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Transport through molecular contacts with a sluggish intramolecular vibrational mode strongly coupled to excess charges is studied far from equilibrium. A Born-Oppenheimer approximation in steady state reveals voltage dependent energy…

Mesoscale and Nanoscale Physics · Physics 2012-06-27 Lars Kecke , Joachim Ankerhold

The interaction of strong laser fields with matter intrinsically provides powerful tools to image transient dynamics with an extremely high spatiotemporal resolution. Here, we study strong-field ionisation of laser-aligned molecules and…

Achieving precise control of photoinduced molecular charge transfer reactions underpins key emerging technologies. As such, the use of hybrid light-matter molecular exciton-polariton states has been proposed as a scheme to directly modify…

Linear polarization analysis of hard x-rays is employed to probe electronic anisotropies in metal-containing complexes with very high selectivity. We use the pronounced linear dichroism of nuclear resonant x-ray scattering to determine…

We present a hybrid method based on a combination of quantum/classical molecular dynamics (MD) simulations and a mod el Hamiltonian approach to describe charge transport through bio-molecular wires with variable lengths in presence o f a…

Soft Condensed Matter · Physics 2015-05-13 R. Gutierrez , R. Caetano , P. B. Woiczikowski , T. Kubar , M. Elstner , G. Cuniberti

We have investigated the charge carrier transport in organic molecular semiconductors. It has been found that mobility is a function of electric field and temperature due to hopping conduction. Several theoretical models for charge…

Materials Science · Physics 2007-05-23 Ajit Kumar Mahapatro , Subhasis Ghosh

Photo-induced charge transfer of positive and negative charges across the interface between an ordered organic semiconductor and a polymeric insulator is observed in the field-effect experiments. Immobilization of the transferred charge in…

Materials Science · Physics 2009-11-10 V. Podzorov , M. E. Gershenson

We numerically investigate photo-responses of the charge ordered state upon stimuli of pulsed laser light, especially paying attention to the differences in the pulse width, whose shortness has been a key to experimentally realize large…

Strongly Correlated Electrons · Physics 2023-03-31 Hitoshi Seo , Yasuhiro Tanaka

As a consequence of the chiral anomaly, the hydrodynamics of hot QCD matter coupled to QED allows for a long-wavelength mode of chiral charge density, the chiral magnetic wave (CMW), that provides for a mechanism of electric charge…

High Energy Physics - Phenomenology · Physics 2015-03-05 Seyed Farid Taghavi , Urs Achim Wiedemann

Interfacial ultrafast electron migration processes are simulated in finite cluster models of dye-sensitized solar cells within a single active electron approach. Initially, three different donor-acceptor $\pi$-conjugated dyes supported on…

Chemical Physics · Physics 2017-07-06 Gunter Hermann , Felix Witte , Jean Christophe Tremblay

We investigate on the same footing the time-dependent electronic transport properties and vibrational dynamics of a molecular junction. We show that fluctuations of both the molecular vibron displacement and the electronic current across…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Rémi Avriller , R Souto , A. Martin-Rodero , A Yeyati

We calculate the inelastic light scattering from X-rays, which allows the photon to transfer both energy and momentum to the strongly correlated charge excitations. We find that the charge transfer peak and the low energy peak both broaden…

Strongly Correlated Electrons · Physics 2009-11-07 T. P. Devereaux , G. E. D. McCormack , J. K. Freericks

Laser-induced electron tunneling underlies numerous emerging spectroscopic techniques to probe attosecond electron dynamics in atoms and molecules. The improvement of those techniques requires an accurate knowledge of the exit momentum for…

We use inhomogeneous nonequilibrium dynamical mean-field theory to investigate the spreading of photo-excited carriers in Mott insulating heterostructures with strong internal fields. Antiferromagnetic correlations are found to affect the…

Strongly Correlated Electrons · Physics 2014-08-15 Martin Eckstein , Philipp Werner

We investigate the role of electron correlation in the two-photon double ionization of helium for ultrashort XUV pulses with durations ranging from a hundred attoseconds to a few femtoseconds. We perform time-dependent ab initio…

We present numerical simulations of ultrafast multiphoton ionization dynamics in a two-dimensional atomic model driven by co- and counterrotating circularly polarized single-color and bichromatic carrier envelope phase (CEP) stable…

Atomic Physics · Physics 2020-07-15 T. Bayer , Ch. Philipp , K. Eickhoff , M. Wollenhaupt

We use three dimensional time-dependent Schr\"odinger equation (3D--TDSE) to calculate angular electron momentum distributions and photoelectron spectra of atoms driven by spatially inhomogeneous fields. An example for such inhomogeneous…

Atomic Physics · Physics 2013-06-26 M. F. Ciappina , J. A. Pérez-Hernández , T. Shaaran , L. Roso , M. Lewenstein

We numerically investigate the dynamics of multiply charged hydrogenic ions in near-optical linearly polarized laser fields with intensities of order 10^16 to 10^17 W/cm^2. Depending on the charge state Z of the ion the relation of strength…

Quantum Physics · Physics 2009-11-06 S. X. Hu , C. H. Keitel

Contact electrification, or contact charging, refers to the process of static charge accumulation after rubbing, or even simple touching, of two materials. Despite its relevance in static electricity, various natural phenomena, and numerous…

Soft Condensed Matter · Physics 2023-12-20 Hang Zhang , Sankaran Sundaresan , Michael A. Webb

Modern intense ultrafast pulsed lasers generate an electric field of sufficient strength to permit tunnel ionization of the valence electrons in atoms. This process is usually treated as a rapid succession of isolated events, in which the…