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Searching for an accurate optical clock which can serve as a better time standard than the present day atomic clock is highly demanding from several areas of science and technology. Several attempts have been made to built more accurate…

Atomic Physics · Physics 2007-09-17 Chiranjib Sur , Rajat K Chaudhuri

Frequency shifts of the ^199Hg^+ 5d^10 6s ^2S_1/2 (F=0, M_F=0) to 5d^9 6s^2 ^2D_5/2 (F=2, M_F=0) electric-quadrupole transition at 282 nm due to external fields are calculated, based on a combination of measured atomic parameters and ab…

Atomic Physics · Physics 2007-05-23 W. M. Itano

The $^{229}$Th nucleus has a unique transition at only 8 eV which could be used for a novel nuclear clock. We investigate theoretically the prospects of driving this transition with vortex light beams carrying orbital angular momentum.…

Atomic Physics · Physics 2024-04-22 Tobias Kirschbaum , Thorsten Schumm , Adriana Pálffy

Iridium ions near $4f$-$5s$ level crossings are the leading candidates for a new type of atomic clocks with a high projected accuracy and a very high sensitivity to the temporal variation of the fine structure constant $\alpha$. To identify…

Atomic Physics · Physics 2015-08-12 U. I. Safronova , V. V. Flambaum , M. S. Safronova

We perform calculations of the energy shift of the nuclear clock transition frequency $^{229}$Th as a function of the number of electrons in Th ion. We demonstrate that the dependence of the nuclear frequency on electron configuration is…

Atomic Physics · Physics 2024-05-21 V. A. Dzuba , V. V. Flambaum

A method for highly accurate calculations of atomic electric quadrupole moments (EQM) is presented, using relativistic general-excitation-rank configuration interaction wavefunctions based on Dirac spinors. Application to the clock…

Atomic Physics · Physics 2023-02-06 Timo Fleig

Thorium-229, with its exceptionally low-energy nuclear excited state, is a key candidate for developing nuclear clocks. $^{229}$Th-doped CaF$_2$ crystals, benefiting from calcium fluoride's wide band gap, show great promise as solid-state…

We study the Ho$^{14+}$ ion as a candidate for extremely accurate and stable optical atomic clock which is sensitive to the time variation of the fine structure constant. We demonstrate that the proposed system has all desired features…

Atomic Physics · Physics 2015-03-05 V. A. Dzuba , V. V. Flambaum , Hidetoshi Katori

We have produced laser-cooled Wigner crystals of 229Th3+ in a linear Paul trap. The magnetic dipole (A) and electric quadrupole (B) hyperfine constants for four low-lying electronic levels and the relative isotope shifts with respect to…

Atomic Physics · Physics 2011-10-12 C. J. Campbell , A. G. Radnaev , A. Kuzmich

We have completed a new measurement of the Stark shift in 115In within the 410 nm 5P1/2- 6S1/2 transition. We measure the Stark shift constant to be kS= - 122.92(33)kHz/(kV/cm)^2, corresponding to a difference in the 6S1/2 and 5P1/2 state…

Atomic Physics · Physics 2015-06-12 G. Ranjit , N. A. Schine , A. T. Lorenzo , A. E. Schneider , P. K. Majumder

We describe a transportable optical lattice clock based on the $^1\mathrm{S}_0 \rightarrow {^3\mathrm{P}_0}$ transition of lattice-trapped $^{87}$Sr atoms with a total systematic uncertainty of $2.1 \times 10^{-18}$. The blackbody radiation…

Atomic Physics · Physics 2025-07-21 I. Nosske , C. Vishwakarma , T. Lücke , J. Rahm , N. Poudel , S. Weyers , E. Benkler , S. Dörscher , C. Lisdat

The isotope $^{229}$Th is the only nucleus known to possess an excited state $^{229m}$Th in the energy range of a few electron volts, a transition energy typical for electrons in the valence shell of atoms, but about four orders of…

We report the results of a direct search for the $^{229}$Th ($I^{p} = 3/2^+\leftarrow 5/2^+$) nuclear isomeric transition, performed by exposing $^{229}$Th-doped LiSrAlF$_6$ crystals to tunable vacuum-ultraviolet synchrotron radiation and…

Dielectric spectroscopy of $SrTiO_3$ single crystal over a broad range of microwave frequency using quasi $TE_{m,1,1}$ and quasi $TM_{m,1,1}$ modes reveals crystal asymmetry from typical measurement of $Q$-factor, transmission or frequency…

Materials Science · Physics 2025-05-22 M. A. Hosain , J-M. Le Floch , J. F. Bourhill , J. Krupka , M. E. Tobar

We present a novel method for engineering an optical clock transition that is robust against external field fluctuations and is able to overcome limits resulting from field inhomogeneities. The technique is based on the application of…

Atomic Physics · Physics 2019-12-03 Nati Aharon , Nicolas Spethmann , Ian D. Leroux , Piet O. Schmidt , Alex Retzker

We use advanced computational techniques to study the electronic structure of the Hf$^{12+}$ ion, with the goal of assessing its potential for use in highly accurate atomic optical clocks and search for new physics. Such clocks should…

Atomic Physics · Physics 2025-11-04 Saleh O. Allehabi , V. A. Dzuba , V. V. Flambaum

Extra-laboratory atomic clocks are necessary for a wide array of applications (e.g. satellite-based navigation and communication). Building upon existing vapor cell and laser technologies, we describe an optical atomic clock, designed…

The isomeric first excited state of the isotope 229Th exhibits the lowest nuclear excitation energy in the whole landscape of known atomic nuclei. For a long time this energy was reported in the literature as 3.5(5) eV, however, a new…

Nuclear Experiment · Physics 2015-06-12 L. v. d. Wense , P. G. Thirolf , D. Kalb , M. Laatiaoui

We identify Ba$^{4+}$ (Te-like) as a promising candidate for a high-accuracy optical clock. The lowest-lying electronic states are part of a $^3P_J$ fine structure manifold with anomalous energy ordering, being non-monotonic in $J$. We…

Atomic Physics · Physics 2020-10-26 Kyle Beloy , Vladimir A. Dzuba , Samuel M. Brewer

In this work, the $4D_{3/2}|3,\pm2\rangle \rightarrow 4D_{5/2}|3,\pm2\rangle$ transition in the Nb$^{4+}$ ion is identified as a promising candidate for a terahertz (THz) atomic clock, with the transition frequency occurring at 56.0224 THz.…

Atomic Physics · Physics 2025-04-23 Jyoti , A. Chakraborty , Zhiyang Wang , Jia Zhang , Jingbiao Chen , Bindiya Arora , B. K. Sahoo