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We describe vacuum fluctuations and photon-field correlations in interacting quantum mechanical light-matter systems, by generalizing the application of mixed quantum-classical dynamics techniques. We employ the multi-trajectory…

Quantum Physics · Physics 2019-06-26 Norah M. Hoffmann , Christian Schäfer , Angel Rubio , Aaron Kelly , Heiko Appel

This paper focuses on investigating high-order harmonic generation (HHG) in graphene quantum dots (GQDs) under intense near-infrared laser fields. To model the GQD and its interaction with the laser field, we utilize a mean-field approach.…

Mesoscale and Nanoscale Physics · Physics 2023-09-15 H. K. Avetissian , A. G. Ghazaryan , Kh. V. Sedrakian , G. F. Mkrtchian

The use of energy conservation arguments is ubiquitous in understanding the process of high harmonic generation, yet a complete quantum optical description of exact photon number exchange remained elusive. Here, we solve this gap in…

Quantum Physics · Physics 2026-03-24 Philipp Stammer

The dynamics of an electronic system interacting with an electromagnetic field is investigated within mixed quantum-classical theory. Beyond the classical path approximation (where we ignore all feedback from the electronic system on the…

Chemical Physics · Physics 2019-02-11 Hsing-Ta Chen , Tao E. Li , Maxim Sukharev , Abraham Nitzan , Joseph E. Subotnik

We present a theoretical study of high-order harmonic generation (HHG) driven by ultrashort optical pulses with different kind of chirps. The goal of the present work is perform a detailed study to clarify the relevant parameters in the…

Atomic Physics · Physics 2016-12-21 E Neyra , F Videla , J A Pérez-Hernández , M F Ciappina , L Roso , G A Torchia

We investigate the high harmonic generation (HHG) in solids driven by laser fields with different ellipticities. The HHG spectra show a two-plateau structure within the energy gap between the valence band and the first conduction band.…

Optics · Physics 2018-06-01 Liang Li , Pengfei Lan , Xiaosong Zhu , Tengfei Huang , Peixiang Lu

Processes involving ultrafast laser driven electron-phonon dynamics play a fundamental role in the response of quantum systems in a growing number of situations of interest, as evidenced by phenomena such as strongly driven phase…

Materials Science · Physics 2024-03-01 Kevin Lively , Shunsuke A. Sato , Guillermo Albareda , Angel Rubio , Aaron Kelly

Contrary to common belief, the current emitted by a contact embedded in a two-dimensional electron gas (2DEG) is quantized in the presence of electric and magnetic fields. This observation suggests a simple, clearly defined model for the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Tobias Kramer

Quantum path interferences or resonances in multilevel dissipative quantum systems play an important and intriguing role in the transport processes of nanoscale systems. Many previous minimalistic models used to describe the quantum path…

Quantum Physics · Physics 2013-10-22 Xin Chen

The extreme nonlinear optical process of high-harmonic generation (HHG) makes it possible to map the properties of a laser beam onto a radiating electron wavefunction, and in turn, onto the emitted x-ray light. Bright HHG beams typically…

Strong field driven electric currents in condensed matter systems open new frontiers in petahertz electronics. In this regime new challenges arise as the role of the band structure and the quantum nature of electron-hole dynamics have yet…

We perform a detailed analysis of high-order harmonic generation in diatomic molecules within the strong-field approximation, with emphasis on quantum-interference effects. Specifically, we investigate how the different types of electron…

Atomic Physics · Physics 2011-11-10 C. Figueira de Morisson Faria

High harmonic generation (HHG) in solids reflects the underlying nonperturbative nonlinear dynamics of electrons in a strong light field and is a powerful tool for ultrafast spectroscopy of electronic structures. Photo-carrier doping allows…

Recent advancements in the generation of mid-infrared and terahertz laser pulses have enabled us to observe strong-field driven non-perturbative high-harmonic generation (HHG) from semiconductors, dielectrics, and semimetals. HHG has added…

Optics · Physics 2022-03-22 M. S. Mrudul

Ehrenfest dynamics is a useful approximation for ab initio mixed quantum-classical molecular dynamics that can treat electronically nonadiabatic effects. Although a severe approximation to the exact solution of the molecular time-dependent…

Chemical Physics · Physics 2021-09-24 Seonghoon Choi , Jiří Vaníček

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

Atomic Physics · Physics 2018-05-18 Peter Mulholland , Daniel Dundas

The long standing issue of separating resonant from non-resonant processes in extreme nonlinear optics is resolved. The theoretical formalism is applied to high harmonic generation (HHG) in solids and reveals a deeper view into the dominant…

Optics · Physics 2022-06-03 A. Thorpe , N. Boroumand , A. M. Parks , E. Goulielmakis , T. Brabec

A theoretical model for high-order harmonic generation (HHG) in bulk solids is considered. Our approach treats laser-induced inter- and intraband currents on an equal footing. The sum of these currents is the source of the high-order…

Quantum Physics · Physics 2017-07-12 Peter Foldi

High order harmonic generation by extremely intense, interacting, electromagnetic waves in the quantum vacuum is investigated within the framework of the Heisenberg-Euler formalism. Two intersecting plane waves of finite duration are…

High Energy Physics - Theory · Physics 2021-10-27 Pavel Sasorov , Francesco Pegoraro , Timur Esirkepov , Sergei Bulanov

We present theoretical investigations of high-order harmonic generation (HHG) resulting from the interaction of noble gases with localized surface plasmons. These plasmonic fields are produced when a metal nanoparticle is subject to a…