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With climate modeling predicting a raise of at least 2 C by year 2100, the fate of ice has become a serious concern, but we still do not understand how ice grows (or melts). In the atmosphere, crystal growth rates of basal and prismatic…

Atmospheric and Oceanic Physics · Physics 2021-01-07 Pablo Llombart , Eva G. Noya , Luis G. MacDowell

We present measurements of growth rates of the (0001) facet surface of ice as a function of water vapor supersaturation over the temperature range $-2$ $\geq T\geq -40$ C. From these data we infer the temperature dependence of premelting on…

Materials Science · Physics 2011-10-27 K. G. Libbrecht , M. E. Rickerby

We describe a comprehensive model for the formation and morphological development of atmospheric ice crystals growing from water vapor, also known as snow crystals. Our model derives in part from empirical measurements of the intrinsic ice…

Materials Science · Physics 2012-11-26 Kenneth G. Libbrecht

We present measurements of the growth rates of the principal facet surfaces of ice from water vapor as a function of supersaturation over the temperature range -2 C > T > -40 C. Our data are well described by a dislocation-free…

Materials Science · Physics 2014-08-26 K. G. Libbrecht , M. E. Rickerby

We present measurements of the diffusion-limited growth of ice crystals from water vapor at a temperature of -5 C, in air at a pressure of $p_{air}=1$ bar. Starting with thin, c-axis ice needle crystals, the subsequent growth morphologies…

Materials Science · Physics 2016-03-01 Kenneth G. Libbrecht

We investigate about the possibility of knowing the thermal history of each snow crystal through the analysis of its individual habitus. Supposition, based on experimental observations, that prevailing growth mechanisms of basal and…

Atmospheric and Oceanic Physics · Physics 2010-05-31 Federico Falcon

We examine ice crystal growth from water vapor at temperatures near the melting point, when surface premelting creates a quasiliquid layer at the solid/vapor interface. Recent ice growth measurements as a function of vapor supersaturation…

Materials Science · Physics 2014-07-04 Kenneth G. Libbrecht

In this paper I examine snow crystal growth near -14 C in comparison with a comprehensive model that includes Structure-Dependent Attachment Kinetics (SDAK). Analyzing a series of ice-growth observations in air, I show that the data…

Materials Science · Physics 2021-08-12 Kenneth G. Libbrecht

We propose a new type of morphological instability in the diffusion-limited growth of faceted crystals from the vapor phase that can explain the formation of thin ice plates at temperatures near -15 C. The instability appears when the…

Materials Science · Physics 2007-05-23 Kenneth G. Libbrecht

I examine the molecular dynamics of ice growth from water vapor, focusing on how the attachment kinetics can be augmented by edge-dependent surface diffusion. Although there are significant uncertainties in developing an accurate physical…

Materials Science · Physics 2020-12-25 Kenneth G. Libbrecht

I describe a semi-empirical molecular model of the surface attachment kinetics governing ice crystal growth from water vapor as a function of temperature, supersaturation, and crystal mesostructure. An important new hypothesis in this model…

Materials Science · Physics 2019-11-14 Kenneth G. Libbrecht

Molecular simulations employing empiric force fields have provided valuable knowledge about the ice growth process in the last decade. The development of novel computational techniques allows us to study this process, which requires long…

Soft Condensed Matter · Physics 2023-06-07 Pablo Montero de Hijes , Salvatore Romano , Alexander Gorfer , Christoph Dellago

We present measurements of the diffusion-limited growth of ice crystals from water vapor at different supersaturation levels in air at a temperature of -15 C. Starting with thin, c-axis ice needle crystals, the subsequent growth…

Materials Science · Physics 2015-12-14 Kenneth Libbrecht , Christopher Miller , Ryan Potter , Nina Budaeva , Cameron Lemon , Sarah Thomas

I examine a variety of snow crystal growth measurements taken at a temperature of -5 C, as a function of supersaturation, background gas pressure, and crystal morphology. Both plate-like and columnar prismatic forms are observed under…

Materials Science · Physics 2019-12-09 Kenneth G. Libbrecht

I examine a variety snow crystal growth experiments performed at temperatures near -2 C, as a function of supersaturation, background gas pressure, and crystal morphology. Although the different experimental data were obtained using quite…

Materials Science · Physics 2020-04-15 Kenneth G. Libbrecht

Facetted growth of snow crystals leads to a rich diversity of forms, and exhibits a remarkable sixfold symmetry. Snow crystal structures result from diffusion limited crystal growth in the presence of anisotropic surface energy and…

Materials Science · Physics 2012-08-02 John W. Barrett , Harald Garcke , Robert Nürnberg

We examine the molecular dynamics of crystal growth in the presence of surface melting and surface impurities, and from this propose a detailed microscopic model for the growth of ice from the vapor phase. Our model naturally accounts for…

Materials Science · Physics 2008-10-06 Kenneth G. Libbrecht

Molecular dynamic simulations were performed for ice Ih with a free surface by using four water models, SPC/E, TIP4P, TIP4P/Ice and TIP4P/2005. The behavior of the basal plane, the primary prismatic plane and of the secondary prismatic…

Other Condensed Matter · Physics 2009-01-14 M. M. Conde , C. Vega , A. Patrykiejew

Close to the triple point, the surface of ice is covered by a thin liquid layer (so-called quasi-liquid layer) which crucially impacts growth and melting rates. Experimental probes cannot observe the growth processes below this layer, and…

Chemical Physics · Physics 2021-01-22 David N. Sibley , Pablo Llombart , Eva G. Noya , Andrew J. Archer , Luis G. MacDowell

I describe techniques for making precise measurements of the growth rates of the principal facets of ice crystals. Particular attention is paid to identifying and reducing systematic errors in the measurements, as these have plagued earlier…

Materials Science · Physics 2007-05-23 Kenneth G. Libbrecht
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