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The Raman effect -- inelastic scattering of light by lattice vibrations (phonons) -- produces an optical response closely tied to a material's crystal structure. Here we show that resonant optical excitation of IR and Raman phonons gives…

Materials Science · Physics 2021-07-07 Guru Khalsa , Nicole A. Benedek , Jeffrey Moses

Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$ is one of the simplest representatives of the class of lead relaxors and often serves as a model system for more complicated compounds. In this paper we analyse both polarized and depolarized Raman scattering…

Materials Science · Physics 2009-11-10 Oleksiy Svitelskiy , Jean Toulouse , Z. -G. Ye

Understanding the scattering properties of various media is of critical importance in many applications, from secure, high-bandwidth communications to extracting information about biological and mineral particles dissolved in sea water. In…

Optics · Physics 2020-02-05 Duncan McArthur , Alison Yao , Francesco Papoff

Many atomic processes result in the emission of photons. Analysis of the properties of emitted photons, such as energy and angular distribution as well as polarization, is regarded as a powerful tool for gaining more insight into the…

Atomic Physics · Physics 2018-04-18 V. A. Zaytsev , A. S. Surzhykov , V. M. Shabaev , Th. Stöhlker

Raman scattering on phonon--plasmon coupled modes in high magnetic fields is considered theoretically. The calculations of the dielectric function were performed in the long-wave approximation for the semiclassical and ultra-quantum…

Materials Science · Physics 2007-05-23 L. A. Falkovsky

When structured light is propagated through the atmosphere, turbulence results in modal scattering and distortions. An extensively studied example is that of light carrying orbital angular momentum (OAM), where the atmosphere is treated as…

Optics · Physics 2021-09-22 Asher Klug , Isaac Nape , Andrew Forbes

We theoretically and experimentally investigated transformations of vortex beams subjected to sector perturbations in the form of hard-edged aperture. The transformations of the vortex spectra, the orbital angular momentum, and the…

Optics · Physics 2020-01-08 A. Volyar , M. Bretsko , Ya. Akimova , Yu. Egorov

Raman spectra obtained by the inelastic scattering of light by crystalline solids contain contributions from first-order vibrational processes (e.g. the emission or absorption of one phonon, a quantum of vibration) as well as higher-order…

Materials Science · Physics 2017-08-22 Yannick Gillet , Stefan Kontur , Matteo Giantomassi , Claudia Draxl , Xavier Gonze

Light beams with azimuthal phase dependence [$exp(i \ell\phi)$] carry orbital angular momentum (OAM) which differs fundamentally from spin angular momentum (SAM) associated with polarization. Striking difference between the two momenta is…

Optics · Physics 2016-07-06 Ahmed H. Dorrah , Michel Zamboni-Rached , Mo Mojahedi

Raman spectroscopy has become an essential technique to characterize and investigate graphene and many other two-dimensional materials. However, there still lacks consensus on the Raman signature and phonon dispersion of atomically thin…

We provide a theoretical framework for the prediction and interpretation of momentum dependent phonon spectra due to coherent inelastic scattering of electrons. We complete the approach with first principles lattice dynamics using periodic…

Materials Science · Physics 2019-04-08 R. J. Nicholls , F. S. Hage , D. G. McCulloch , Q. M. Ramasse , K. Refson , J. R. Yates

We introduce a matter wave interference scheme based on the quantization of orbital angular momentum in a ring trap. It operates without beam splitters, is sensitive to geometric phases induced by external gauge fields, and allows measuring…

Quantum Physics · Physics 2021-04-01 Filip Kiałka , Benjamin A. Stickler , Klaus Hornberger

We report on the amplification of an optical vortex beam carrying orbital angular momentum via induced narrow Raman gain in an ensemble of cold cesium atoms. A 20\% single-pass Raman gain of a weak vortex signal field is observed with a…

Quantum Physics · Physics 2016-05-09 G. C. Borba , S. Barreiro , L. Pruvost , D. Felinto , J. W. R. Tabosa

Anisotropy of light-matter interactions in materials give remarkable information about the phonons and their interactions with electrons. We report the angle-resolved polarized Raman spectroscopy of single-crystal of Bi2Se3 to obtain the…

Materials Science · Physics 2023-04-18 Divya Rawat , Aditya Singh , Niraj Kumar Singh , Ajay Soni

Time-resolved Raman spectroscopy techniques offer various ways to study the dynamics of molecular vibrations in liquids or gases and optical phonons in crystals. While these techniques give access to the coherence time of the vibrational…

Quantum Physics · Physics 2021-04-06 Santiago Tarrago Velez , Vivishek Sudhir , Nicolas Sangouard , Christophe Galland

The orbital angular momentum (OAM) of light provides an unbounded set of orthogonal modes for ultrahigh-capacity optical information processing. However, current OAM detection schemes typically rely on light interference or diffraction,…

We compute Raman scattering intensities via the lowest-order coupling to the bosonic propagator associated with orbital nematic fluctuations in a minimal model for iron pnictides. The model consists of two bands on a square lattice…

Strongly Correlated Electrons · Physics 2013-10-15 Hiroyuki Yamase , Roland Zeyher

We calculate the eigenstates of a diatomic molecule in a range of model mean-field potentials, and evaluate the evolution of their associated Raman spectra with field strength. We demonstrate that dramatic changes in the appearance of the…

Materials Science · Physics 2022-02-22 Peter I. C. Cooke , Ioan B. Magdău , Graeme J. Ackland

Phonon-polaritons propagating in crystal volume offer the possibility of transferring information throughout matter (via phonons) at high (photon-like) velocity and tunable frequency/wavelength in the far-infrared. However, from the…

Optics · Physics 2025-09-03 Mayssoune Mina , Toni Alhaddad , Olivier Pagès

An experimental study of optical phonon modes, both normal and interface (IF) phonons, in bilayer strain-coupled InAs/GaAs_(1-x)Sb_x quantum dot heterostructures has been presented by means of low-temperature polarized Raman scattering. The…

Mesoscale and Nanoscale Physics · Physics 2024-09-17 Priyesh Kumar , Sudip Kumar Deb , Subhananda Chakrabarti , Jhuma Saha
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