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Attosecond science promises to reveal the most fundamental electronic dynamics occurring in matter and it can develop further by meeting two linked technological goals related to high-order harmonic sources: higher photon flux (permitting…

Harmonic generation from solid surfaces is a promising tool for producing high energy attosecond pulses. We report shaping of the harmonic spectrum to achieve the bandwidth necessary for attosecond pulse generation. The shaping is…

Plasma Physics · Physics 2019-03-27 A. Seyen , R. Kohn , U. Bovensiepen , D. von der Linde , A. Tarasevitch

Probing coherent quantum dynamics in light-matter interactions at the microscopic level requires high-repetition-rate isolated attosecond pulses (IAPs) in pump-probe experiments. To date, the generation of IAPs has been mainly limited to…

Isolated attosecond pulses (IAP) generated by high-order harmonic generation are valuable tools that enable dynamics to be studied on the attosecond time scale. The applicability of these IAP would be widened drastically by increasing their…

Generation of ultrabroadband isolated attosecond pulses (IAPs) is essential for time-resolved applications in chemical and material sciences, as they have the potential to access the spectral water window region of chemical elements, which…

Mesoscale and Nanoscale Physics · Physics 2022-04-20 Younes Adnani , Abdelmalek Taoutioui , Abdelkader Makhoute , Károly Tökési , Hicham Agueny

A thin and dense plasma layer is created when a sufficiently strong laser pulse impinges on a solid target. The nonlinearity introduced by the time-dependent electron density leads to the generation of harmonics. The pulse duration of the…

Plasma Physics · Physics 2009-10-31 D. Bauer , R. R. E. Salomaa , P. Mulser

A new method to coherently control the electron dynamics is proposed using a few-cycle laser pulse in combination with a controlling field. It is shown that this method not only broadens the attosecond pulse bandwidth, but also reduces the…

Atomic Physics · Physics 2015-04-06 Pengfei Lan , Peixiang Lu , Wei Cao , Yuhua Li , Xinlin Wang

The ability to perform attosecond-pump attosecond-probe spectroscopy (APAPS) is a longstanding goal in ultrafast science. While first pioneering experiments demonstrated the feasibility of APAPS, the low repetition rates (10-120 Hz) and the…

High harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, to date the shortest attosecond (as) pulses have been produced only in the extreme ultraviolet…

Attosecond electron pulses enable real-time probing of ultrafast matter dynamics, yet conventional modulation schemes suffer from drastically shortened longitudinal focal lengths when targeting sub-attosecond durations. To address this…

Plasma Physics · Physics 2026-05-15 Qi Huang , Qing Jia , Zhongxuan Wang , Jian Zheng

High harmonic generation by relativistically intense laser pulses from overdense plasma layers is surveyed. High harmonics are generated in form of (sub-)attosecond pulses when the plasma surface rebounds towards the observer with…

Plasma Physics · Physics 2011-11-18 Daniel an der Brügge , Alexander Pukhov

The creation of attosecond pulses via laser-plasma interaction has been a subject of great scientific interest for more than three decades. This process is investigated by using particle-in-cell simulation with varying the plasma and laser…

Plasma Physics · Physics 2021-09-24 Lin Cheng , Zhixin Fan , Liguang Jiao , Aihua Liu

An optical coherent control scheme has been proposed and theoretically investigated where an extreme ultraviolet single attosecond pulse (SAP) propagates through a dense helium gas dressed by a time-delayed femtosecond laser pulse. The…

Atomic Physics · Physics 2012-09-26 Wei-Chun Chu , C. D. Lin

We report theoretical calculations of high-order harmonic generation (HHG) of Xe with the inclusion of multi-electron effects and macroscopic propagation of the fundamental and harmonic fields in an ionizing medium. By using the…

Atomic Physics · Physics 2011-10-11 Cheng Jin , Anh-Thu Le , Carlos A. Trallero-Herrero , C. D. Lin

Strongly laser-driven semiconductor crystals offer substantial advantages for the study of many-body physics and ultrafast optoelectronics via the high harmonic generation process. While this phenomenon has been employed to investigate the…

Isolated attosecond pulses (IAPs) generated by few-cycle femtosecond lasers are essential for capturing ultrafast dynamics in atoms, molecules, and solids. Nonetheless, the advancement of attosecond science critically depends on achieving…

The generation of ultrashort light pulses is essential for the advancement of attosecond science. Here, we show that attosecond pulses approaching the Fourier limit can be generated through optimized optical driving of tunneling particles…

Mesoscale and Nanoscale Physics · Physics 2024-02-19 Shohei Imai , Atsushi Ono

Ultrafast processes in matter can be captured and even controlled by using sequences of few-cycle optical pulses, which need to be well characterized, both in amplitude and phase. The same degree of control has not yet been achieved for…

The shortest light pulses produced to date are of the order of a few tens of attoseconds, with central frequencies in the extreme ultraviolet range and bandwidths exceeding tens of eV. They are often produced as a train of pulses separated…

We generate high-order harmonics in gaseous medium with tunable photon energy using time domain interferometry of double pulses in a non-collinear generation geometry. The method is based on the fact that the generated harmonics inherit…

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