding theory to periodic systems, resulting in an electronic band structure method for solid-state materials. The electron correlation can be captured by means of a local impurity model using various choices of…

Strongly Correlated Electrons · Physics 2019-09-27 Hung Q. Pham , Matthew R. Hermes , Laura Gagliardi

We report the first electronic structure calculation performed on a quantum computer without exponentially costly precompilation. We use a programmable array of superconducting qubits to compute the energy surface of molecular hydrogen…

We present a molecular extension of our recently proposed Green's function embedding method, interacting-bath dynamical embedding theory (ibDET), for computing charged excitation energies at the $GW$ and EOM-CCSD levels. Starting from…

Chemical Physics · Physics 2026-04-06 Christian Venturella , Jiachen Li , Tianyu Zhu

Structured State Space models (SSM) have recently emerged as a new class of deep learning models, particularly well-suited for processing long sequences. Their constant memory footprint, in contrast to the linearly scaling memory demands of…

Machine Learning · Computer Science 2025-07-09 Sebastian Siegel , Ming-Jay Yang , Younes Bouhadjar , Maxime Fabre , Emre Neftci , John Paul Strachan

Quantum subspace diagonalization (QSD) methods are quantum-classical hybrid methods, commonly used to find ground and excited state energies by projecting the Hamiltonian to a smaller subspace. In applying these, the choice of subspace…

Quantum Physics · Physics 2022-09-23 Akhil Francis , Anjali A. Agrawal , Jack H. Howard , Efekan Kökcü , A. F. Kemper

We present a method for calculating the ground state energy of the Fermi-Hubbard model leveraging Rydberg atom processors and sample-based quantum diagonalization (SQD). By exploiting the perturbative relationship between the Fermi-Hubbard…

Quantum Physics · Physics 2026-03-09 Kübra Yeter-Aydeniz , Nora M. Bauer

A cardinal obstacle to performing quantum-mechanical simulations of strongly-correlated matter is that, with the theoretical tools presently available, sufficiently-accurate computations are often too expensive to be ever feasible. Here we…

Strongly Correlated Electrons · Physics 2021-02-10 John Rogers , Tsung-Han Lee , Sahar Pakdel , Wenhu Xu , Vladimir Dobrosavljević , Yong-Xin Yao , Ove Christiansen , Nicola Lanatà

We introduce a scheme for molecular simulations, the Deep Potential Molecular Dynamics (DeePMD) method, based on a many-body potential and interatomic forces generated by a carefully crafted deep neural network trained with ab initio data.…

Computational Physics · Physics 2018-04-11 Linfeng Zhang , Jiequn Han , Han Wang , Roberto Car , Weinan E

High-energy particle collisions can convert energy into matter through the inelastic production of new particles. Quantum computers are an ideal platform for simulating the out-of-equilibrium dynamics of collisions and the formation of…

Quantum Physics · Physics 2025-10-31 Roland C. Farrell , Nikita A. Zemlevskiy , Marc Illa , John Preskill

A universal quantum computer can simulate diverse quantum systems, with electronic structure for chemistry offering challenging problems for practical use cases around the hundred-qubit mark. While current quantum processors have reached…

Density matrix exponentiation (DME) is a general procedure that converts an unknown quantum state into the Hamiltonian evolution. This enables state-dependent operations and can reveal nontrivial properties of the state, among other…

Quantum Physics · Physics 2025-09-19 Kaito Wada , Jumpei Kato , Hiroyuki Harada , Naoki Yamamoto

We perform a detailed resource estimate for the prospect of using deep entanglement renormalization ansatz (DMERA) on a fault-tolerant quantum computer, focusing on the regime in which the target system is large. For probing a relatively…

Quantum Physics · Physics 2024-04-18 Joshua Job , Isaac H. Kim , Eric Johnston , Steve Adachi
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