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Nonlinear optical property of transition metal dichalcogenide (TMDC) nanosheet dispersions, including MoS2, MoSe2, WS2, and WSe2, was performed by using Z-scan technique with ns pulsed laser at 1064 nm and 532 nm. The results demonstrate…

The new generation of two-dimensional (2D) materials has shown a broad range of applications for optical and electronic devices. Understanding the properties of these materials when integrated with the more traditional three-dimensional…

Nanoscale materials usually can trap light and strongly interact with it leading to many photonic device applications. The light-matter interactions are commonly probed by optical spectroscopy, which, however, have some limitations such as…

Mesoscale and Nanoscale Physics · Physics 2022-08-24 Jinlong Du , Jin-hui Chen , Yuehui Li , Ruochen Shi , Mei Wu , Yun-Feng Xiao , Peng Gao

The coupling of light to electrical charge carriers in semiconductors is the foundation of many technological applications. Attosecond transient absorption spectroscopy measures simultaneously how excited electrons and the vacancies they…

Materials Science · Physics 2023-05-03 Z. Schumacher , S. A. Sato , S. Neb , A. Niedermayr , L. Gallmann , A. Rubio , U. Keller

As superconductors are thinned down to the 2D limit, their critical temperature $T_c$ typically decreases. Here we report the opposite behavior, a substantial enhancement of $T_c$ with decreasing thickness, in 2D crystalline superconductor…

Femtosecond time-resolved core-level photoemission spectroscopy with a free-electron laser is used to measure the atomic-site specific charge-order dynamics in the charge-density-wave/Mott insulator 1T-TaS2. After strong photoexcitation, a…

Semiconducting monolayer of 2D material are able to concatenate multiple interesting properties into a single component. Here, by combining opto-mechanical and electronic measurements, we demonstrate the presence of a partial 2H-1T phase…

Monolayers of group-VI transition-metal dichalcogenides (TMDs) are two-dimensional semiconductors that exhibit exceptionally strong light-matter coupling yet typically suffer from low emission quantum yields. In this letter, we investigate…

Confining light in extreme subwavelength scales is a tantalizing task. In this work, we report a study of individual plasmonic film-coupled nanostar resonators where plasmonic optical modes are trapped in ultrasmall volumes. Individual gold…

Two-dimensional Transition-Metal Dichalcogenides (TMDs) are of great interest for second harmonic (SH) generation due to their large second-order susceptibility, atomically thin structure, and relaxed phase-matching conditions. TMDs are…

Nanophotonic technologies offer great promise for ultra-low power optical signal processing, but relatively few nonlinear-optical phenomena have yet been explored as bases for robust digital…

Vanadium dioxide (VO$_2$) is a strongly-correlated material that exhibits insulator-to-metal transition (IMT) near room temperature, which makes it a promising candidate for applications in nanophotonics or optoelectronics. However,…

Engineering optical emission from two dimensional, transition metal dichalcogenides (TMDs) materials such as Tungsten disulphide (WS2) has implications in creating and understanding nanophotonic sources. One of the challenges in controlling…

Semiconducting transition metal dichalcogenides (TMDs) have gained significant attention as a gain medium for nanolasers, owing to their unique ability to be easily placed and stacked on virtually any substrate. However, the atomically thin…

Monolayer transition metal dichalcogenides (TMDs) provide the most efficient optical gain materials and have potential for making nanolasers with the smallest gain media with lowest energy consumption. But lasing demonstrations based on…

Mesoscale and Nanoscale Physics · Physics 2017-10-25 Yongzhuo Li , Jianxing Zhang , Dandan Huang , Hao Sun , Fan Fan , Jiabi Feng , Zhen Wang , C. Z. Ning

Large chemical tunability and strong light-matter interactions make colloidal transition metal dichalcogenide (TMD) nanostructures particularly suitable for light-emitting applications. However, ultrafast exciton decay and quenched…

Newly measured optical absorption and photoluminescence spectra reveal substantial frequency shifts of both exciton and trion peaks as monolayer MoS2 is cooled from 363 K to 4 K. First-principles simulations using the GW-Bethe-Salpeter…

Mesoscale and Nanoscale Physics · Physics 2014-05-22 Ryan Soklaski , Yufeng Liang , Changjian Zhang , Haining Wang , Farhan Rana , Li Yang

The p-n diodes represent the most fundamental device building block for diverse optoelectronic functions, but are difficult to achieve in atomically thin transition metal dichalcogenides (TMDs) due to the inability to selectively dope them…

Mesoscale and Nanoscale Physics · Physics 2014-09-17 Rui Cheng , Dehui Li , Hailong Zhou , Chen Wang , Anxiang Yin , Shan Jiang , Yuan Liu , Yu Chen , Yu Huang , Xiangfeng Duan

The low temperature properties of amorphous solids are usually explained in terms of atomic-scale tunneling two level systems (TLS). For almost 20 years, individual TLS have been probed in insulating layers of superconducting quantum…

Mesoscale and Nanoscale Physics · Physics 2024-01-17 Richard Pedurand , Ilya Golokolenov , Mika Sillanpää , Laure Mercier de Lépinay , Eddy Collin , Andrew Fefferman

Monolayers of semiconducting transition metal dichalcogenides (TMDs) have long attracted interest for their intriguing optical and electronic properties. Recently TMDs in their quasi-bulk form have started to show considerable promise for…

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