Related papers: Terahertz-Induced Nonlinear Response in ZnTe
The spectrum of terahertz (THz) emission in gases via ionizing two-color femtosecond pulses is analyzed by means of a semi-analytic model and finite-difference-time-domain simulations in 1D and 2D geometries. We show that produced THz…
The nonlinear metamaterials have been shown to provide nonlinear properties with high nonlinear conversion efficiency and in a myriad of light manipulation. Here we study terahertz generation from nonlinear metasurface consisting of single…
We report a novel experimental technique to investigate ultrafast dynamics in photoexcited molecules by probing the third-order nonlinear optical susceptibility. A non-colinear 3-pulse scheme is developed to probe the ultrafast dynamics of…
We present an experimental and computational study of the nonlinear optical response of conduction electrons to intense terahertz (THz) electric field. Our observations (saturable absorption and an amplitude-dependent group refractive…
A calibration scheme is presented for improved polarization state measurement of terahertz pulses. In this scheme the polarization response of a two-contact terahertz photoconductive detector is accurately measured, and is used to correct…
Nonlinear processes involving frequency-mixing of light fields set the basis for ultrafast coherent spectroscopy of collective modes in solids. In certain semimetals and semiconductors, generation of coherent phonon modes can occur by a…
Nonlinear frequency conversion provides an elegant method to detect photons in a spectral range which differs from the pump wavelength, making it highly attractive for photons with inherently low energy. Aside from the intensity of the…
We demonstrate an efficient procedure for terahertz-wave radiation generation by applying a nonlinear wavelength conversion approach using a mid-infrared pump source. We used a 3.3 {\mu}m dual-chirped optical parametric amplification source…
High-energy terahertz pulses are challenging to produce due to the low conversion efficiency and limited optical damage threshold of nonlinear crystals. Here, we describe the high-efficiency generation of terahertz radiation pulses with…
The terahertz (THz) response of solvated electrons in liquid water is studied in nonlinear ultrafast pump-probe experiments. Free electrons with concentrations from c_e = 4 to 140 \times 10-6 moles/liter are generated by high-field THz or…
Coherent manipulation of magnetism through the lattice provides unprecedented opportunities for controlling spintronic functionalities on the ultrafast timescale. Such nonthermal control conventionally involves nonlinear excitation of…
We disclose an unanticipated link between plasmonics and nonlinear frequency down-conversion in laser-induced gas-plasmas. For two-color femtosecond pump pulses, a plasmonic resonance is shown to broaden the terahertz emission spectra…
Terahertz nonlinear optics is a viable method to interrogate collective phenomena in quantum materials spanning ferroelectrics, charge-density waves, and superconductivity. In superconductors this includes the Higgs amplitude and Josephson…
We demonstrate theoretically that ultrafast heating of metal nanoparticles by the laser pulse should lead to the generation of coherent terahertz (THz) radiation during the heat redistribution process. It is shown that after the femtosecond…
Coherent terahertz (THz) emission is emerging as a powerful new tool to probe symmetry breakings in quantum materials. This method relies on second order optical nonlinearities and is complementary to second harmonic generation…
We study theoretically the nonlinear optical response of disordered electrons in the regime of weak (anti)localization. Our analytical and numerical calculations reveal that, in orthogonal/symplectic class systems, two consecutive, phase…
We report on terahertz (THz) radiation under electrical pumping from a degenerate semiconductor possessing an electron accumulation layer. In InN, the random grating formed by topographical defects provides high-efficiency coupling of…
Terahertz time domain spectroscopy employing free-space radiation has frequently been used to probe the elementary excitations of low-dimensional systems. The diffraction limit blocks its use for the in-plane study of individual laterally…
Terahertz (THz) radiation, spanning from 0.3 to 3x10^12 Hz, fills the crucial gap between the microwave and infrared spectral range. THz technology has found applications in various fields, from imaging and sensing to telecommunication and…
Quantum sensing is highly attractive for accessing spectral regions in which the detection of photons is technically challenging: sample information is gained in the spectral region of interest and transferred via entanglement into another…