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Molecular bridges covalently bonded to two ferromagnetic electrodes can transform ferromagnetic materials and produce intriguing spin transport characteristics. This paper discusses the impact of molecule induced strong coupling on spin…

Materials Science · Physics 2019-12-04 Pawan Tyagi , Edward Friebe

We propose a mechanism to use scanning tunneling microscopy (STM) for direct measurements of the two-electron singlet-triplet exchange splitting $J$ in diatomic molecular systems, unsing the coupling between the molecule and the substrate…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 J. Fransson , A. V. Balatsky

A scanning tunneling microscope (STM) with a magnetic tip that has a sufficiently strong spin-polarization can be used to map the sample's spin structure down to the atomic scale but usually lacks the possibility to absolutely determine the…

Superconductivity · Physics 2021-04-26 Lucas Schneider , Philip Beck , Jens Wiebe , Roland Wiesendanger

Artificial nanostructures, fabricated by placing building blocks such as atoms or molecules in well-defined positions, are a powerful platform in which quantum effects can be studied and exploited on the atomic scale. Here, we report a…

Mesoscale and Nanoscale Physics · Physics 2023-12-04 Taner Esat , Markus Ternes , Ruslan Temirov , F. Stefan Tautz

The nuclear spin, being much more isolated from the environment than its electronic counterpart, enables quantum experiments with prolonged coherence times and presents a gateway towards uncovering the intricate dynamics within an atom.…

Mesoscale and Nanoscale Physics · Physics 2023-09-08 Lukas M. Veldman , Evert W. Stolte , Mark P. Canavan , Rik Broekhoven , Philip Willke , Laëtitia Farinacci , Sander Otte

Among the possible types of magnetic dipole interactions in molecular systems, couplings between nuclear motion and the nuclear spin have probably received the least attention in molecular spectroscopy. Although very small in comparison to…

Chemical Physics · Physics 2026-04-22 Matthias Diez , Johannes K. Krondorfer , Albert Hirtenfelder , Andreas W. Hauser

Molecular magnets are a promising class of materials with exciting properties and applications. However, a profound understanding and application of such materials depends on the accurate detection of their electronic and magnetic…

Molecular nanomagnets show clear signatures of coherent behavior and have a wide variety of effective low-energy spin Hamiltonians suitable for encoding qubits and implementing spin-based quantum information processing. At the nanoscale,…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Mircea Trif , Filippo Troiani , Dimitrije Stepanenko , Daniel Loss

Transition-metal phthalocyanine molecules have attracted considerable interest in the context of spintronics device development due to their amenability to diverse bonding regimes and their intrinsic magnetism. The latter is highly…

Strongly Correlated Electrons · Physics 2024-12-19 Sumanta Bhandary , Emiliano Poli , Gilberto Teobaldi , David D. O'Regan

The ongoing miniaturization in nanoscience and -technology challenges the sensitivity and selectivity of experimental analysis methods to the ultimate level of single atoms and molecules. A promising new approach, addressed here, focuses on…

Mesoscale and Nanoscale Physics · Physics 2014-03-28 Stefan Müllegger , Stefano Tebi , Amal K. Das , Wolfgang Schöfberger , Felix Faschinger , Reinhold Koch

We present a theoretical study of spin-dependent transport through molecular wires bridging ferromagnetic metal nanocontacts. We extend to magnetic systems a recently proposed model that provides a em quantitative explanation of the…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Eldon Emberly , George Kirczenow

A key to building functional devices on the basis of single molecule magnets in the framework of molecular electronics is the ability to deposit and study these molecules on a surface, because the structural, electronic and magnetic…

Mesoscale and Nanoscale Physics · Physics 2016-01-26 Judith Donner , Jan-Philipp Broschinski , Bastian Feldscher , Anja Stammler , Hartmut Bögge , Thorsten Glaser , Daniel Wegner

The plasmonic tip of a scanning tunnelling microscope (STM) is functionalized with a single fluorescent molecule and is scanned on a plasmonic substrate. The tunneling current flowing through the tip-molecule-substrate junction generates a…

We report on inelastic electron tunneling spectroscopy measurements carried out on single molecules incorporated into a mechanically controllable break-junction of Au and Pt electrodes at low temperature. Here we establish a correlation…

Mesoscale and Nanoscale Physics · Physics 2010-11-16 Youngsang Kim , Hyunwook Song , Florian Strigl , Hans-Fridtjof Pernau , Takhee Lee , Elke Scheer

The conductance profiles of magnetic transition metal atoms, such as Fe, Co and Mn, deposited on surfaces and probed by a scanning tunneling microscope (STM), provide detailed information on the magnetic excitations of such nano-magnets. In…

Mesoscale and Nanoscale Physics · Physics 2013-05-30 Aaron Hurley , Nadjib Baadji , Stefano Sanvito

The effect of magnetic STM-tip on electronic, magnetic and electronic transport properties through the molecule junction STM-tip-Co/CoPc/Co(111), has been investigated by mean of ab initio electronic structure calculations. The spin…

Quantum Physics · Physics 2025-02-25 Ali Jaafar , Tarek Khalil

The spin dynamics of all ferromagnetic materials are governed by two types of collective excitations: spin waves and domain walls. The fundamental processes underlying these collective modes, such as exchange interactions and magnetic…

Mesoscale and Nanoscale Physics · Physics 2015-09-22 A. Spinelli , B. Bryant , F. Delgado , J. Fernández-Rossier , A. F. Otte

It is proposed that nuclear (or electron) spins in a trapped molecule would be well isolated from the environment and the state of each spin can be measured by means of mechanical detection of magnetic resonance. Therefore molecular traps…

Quantum Physics · Physics 2007-05-23 Haiqing Wei , Xin Xue

Single molecular magnet (SMM) like paramagnetic molecules interacting with the ferromagnetic electrodes of a magnetic tunnel junction (MTJ) produce a new system that differs dramatically from the properties of isolated molecules and…

Materials Science · Physics 2021-05-26 Andrew Grizzle , Christopher DAngelo , Pawan Tyagi

We present measurements of magnetic tunnel junctions made using a self-assembled-monolayer molecular barrier. Ni/octanethiol/Ni samples were fabricated in a nanopore geometry. The devices exhibit significant changes in resistance as the…

Mesoscale and Nanoscale Physics · Physics 2010-10-05 J. R. Petta , S. K. Slater , D. C. Ralph