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Recent advances in increasing the spectroscopic energy resolution in scanning tunneling microscopy (STM) have been achieved by integrating electron spin resonance (ESR) with STM. Here, we demonstrate the design and performance of a…

Electron spin resonance with a scanning tunneling microscope (ESR-STM) combines the high energy resolution of spin resonance spectroscopy with the atomic scale control and spatial resolution of STM. Here we describe the upgrade of a…

Instrumentation and Detectors · Physics 2019-01-30 Fabian D. Natterer , François Patthey , Tobias Bilgeri , Patrick R. Forrester , Nicolas Weiss , Harald Brune

Electron spin resonance (ESR) spectroscopy in scanning tunneling microscopy (STM) has enabled probing the electronic structure of single magnetic atoms and molecules on surfaces with unprecedented energy resolution, as well as demonstrating…

Integration of electron spin resonance (ESR) in a scanning tunneling microscope (STM) has enabled an all-electrical control of atomic and molecular spins on solid surfaces with atomic-scale precision and energy resolution beyond thermal…

Mesoscale and Nanoscale Physics · Physics 2025-09-03 Deung-Jang Choi , Soo-hyon Phark , Andreas J. Heinrich , Nicolás Lorente

Magnetic media remain a key in information storage and processing. The continuous increase of storage densities and the desire for quantum memories and computers pushes the limits of magnetic characterisation techniques. Ultimately, a tool…

Electron paramagnetic resonance (EPR) performed with a scanning tunneling microscope (STM) allows for probing the spin excitation of single atomic species with MHz energy resolution. One of the basic applications of conventional EPR is the…

Mesoscale and Nanoscale Physics · Physics 2021-11-10 Tom S. Seifert , Stepan Kovarik , Pietro Gambardella , Sebastian Stepanow

Thermometry based on magnetic resonance has been extensively studied due to its important application in biomedical imaging. In our previous work, we showed that the spin-spin relaxation time (T2) of nuclear magnetic resonance (NMR) in…

Applied Physics · Physics 2024-11-05 Pei-Yun Lin , Darshan Chalise , David G. Cahill

In the last decade, detecting spin dynamics at the atomic scale has been enabled by combining techniques like electron spin resonance (ESR) or pump-probe spectroscopy with scanning tunneling microscopy (STM). Here, we demonstrate an…

Scanning tunneling microscopy (STM) and micro-electromechanical systems (MEMS) have traditionally addressed vastly different length scales - one resolving atoms, the other engineering macroscopic motion. Here we unite these two fields to…

Mesoscale and Nanoscale Physics · Physics 2026-01-09 R. J. G. Elbertse , M. Xu , A. Keşkekler , S. Otte , R. A. Norte

Electrically detected electron spin resonance (EDESR) signals were acquired as a function of temperature in the 0.3-4.2 K temperature range in a AlGaAs/GaAs multiple quantum well sample at the filling factor at 5.7 T. In the particular…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Eugene Olshanetsky , Manyam Pilla , Joshua D. Caldwell , Shu-chen Liu , Clifford R. Bowers , Jerry A. Simmons , John L. Reno

Combining electron paramagnetic resonance (EPR) with scanning tunneling microscopy (STM) enables detailed insight into the interactions and magnetic properties of single atoms on surfaces. A requirement for EPR-STM is the efficient coupling…

Mesoscale and Nanoscale Physics · Physics 2020-01-15 T. S. Seifert , S. Kovarik , C. Nistor , L. Persichetti , S. Stepanow , P. Gambardella

Magnetic nanoparticles (MNPs) have excellent magnetic-temperature characteristic. However, current temperature measurement based on MNPs is interfered by concentration. Utilizing the electron spin resonance (ESR), we propose a highly…

Mesoscale and Nanoscale Physics · Physics 2021-08-25 Shuai Wang , Jing Zhong , Wenzhong Liu

We propose a model to account for the observed ESR-like signal at the Larmor frequency in the current noise STM experiments identifying spin centers on various substrates. The theoretical understanding of this phenomenon, which allows for…

Mesoscale and Nanoscale Physics · Physics 2014-02-19 Alvaro Caso , Baruch Horovitz , Liliana Arrachea

Spin resonance of single spin centers bears great potential for chemical structure analysis, quantum sensing and quantum coherent manipulation. Essential for these experiments is the presence of a two-level spin system whose energy…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Philip Willke , Aparajita Singha , Xue Zhang , Taner Esat , Christopher P. Lutz , Andreas J. Heinrich , Taeyoung Choi

Understanding and controlling decoherence in open quantum systems is of fundamental interest in science, while achieving long coherence times is critical for quantum information processing. Although great progress was made for individual,…

Mesoscale and Nanoscale Physics · Physics 2023-03-23 Lisanne Sellies , Raffael Spachtholz , Philipp Scheuerer , Jascha Repp

Electron-spin resonance carried out with scanning tunneling microscopes (ESR-STM) is a recently developed experimental technique that is attracting enormous interest on account of its potential to carry out single-spin on-surface resonance…

Mesoscale and Nanoscale Physics · Physics 2023-04-19 Santiago A. Rodríguez , Sergio S. Gómez , Joaquín Fernández-Rossier , Alejandro Ferrón

A light-beam-assisted temperature-control system operating within a temperature range from 77 to 180 K is developed for investigating the absorption of electromagnetic waves by high-temperature superconductors in the vicinity of…

Superconductivity · Physics 2019-08-17 M. K. Aliev , G. R. Alimov , I. Kholbaev , T. M. Muminov , B. Olimov , B. Yu. Sokolov , R. R. Usmanov

Atomic-resolution cryogenic scanning transmission electron microscopy (cryo-STEM) has provided a path to probing the microscopic nature of select low-temperature phases in quantum materials. Expanding cryo-STEM techniques to broadly tunable…

Applied Physics · Physics 2020-11-05 Berit H. Goodge , Elisabeth Bianco , Henny W. Zandbergen Lena F. Kourkoutis

We used electron spin resonance (ESR) combined with scanning tunneling microscopy (STM) to measure hydrogenated Ti (spin-1/2) atoms at low-symmetry binding sites on MgO in vector magnetic fields. We found strongly anisotropic g-values in…

The integration of scanning tunneling microscopy (STM) and electron spin resonance (ESR) spectroscopy has emerged as a powerful and innovative tool for discerning spin excitations and spin-spin interactions within atoms and molecules…

Mesoscale and Nanoscale Physics · Physics 2024-11-04 Lyuzhou Ye , Xiao Zheng , Xin Xu
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