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Recent advances in attosecond science have made it increasingly important to develop stable, reliable and accurate algorithms and methods to model the time evolution of atoms and molecules in intense laser fields. A key process in…

Chemical Physics · Physics 2024-08-19 Simon Elias Schrader , Håkon Emil Kristiansen , Thomas Bondo Pedersen , Simen Kvaal

A challenge in modeling time-dependent strong-field processes such as high-harmonic generation for many-body systems, is how to effectively represent the electronic continuum. We apply Rothe's method to the time-dependent Hartree-Fock…

Chemical Physics · Physics 2025-08-22 Simon Elias Schrader , Håkon Emil Kristiansen , Thomas Bondo Pedersen , Simen Kvaal

Solving the time-dependent Schr\"odinger equation (TDSE) is pivotal for modeling non-adiabatic electron dynamics, a key process in ultrafast spectroscopy and laser-matter interactions. However, exact solutions to the TDSE remain…

Chemical Physics · Physics 2025-12-29 Bizi Huang , Weizhong Fu , Ji Chen

When time-propagating a wave packet representing a molecular system interacting with strong attosecond laser pulses, one needs to use an approach that is capable of describing intricate coupled electronic-nuclear events that require…

Chemical Physics · Physics 2025-03-14 Aleksander P. Woźniak , Ludwik Adamowicz , Thomas Bondo Pedersen , Simen Kvaal

We present a new algorithm to solve the equations of radiation hydrodynamics (RHD) in a frequency-integrated, two-moment formulation. Novel features of the algorithm include i) the adoption of a non-local Variable Eddington Tensor (VET)…

Instrumentation and Methods for Astrophysics · Physics 2023-01-25 Shyam H. Menon , Christoph Federrath , Mark R. Krumholz , Rolf Kuiper , Benjamin D. Wibking , Manuel Jung

A Gaussian resolution method for the computation of equilibrium density matrices rho(T) for a general multidimensional quantum problem is presented. The variational principle applied to the ``imaginary time'' Schroedinger equation provides…

Quantum Physics · Physics 2009-11-10 P. Frantsuzov , A. Neumaier , V. A. Mandelshtam

Linear combinations of complex gaussian functions, where the linear and nonlinear parameters are allowed to vary, are shown to provide an extremely flexible and effective approach for solving the time-dependent Schr\"odinger equation in one…

Quantum Physics · Physics 2023-03-08 Simen Kvaal , Caroline Lasser , Thomas Bondo Pedersen , Ludwik Adamowicz

Many approximate solutions of the time-dependent Schr\"odinger equation can be formulated as exact solutions of a nonlinear Schr\"odinger equation with an effective Hamiltonian operator depending on the state of the system. We show that…

Quantum Physics · Physics 2024-09-26 Jiří J. L. Vaníček

A precise understanding of mechanisms governing the dynamics of electrons in atoms and molecules subjected to intense laser fields has a key importance for the description of attosecond processes such as the high-harmonic generation and…

The exact factorization of an electron-nuclear wavefunction [A. Abedi, N. T. Maitra, and E. K. U. Gross, Phys. Rev. Lett. 105, 123002 (2010)] allows us to define the rigorous nuclear time-dependent Schr\"{o}dinger equation (TDSE) with a…

Chemical Physics · Physics 2016-11-03 Yasumitsu Suzuki , Kazuyuki Watanabe

Generalized Hydrodynamics (GHD) has recently been devised as a method to solve the dynamics of integrable quantum many-body systems beyond the mean-field approximation. In its original form, a major limitation is the inability to predict…

We study the massless limit of the Klein-Gordon (K-G) equation in 1+1 dimensions with static complex potentials as an attempt to give an alternative, but equivalent, representation of plane electromagnetic (em) wave propagation in active…

Disordered Systems and Neural Networks · Physics 2009-11-11 H. Bahlouli , A. D. Alhaidari , A. Al-Zahrani , E. N. Economou

The semiclassically scaled time-dependent multi-particle Schr\"odinger equation describes, inter alia, quantum dynamics of nuclei in a molecule. It poses the combined computational challenges of high oscillations and high dimensions. This…

Numerical Analysis · Mathematics 2020-12-02 Caroline Lasser , Christian Lubich

We describe a numerical algorithm to integrate the equations of radiation magnetohydrodynamics in multidimensions using Godunov methods. This algorithm solves the radiation moment equations in the mixed frame, without invoking any…

High Energy Astrophysical Phenomena · Physics 2012-03-05 Yan-Fei Jiang , James M. Stone , Shane W. Davis

In the preceding paper [T. Fabcic et al., preprint] "restricted Gaussian wave packets" were introduced for the regularized Coulomb problem in the four-dimensional Kustaanheimo-Stiefel coordinates, and their exact time propagation was…

Atomic Physics · Physics 2009-04-21 T. Fabčič , J. Main , G. Wunner

Fully numerical mesh solutions of 2D and 3D quantum equations of Schroedinger and Hartree-Fock type allow us to work with wavefunctions which possess a very flexible geometry. This flexibility is especially important for calculations of…

Atomic Physics · Physics 2007-05-23 Mikhail V. Ivanov

The time-dependent Schrodinger equation (TDSE) is usually treated in real space in the textbook. However, it makes the numerical simulations of strong-field processes difficult due to the wide dispersion and fast oscillation of the electron…

Atomic Physics · Physics 2020-01-20 Yan Xu , Xue-Bin Bian

The time-dependent Schr\"{o}dinger equation for the hydrogen atom and its interaction with coherent intense high-frequency short laser pulses is solved numerically exactly by propagating the single-electron wave packets. Thereby, the…

Atomic Physics · Physics 2013-09-11 Philipp V. Demekhin , David Hochstuhl , Lorenz S. Cederbaum

Time-dependent quantum chemical methods coupled to Gaussian basis sets are gaining popularity in modeling the electron dynamics of atoms and molecules interacting with intense laser fields. Two approaches most widely used for this purpose,…

Chemical Physics · Physics 2023-01-18 Aleksander P. Woźniak , Maciej Lewenstein , Robert Moszyński

In parallel with the evolution of femtosecond and attosecond laser as well as free-electron laser technology, a variety of theoretical methods have been developed to describe the behavior of atoms, molecules, clusters, and solids under the…

Atomic Physics · Physics 2015-11-12 Kenichi L. Ishikawa , Takeshi Sato
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