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Photochemical reactions on semiconductors are anisotropic, since they occur with different rates on surfaces of different orientation. Understanding the origin of this anisotropy is crucial to engineering more efficient photocatalysts. In…

Materials Science · Physics 2022-05-04 Chiara Ricca , Ulrich Aschauer

We investigate fast collisions between pulsed optical beams in a linear medium with weak cubic loss that arises due to nondegenerate two-photon absorption. We introduce a perturbation method with two small parameters and use it to obtain…

Pattern Formation and Solitons · Physics 2024-01-30 Avner Peleg , Toan T. Huynh

The amplitude and phase of a material's nonlinear optical response provide insight into the underlying electronic dynamics that determine its optical properties. Phase-sensitive nonlinear spectroscopy techniques are widely implemented to…

Mesoscale and Nanoscale Physics · Physics 2018-07-12 Galan Moody , Corey McDonald , Ari Feldman , Todd Harvey , Richard P. Mirin , Kevin L. Silverman

We calculated third order non-linear polarization to estimate the two-photon absorption of non-interacting two-level molecules in the transmission-type degenerate pump-probe geometry. The spectral intensity and the phase changes of the…

Optics · Physics 2019-05-01 Tsogvoo Khos-Ochir , Kim Myung-Whun , Purevdorj Munkhbaatar

Low-energy Fermions in semi-Dirac systems depict linear momentum dispersion along one direction while having the features of parabolic dispersion in the other direction. Equilibrium optical responses of such highly anisotropic dispersion…

Mesoscale and Nanoscale Physics · Physics 2024-10-30 Bristi Ghosh , Malay Bandopadhyay , Ashutosh Singh

Nonlinear effects are omnipresent in thin films of ion conducting materials showing up as a significant increase of the conductivity. For a disordered hopping model general physical mechanisms are identified giving rise to the occurrence of…

Disordered Systems and Neural Networks · Physics 2015-06-18 Andreas Heuer , Lars Luehning

Optical pump-probe techniques like absorption spectroscopy and microwave conductivity are widely used to characterize the carrier dynamics in perovskites for optoelectronic applications. In contrast to the prevalent assumption of…

Materials Science · Physics 2023-04-25 Pradeep R. Nair

Femtosecond spectroscopy is an important tool for tracking rapid photoinduced processes in a variety of materials. To spatially map the processes in a sample would substantially expand the capabilities of the method. This is, however,…

Optics · Physics 2019-05-01 Ondřej Denk , Kaibo Zheng , Donatas Zigmantas , Karel Žídek

In this paper, we concerned with the propagation of sound waves through stratified media. Transport equation of nonlinear geometric optics in media with mixed nonlinearity, in the case of spatially varying density and entropy fields, is…

Analysis of PDEs · Mathematics 2020-07-16 Harsh V. Mahara , V. D. Sharma

Using the functional-integral method we investigate the effective dynamics of a charged particle coupled to a set of two-level systems as a function of temperature and external electric field. The optical conductivity and the direct current…

Other Condensed Matter · Physics 2009-11-11 A. Villares Ferrer , A. O. Caldeira , C. Morais Smith

The nonlinear oscillator model is useful to basically understand the most important properties of nonlinear optical processes. It has been shown to give the correct asymptotic behaviour and to provide the general feature of harmonic…

Optics · Physics 2009-10-31 Franco Bassani , Valerio Lucarini

We propose a new method of calculating nonlinear optical responses of interacting electronic systems. In this method, the total Hamiltonian (system + system-pump interaction) is transformed into a different form that (apparently) does not…

Materials Science · Physics 2009-10-31 Jun-ichi Inoue , Akira Shimizu

Nonlinear absorption in four and five energy level systems have been studied with the aid of steady-state rate equation approach. We report on the tunability of saturable and reverse saturable absorption as a function of spectroscopic…

Optics · Physics 2018-02-28 A. Srinivasa Rao

We demonstrate a new technique for saturated-absorption spectroscopy using co-propagating beams that does not have the problem of crossover resonances. The pump beam is locked to a transition and its absorption signal is monitored while the…

Atomic Physics · Physics 2009-11-10 Ayan Banerjee , Vasant Natarajan

We analytically treat the scattering of two counter-propagating photons on a two-level emitter embedded in an optical waveguide. We find that the non-linearity of the emitter can give rise to significant pulse-dependent directional…

Quantum Physics · Physics 2015-06-24 Anders Nysteen , Dara P. S. McCutcheon , Jesper Mørk

We present a detailed analysis of strongly driven spontaneous four-wave mixing in a lossy integrated microring resonator side-coupled to a channel waveguide. A nonperturbative, analytic solution within the undepleted pump approximation is…

Quantum Physics · Physics 2015-10-28 Z. Vernon , J. E. Sipe

We investigate the linear correlation coefficient between the intensities at different wavelengths in photospheric and chromospheric spectral lines. Waves that propagate vertically through the stratified solar atmosphere affect different…

Solar and Stellar Astrophysics · Physics 2015-05-14 C. Beck , W. Rammacher

The photon statistics of Spontaneous Parametric Down Conversion (SPDC) exhibit dependencies on wavelength, pump power, and coincidence time. Notably, the average photon numbers were found to asymmetrically increase with increasing pump…

Quantum Physics · Physics 2026-05-01 Jeffrey Carvalho , Chiran Wijesundara , Tim Thomay

Topological photonics was initially inspired by the quantum-optical analogy between the Schr\"odinger equation for an electron wavefunction and the paraxial equation for a light beam. Here, we reveal an unexpected phenomenon in topological…

Pump-probe microscopy is an emerging nonlinear imaging technique based on high repetition rate lasers and fast intensity modulation. Here we present new methods for pump-probe microscopy that keep the beam intensity constant and instead…

Optics · Physics 2021-04-07 Jun Jiang , David Grass , Yue Zhou , Warren S. Warren , Martin C. Fischer
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