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Atomically-thin films of phosphorene (also known as black phosphorus) are a low dimensional optical material with direct exciton emission, whose wavelength is tunable by controlling the number of layers. In addition to this excitonic…

Mesoscale and Nanoscale Physics · Physics 2017-07-03 Shahriar Aghaeimeibodi , Je-Hyung Kim , Edo Waks

Artificial monolayer black phosphorus, the so-called phosphorene has attracted global interest with its distinguished anisotropic optoelectronic and electronic properties. Here, we unraveled the shear-induced direct to indirect gap…

Materials Science · Physics 2015-05-14 Baisheng Sa , Yan-Ling Li , Zhimei Sun , Jingshan Qi , Cuilian Wen , Bo Wu

Phosphorene has been attracted intense interest due to its unexpected high carrier mobility and distinguished anisotropic optoelectronic and electronic properties. In this work, we unraveled strain engineered phosphorene as a photocatalyst…

Materials Science · Physics 2014-11-25 Baisheng Sa , Yan-Ling Li , Jingshan Qi , Rajeev Ahuja , Zhimei Sun

Group-V elemental monolayers including phosphorene are emerging as promising 2D materials with semiconducting electronic properties. Here, we present the results of first principles calculations on stability, mechanical and electronic…

Computational Physics · Physics 2015-05-12 Gaoxue Wang , Ravindra Pandey , Shashi P. Karna

We report that two rotated layers of blue phosphorene behave as a direct band gap semiconductor. The optical spectrum shows absorption peaks in the visible region of the spectrum and in addition the energy of these peaks can be tuned with…

Mesoscale and Nanoscale Physics · Physics 2016-08-01 D. A. Ospina , C. A. Duque , J. D. Correa , Eric Suárez Morell

In this article, we explore the anisotropic electron energy loss spectrum (EELS) in monolayer phosphorene based on ab-initio time dependent density functional theory calculations. Similar to black phosphorous, the EELS of undoped monolayer…

Mesoscale and Nanoscale Physics · Physics 2017-07-26 Barun Ghosh , Piyush Kumar , Anmol Thakur , Yogesh Singh Chauhan , Somnath Bhowmick , Amit Agarwal

The prospects of phosphorene as an anode material for high performance Li-ion battery was systematically investigated from the first principle calculations and experimental measurements. The diffusion energy barriers of a Li atom moving…

Materials Science · Physics 2016-07-04 Congyan Zhang , George Anderson , Ruchira Ravinath Dharmasena , Gamini Sumanasekera , Ming Yu

We investigate the spontaneous emission lifetime of a quantum emitter near a substrate coated with phosphorene under the influence of uniaxial strain. We consider both electric dipole and magnetic dipole-mediated spontaneous transitions…

Mesoscale and Nanoscale Physics · Physics 2023-10-30 P. P. Abrantes , W. J. M. Kort-Kamp , F. S. S. Rosa , C. Farina , F. A. Pinheiro , Tarik P. Cysne

We present a paradigm in constructing very stable, faceted nanotube and fullerene structures by laterally joining nanoribbons or patches of different planar phosphorene phases. Our ab initio density functional calculations indicate that…

Materials Science · Physics 2015-06-23 Jie Guan , Zhen Zhu , David Tománek

We investigate two dimensional monolayer structures of arsenic phosphorus ( AsP) by means of first principles plane wave method within density functional theory using the generalized gradient approximation. Two structures of arsenic…

Materials Science · Physics 2016-09-30 Zhaleh Benam , Handan Arkin , Ethem Akturk

Using the first-principles GW-Bethe-Salpeter equation method, here we study the excited-state properties, including quasi-particle band structures and optical spectra, of phosphorene, a two-dimensional (2D) atomic layer of black phosphorus.…

Materials Science · Physics 2015-07-28 Vellayappan Dheivanayagam S/O Ganesan , Chun Zhang , Yuan Ping Feng , Lei Shen

Few-layer black phosphorus (BP), also known as phosphorene, is poised to be the most attractive graphene analogue owing to its high mobility approaching that of graphene, and its thickness- tunable band gap that can be as large as that of…

Materials Science · Physics 2015-03-13 Joon-Seok Kim , Yingnan Liu , Weinan Zhu , Seohee Kim , Di Wu , Li Tao , Ananth Dodabalapur , Keji Lai , Deji Akinwande

Due to the relatively low formation energies and highly mobile characteristics of atomic vacancies in phosphorene, understanding their evolutions becomes crucial for its structural integrity, chemical activities and applications. Herein, by…

Materials Science · Physics 2019-10-10 Yongqing Cai , Shuai Chen , Junfeng Gao , Gang Zhang , Yong-Wei Zhang

By taking account of the electric-field-induced charge screening, a self-consistent calculation within the framework of the tight-binding approach is employed to obtain the electronic band structure of gated multilayer phosphorene and the…

Mesoscale and Nanoscale Physics · Physics 2018-05-09 L. L. Li , B. Partoens , F. M. Peeters

We explore the oxidation of a single layer of black phosphorous using ab initio density functional theory calculation. We search for the equilibrium structures of phosphorene oxides, PO$_x$ with various oxygen concentrations $x$…

Materials Science · Physics 2020-07-22 Seoung-Hun Kang , Jejune Park , Sungjong Woo , Young-Kyun Kwon

Black phosphorous is a layered material having a high capacity of 2596 mAh/g as a battery electrode, however it suffers from cracking due to high volume expansion during lithiation. These cracks causes loss of electrical contact in the…

Materials Science · Physics 2020-07-21 Burak Ozdemir

In this work, we provide a detailed analysis of phosphorene performance as n-type and p-type active materials. The study is based on first principles calculation of phosphorene electronic structure, and resulting electron and hole…

Materials Science · Physics 2016-11-09 Eric Tea , Celine Hin

We investigate the electronic and optical properties of monolayer and stacking dependent bilayer blue phosphorus in the framework of density functional theory (DFT) and tight-binding approximations. We extract the hopping parameters of TB…

Mesoscale and Nanoscale Physics · Physics 2016-07-27 Y. Mogulkoc , M. Modarresi , A. Mogulkoc , Y. O. Ciftci

We report the quasiparticle band gap, excitons, and highly anisotropic optical responses of few-layer black phosphorous (phosphorene). It is shown that these new materials exhibit unique many-electron effects; the electronic structures are…

Mesoscale and Nanoscale Physics · Physics 2014-06-27 Vy Tran , Ryan Soklaski , Yufeng Liang , Li Yang

Monolayer and few-layer phosphorene are anisotropic quasi-two-dimensional (quasi-2D) van der Waals (vdW) semiconductors with a linear-dichroic light-matter interaction and a widely-tunable direct-band gap in the infrared frequency range.…