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We demonstrate, numerically, the possibility of manipulating the spin states of molecular nanomagnets with shaped microwave pulses designed with quantum optimal control theory techniques. The state-to-state or full gate transformations can…

Quantum Physics · Physics 2021-12-01 Alberto Castro , Adrian Garcia Carrizo , David Zueco , Fernando Luis

We present a general method to realize resonant coupling between spins even though their energies are of different scales. Applying the method to the electron and nuclear spin systems such as a nitrogen-vacancy (NV) center with its nearby…

Quantum Physics · Physics 2023-11-20 Sichen Xu , Chanying Xie , Zhen-Yu Wang

Cavities in large-scale photonic integrated circuits often suffer from a wider distribution of resonance frequencies due to fabrication errors. It is crucial to adjust the resonances of cavities using post-processing methods to minimize the…

Optics · Physics 2024-09-26 Mohit Khurana , Sahar Delfan , Zhenhuan Yi

A nitrogen-vacancy (NV) center in a diamond enables the access to an electron spin, which is expected to present highly sensitive quantum sensors. Although exploiting a nitrogen nuclear spin improves the sensitivity, manipulating it using a…

The experimental optimization of a two-qubit controlled-Z (CZ) gate is realized following two different data-driven gradient ascent pulse engineering (GRAPE) protocols in the aim of optimizing the gate operator and the output quantum state,…

Spin relaxometry with nitrogen-vacancy (NV) centers in diamond offers a spectrally selective, atomically localized, and calibrated measurement of microwave-frequency magnetic noise, presenting a versatile probe for condensed matter and…

Controlling ensembles of weakly coupled spins typically requires computationally expensive multispin optimisations. We present a compact framework that enables control of weakly coupled spin systems (of any spin), but using RF pulses…

Quantum Physics · Physics 2026-02-12 Suzanne Lim , Bowen Guo , Abi Turner , Charles Buchanan , Andrew Baldwin , Jonathan A. Jones

NV-diamonds have attracted keen interest for nanoscale sensing and spin manipulation. In particular, the non-equilibrium electron spin polarization after optical excitation of single NV centers has successfully been transferred to nuclear…

Mesoscale and Nanoscale Physics · Physics 2021-11-24 R. Rizzato , F. Bruckmaier , K. S. Liu , S. J. Glaser , D. B. Bucher

Nitrogen-Vacancy (NV) centers in diamond are attractive tools for sensing and quantum information. Realization of this potential requires effective tools for controlling the spin degree of freedom by microwave (mw) magnetic fields. In this…

Quantum Physics · Physics 2023-02-06 Anton Savitsky , Jingfu Zhang , Dieter Suter

We propose the use of non-equally spaced decoupling pulses for high-resolution selective addressing of nuclear spins by a quantum sensor. The analytical model of the basic operating principle is supplemented by detailed numerical studies…

Quantum Physics · Physics 2015-10-13 J. Casanova , Z. -Y. Wang , J. F. Haase , M. B. Plenio

In our recent study [arXiv:2601.03407] we showed that a hybrid non-degenerate parametric amplifier could be realized for a microwave mode and an ensemble of NV-centers (or other spins) by parametrically driving the spin ensemble. The…

Nuclear magnetic resonance (NMR) schemes can be applied to micron-, and nanometer-sized samples by the aid of quantum sensors such as nitrogen-vacancy (NV) color centers in diamond. These minute devices allow for magnetometry of nuclear…

Quantum Physics · Physics 2021-07-19 C. Munuera-Javaloy , R. Puebla , J. Casanova

In cavity magnomechanical systems, magnetic excitations couple simultaneously with mechanical vibrations and microwaves, incorporating the tunability of magnetism and the long lifetimes of mechanical modes. Applications of such systems,…

Mesoscale and Nanoscale Physics · Physics 2025-10-13 V. A. S. V. Bittencourt , C. A. Potts , J. P. Davis , A. Metelmann

On the basis of optimal control theory, we numerically study how to optimally manipulate molecular vibrational dynamics by using cycle-averaged polarizability interactions induced by mildly intense non-resonant laser (NR) pulses. As the…

Quantum Physics · Physics 2024-09-05 Reon Ishii , Tomotaro Namba , Hiroyuki Katsuki , Kenji Ohmori , Yukiyoshi Ohtsuki

A pulse generation scheme is proposed based on a structured resonance in a cavity where the non-conventional energy distribution is concentrated in its middle part. The cavity is first used as an oscillator during the energy charging step…

Applied Physics · Physics 2022-06-29 Dmitry Oshmarin , Alireza Nikzamir , Michael M. Green , Filippo Capolino

Spin defects in solids, such as the nitrogen-vacancy (NV) center in diamond, have emerged as a key tool for detecting nuclear spins at the nanoscale. While active nuclear spin control via radio-frequency (RF) irradiation is often…

Ensembles of nitrogen-vacancy (NV) centers are used as sensors to detect NMR signals from micron-sized samples at room temperature. In this scenario, the regime of large magnetic fields is especially interesting as it leads to a large…

Quantum Physics · Physics 2023-04-04 C. Munuera-Javaloy , A. Tobalina , J. Casanova

The nitrogen-vacancy (NV) centre in diamond is a leading platform for nanoscale sensing and imaging, as well as quantum information processing in the solid state. To date, individual control of two NV electronic spins at the nanoscale has…

We present a continuous-time, neural-network-based approach to optimal control in quantum systems, with a focus on pulse engineering for quantum gates. Leveraging the framework of neural ordinary differential equations, we construct control…

Detecting nuclear spins using single Nitrogen-Vacancy (NV) centers is of particular importance in nano-scale science and engineering, but often suffers from the heating effect of microwave fields for spin manipulation, especially under high…

Quantum Physics · Physics 2024-09-06 Zhiyi Hu , Fengjian Jiang , Jingyan He , Yulin Dai , Ya Wang , Nanyang Xu , Jiangfeng Du
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