Related papers: Terahertz-Induced Nonlinear Response in ZnTe
We investigate spin dynamics in the antiferromagnetic (AFM) multiferroic TbMnO3 using optical- pump, terahertz (THz)-probe spectroscopy. Photoexcitation results in a broadband THz transmission change, with an onset time of 25 ps at 6 K that…
We discuss terahertz pump-probe experiments in hBN from the perspective of Floquet optical materials and photonic time crystals. Anisotropic nature of this material results in a large separation of frequencies of in-plane and out-of-plane…
Strong field terahertz pulses are increasingly used to excite and control quantum materials at the ultrafast timescale. They have found widespread application by enabling direct addressing of the superconducting gap or Josephson resonances…
Anisotropy is ubiquitous in solids and enhanced in low-dimensional materials. In response to an electromagnetic wave, anisotropic absorptive and refractive properties result in dichroic and birefringent optical phenomena both in the linear…
We report the coherent generation and detection of terahertz (THz) pulses covering the bandwidth of 0.1-9 THz in a high repetition rate, low pulse energy laser system. In this work we demonstrate the application and evaluation of…
We present a general analysis of the influence of nonlinear optical absorption on terahertz generation via optical difference frequency generation, when reaching for the quantum conversion efficiency limit. By casting the equations…
We report a systematic investigation of both three-photon absorption (3PA)spectra and wavelength dispersions of Kerr-type nonlinear refraction in wide-gap semiconductors. The Z-scan measurements are recorded for both ZnO and ZnS with…
Contribution of plasma oscillation to the broadband terahertz emission is revealed by interacting two-color laser pulses with a supersonic jet of nitrogen molecules. Temporal and spectral shifts of THz waves are observed as the plasma…
We propose a theoretical and computational approach to investigate temporal behavior of a nonlinear polarization in perturbative regime induced by an intense and ultrashort pulsed electric field. First-principles time-dependent density…
Terahertz (THz) sciences and technologies have contributed to a rapid development of a wide range of applications and expanded the frontiers in fundamental science. Spintronic terahertz emitters offer conceptual advantages since the spin…
High input intensities are usually required to efficiently excite optical nonlinear effects in ultrathin structures. This problem is particularly critical at terahertz (THz) frequencies because high input power THz sources are not…
We introduce THz Stark spectroscopy by using intense single-cycle terahertz pulses as the electric field source and monitoring the induced spectral response of an isotropic molecular ensemble with a coincident femtosecond supercontinuum…
Terahertz microscopy has attracted attention owing to distinctive characteristics of the THz frequency region, particularly non-ionizing photon energy, spectral fingerprint, and transparency to most nonpolar materials. Nevertheless, the…
A compact terahertz (THz) polarimetric spectrometer and imaging system is demonstrated using polarization-sensitive frequency-selective surfaces (PS-FSS) and rapid, intensity-based detection. Real-time Stokes parameter extraction enables…
We present a combined theoretical and experimental study of spatio-temporal propagation effects in terahertz (THz) generation in gases using two-color ionizing laser pulses. The observed strong broadening of the THz spectra with increasing…
The spatial and spectral distributions of terahertz (THz) pulses emitted by two-color air plasmas are theoretically investigated for focused laser pulses and in the filamentation regime. We derive a so-called ''augmented'' conical emission…
We study the nonlinear optical response in a superconducting NbN thin film with strong terahertz (THz)wave. Besides the expected third harmonic generation, we observe a new transient oscillation which softensin frequency with temperature…
The anharmonic response of charge-density wave (CDW) order to strong laser-pulse perturbations in 1T-TaS_2 and TbTe_3 is investigated by means of a multiple-pump-pulse time-resolved femtosecond optical spectroscopy. We observe remarkable…
We report multicycle, narrowband, terahertz radiation at 14.8 THz produced by phase-matched optical rectification of femtosecond laser pulses in bulk lithium niobate (LiNbO$_3$) crystals. Our experiment and simulation show that the output…
Terahertz Kerr-effect (TKE) spectroscopy provides a time-domain optical probe of the intermolecular structural dynamics of liquids, but the measured birefringence can only be interpreted microscopically if transient molecular structure,…