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High degree of valley polarization of optically active excitons in transition-metal dichalcogenide monolayers (TMD-MLs) is vital in valley-based photonic applications but known to be likely spoiled by the intrinsic electron-hole exchange…

Mesoscale and Nanoscale Physics · Physics 2021-06-15 Ping-Yuan Lo , Guan-Hao Peng , Wei-Hua Li , Yi Yang , Shun-Jen Cheng

Localised emission from defect states in monolayer transition metal dichalcogenides is of great interest for optoelectronic and quantum device applications. Recent progress towards high temperature localised emission relies on the…

Mesoscale and Nanoscale Physics · Physics 2023-11-10 Sebastian Wood , Filipe Richheimer , Tom Vincent , Vivian Tong , Alessandro Catanzaro , Yameng Cao , Olga Kazakova , Fernando A. Castro

Optical communication can be revolutionized by encoding data into the orbital angular momentum of light beams. However, state-of-the-art approaches for dynamic control of complex optical wavefronts are mainly based on liquid crystal spatial…

Monolayer semiconducting transition metal dichalcogenides possess broken inversion symmetry and strong spin-orbit coupling, which leads to unique spin-valley locking effect. In 2H stacked pristine multilayers, the spin-valley locking yields…

Mesoscale and Nanoscale Physics · Physics 2023-06-07 Yinong Zhang , Chengxin Xiao , Dmitry Ovchinnikov , Jiayi Zhu , Xi Wang , Takashi Taniguchi , Kenji Watanabe , Jiaqiang Yan , Wang Yao , Xiaodong Xu

At the 2D limit, hexagonal systems such as monolayer transition metal dichalcogenides (TMDs) and graphene exhibit unique coupled spin and momentum-valley physics (valley pseudospin) owing to broken spatial inversion symmetry and strong…

Materials Science · Physics 2023-06-21 Tristan L Britt , Bradley J. Siwick

Strongly interacting electrons in layered materials give rise to a plethora of emergent phenomena, such as unconventional superconductivity. heavy fermions, and spin textures with non-trivial topology. Similar effects can also be observed…

Mesoscale and Nanoscale Physics · Physics 2022-08-23 Soroush Arabi , Taner Esat , Aizhan Sabitova , Yuqi Wang , Hovan Lee , Cedric Weber , Klaus Kern , F. Stefan Tautz , Ruslan Temirov , Markus Ternes

Electronic states in two-dimensional layered materials can exhibit a remarkable variety of correlated phases including Wigner-crystals, Mott insulators, charge density waves, and superconductivity. Recent experimental and theoretical…

Mesoscale and Nanoscale Physics · Physics 2021-08-16 Kai Hao , Robert Shreiner , Alexander A. High

Ultrafast nonlinear optical phenomena in solids have been attracting major interest as novel methodologies for femtosecond spectroscopy of electron dynamics and control of material properties. Here, we theoretically investigate strong-field…

Optics · Physics 2023-12-18 Anna Galler , Angel Rubio , Ofer Neufeld

The ultrafast polarization response to incident light and ensuing exciton/carrier generation are essential to outstanding optoelectronic properties of lead halide perovskites (LHPs). A large number of mechanistic studies in the LHP field to…

Altermagnets constitute an emerging materials platform for spintronic technologies by combining compensated magnetic order with ferromagnet-like spin-split electronic bands. Here, we investigate the proposed d-wave altermagnetic material…

Spatially indirect excitons with displaced wavefunctions of electrons and holes play a pivotal role in a large portfolio of fascinating physical phenomena and emerging optoelectronic applications, such as valleytronics, exciton spin Hall…

Atomic-scale heterostructures of van der Waals (vdW) magnets and semiconductors provide a unique environment for exploring magnetic dynamics. In contrast to typical photothermal excitation of precessional magnetization dynamics by a pump…

Inverted type-I heterostructure core/crown quantum rings (QRs) are quantum-efficient luminophores, whose spectral characteristics are highly tunable. Here, we study the optoelectronic properties of type-I core/crown CdS/CdSe QRs in the…

Mesoscale and Nanoscale Physics · Physics 2017-10-25 Sumanta Bose , Weijun Fan , Dao Hua Zhang

The spin polarization induced by the spin Hall effect (SHE) in thin films typically points out of the plane. This is rooted on the specific symmetries of traditionally studied systems, not in a fundamental constraint. Recently, experiments…

Alloyed transition metal dichalcogenides provide an opportunity for coupling band engineering with valleytronic phenomena in an atomically-thin platform. However, valley properties in alloys remain largely unexplored. We investigate the…

Mesoscale and Nanoscale Physics · Physics 2020-01-17 Sean M. Oliver , Joshua Young , Sergiy Krylyuk , Thomas L. Reinecke , Albert V. Davydov , Patrick M. Vora

Topological properties in quantum materials are often governed by symmetry and tuned by crystal structure and external fields, and hence symmetry-sensitive nonlinear optical measurements in a magnetic field are a valuable probe. Here we…

Mesoscale and Nanoscale Physics · Physics 2023-09-19 Shuang Wu , Zaiyao Fei , Zeyuan Sun , Yangfan Yi , Wei Xia , Dayu Yan , Yanfeng Guo , Youguo Shi , Jiaqiang Yan , David H. Cobden , Wei-Tao Liu , Xiaodong Xu , Shiwei Wu

In crystals, energy band extrema in momentum space can be identified by their valley index. The internal quantum degree of freedom associated with valley pseudospin indices can act as a useful information carrier analogous to electronic…

Electrons in two-dimensional hexagonal materials have valley degree of freedom, which can be used to encode and process quantum information. The valley-selective excitations, governed by the circularly polarised light resonant with the…

Mesoscale and Nanoscale Physics · Physics 2021-03-19 M. S. Mrudul , Álvaro Jiménez-Galán , Misha Ivanov , Gopal Dixit

The precise control of Weyl physics in realistic materials oers a promising avenue to construct accessible topological quantum systems, and thus draw widespread attention in condensed-matter physics. Here, based on rst-principles…

Computational Physics · Physics 2023-08-22 Ruoning Ji , Xianyong Ding , Fangyang Zhan , Xiaoliang Xiao , Jing Fan , Zhen Ning , Rui Wang

Monolayer transition metal dichalcogenides are promising materials for spintronics due to their robust spin-valley locked valence states, enabling efficient charge-to-spin conversion via valley Hall effect with non-equilibrium spins…

Mesoscale and Nanoscale Physics · Physics 2022-11-23 D. J. P. de Sousa , M. J. Sammon , Raseong Kim , Hai Li , Ian A. Young , Tony Low