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Bimetallic catalysts provide new routes toward sustainable ammonia synthesis, but the structural dynamics controlling their performance under real-world conditions remain poorly understood. Here, we combine in situ gas-cell and multimodal…

Alloys present the great potential in catalysis because of their adjustable compositions, structures and element distributions, which unfortunately also limit the fast screening of the potential alloy catalysts. Machine learning methods are…

Materials Science · Physics 2021-07-07 Xin Li , Bo Li , Zhiwen Chen , Wang Gao , Qing Jiang

Oxide-supported single-atom catalysts are commonly modelled as a metal atom substituting surface cation sites in a low-index surface. Adatoms with dangling bonds will inevitably coordinate molecules from the gas phase, and adsorbates such…

M-N-C single-atom catalysts (SACs) have emerged as a potential substitute for the costly platinum-group catalysts in oxygen reduction reaction (ORR). However, several critical aspects of M-N-C SACs in ORR remain poorly understood, including…

Chemical Physics · Physics 2023-12-27 Di Zhang , Zhuyu Wang , Fangzhou Liu , Peiyun Yi , Linfa Peng , Yuan Chen , Li Wei , Hao Li

It has long been anticipated that the ultimate in miniature circuitry will be crafted of single atoms. Despite many advances made in scanned probe microscopy studies of molecules and atoms on surfaces, challenges with patterning and limited…

Ultracold atoms are crucial for unlocking truly precise and accurate quantum metrology, and provide an essential platform for quantum computing, communication and memories. One of the largest ongoing challenges is the miniaturization of…

Quantum Gases · Physics 2025-01-06 Alan Bregazzi , James P. McGilligan , Paul F. Griffin , Erling Riis , Aidan S. Arnold

Silanization bases on the adsorption, selfassembly and covalent binding of silane molecules onto surfaces, resulting in a densely packed self-assembled monolayer (SAM). Following standard recipes, however, the quality of the monolayer is…

Single atom catalysts (SACs) based on 2D materials are identified to be efficient in many catalytic reaction. In this work, the catalytic performance of Pd/Pt embedded planar carbon nitride (CN) for CO oxidation, has been investigated via…

Chemical Physics · Physics 2020-01-08 Yongchao Rao , Xiangmei Duan

Trapped atoms near nanophotonics form an exciting platform for bottom-up synthesis of strongly interacting quantum matter. The ability to induce tunable long-range atom-atom interactions with photons presents an opportunity to explore…

Quantum Physics · Physics 2019-04-12 May E. Kim , Tzu-Han Chang , Brian M. Fields , Cheng-An Chen , Chen-Lung Hung

Electrode-potential-induced dynamic coordination is an essential factor governing the performance of graphene-embedded single-atom catalysts (SACs). While previous studies have primarily centered on structural dynamics at the metal site,…

Materials Science · Physics 2026-02-05 Jiahang Li , Suhang Li , Chong Yan , Qinzhuang Liu , Jiajun Yu , Dongwei Ma

A new theoretical approach to 1:1 electrolytes at low temperature is developed, RPM and SAPM are studied with this approach, and their critical points of first order phase transition are calculated. The result is in very good agreement with…

Soft Condensed Matter · Physics 2007-05-23 Weimin Zhou , Jerome K. Percus

Chemical reactions typically proceed via stochastic encounters between reactants. Going beyond this paradigm, we combine exactly two atoms into a single, controlled reaction. The experimental apparatus traps two individual laser-cooled…

Atomic Physics · Physics 2018-04-25 L. R. Liu , J. D. Hood , Y. Yu , J. T. Zhang , N. R. Hutzler , T. Rosenband , K. -K. Ni

Sodium-ion batteries (SIBs) share similar electrochemistry with Li but offer several advantages, including high abundance in nature and low cost, as well as suitability for fast charging due to a Na-ion mobility higher than that of Li. The…

Materials Science · Physics 2026-05-27 Suchona Akter , Mohammad R. Momeni

Single dopant atoms or dopant-related defect centers in a solid state matrix provide an attractive platform for quantum simulation of topological states, for quantum computing and communication, due to their potential to realize a scalable…

Nanoparticles (NPs) make for intriguing heterogeneous catalysts due to their large active surface area and excellent and often size-dependent catalytic properties that emerge from a multitude of chemically different surface reaction sites.…

We show that single-atoms can be trapped on the surface of a subwavelength-diameter silica-fiber, an optical nanofiber, without any external field, and that single photons spontaneously emitted from the atoms can be readily detected through…

Quantum Physics · Physics 2009-11-13 K. P. Nayak , K. Hakuta

Unlocking the design of Li-S batteries where no shuttle effects appears, and thus their energy storage capacity does not diminish over time, would enable the manufacturing of energy storage devices more performant than the current Li-ion…

Materials Science · Physics 2022-06-22 Eleftherios I. Andritsos , Kevin Rossi

Designing a thin film structure often begins with choosing a film deposition method that employs a specific primary process by which chemical species are formed and transported. In other words, a film deposition system in which two…

Applied Physics · Physics 2020-07-31 Brian Giraldo , David M. Fryauf , Brandon Cheney , Nobuhiko P. Kobayashi

On-surface synthesis (OSS) involving relatively high energy barriers remains challenging due to a typical dilemma: firm molecular anchor is required to prevent molecular desorption upon the reaction, whereas sufficient lateral mobility is…

Optical tweezers have become essential tools to manipulate atoms or molecules at a single particle level. However, using standard diffracted-limited optical systems, the transverse size of the trap is lower bounded by the optical…