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We present a theory of tunneling and resonant transitions in one-dimensional molecular systems which is based on Green's function theory of electron sub-barrier scattering off the structural units (or functional groups) of a molecular…

Other Condensed Matter · Physics 2007-05-23 I. I. Oleynik , M. A. Kozhushner , V. S. Posvyanskii

We have used the method of generating functional in imaginary time to derive the current-voltage characteristics of a tunnel junction with arbitrary tunneling conductance, connected in series with an external impedance and a voltage source.…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 X. H. Wang , K. A. Chao

Accurate electrical amplification is essential in molecular electronics for measuring conductance through atomic and molecular junctions, where currents often span several orders of magnitude. In this work, we present a systematic design…

Mesoscale and Nanoscale Physics · Physics 2026-04-20 J. Escorza , G. Pellicer , T. de Ara , J. Hurtado-Gallego , E. Scheer , C. Untiedt , C. Sabater

The dynamics of a molecular junction consisting of a PTCDA molecule between the tip of a scanning tunneling microscope and a Ag(111) surface have been investigated experimentally and theoretically. Repeated switching of a PTCDA molecule…

Understanding of charge transport mechanisms in nanoscale structures is essential for the development of molecular electronic devices. Charge transport through 1D molecular systems connected between two contacts is influenced by several…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Daijiro Nozaki , Horacio M. Pastawski , Gianaurelio Cuniberti

We develope a model to describe the transmission coefficient and tunneling current in the presence of photon-electron coupling in a resonant diode. Our model takes into account multiphoton processes as well as the transitions between…

Condensed Matter · Physics 2019-08-17 Jesus Inarrea , Ramon Aguado , Gloria Platero

The conductance of a molecular junction is commonly determined by either charge-transfer-doping, where alignment of the Fermi energy to the molecular levels is achieved, or tunnelling through the tails of molecular resonances within the…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 R. Gutierrez , G. Fagas , K. Richter , F. Grossmann , R. Schmidt

Understanding the properties of electronic transport across metal-molecule interfaces is of central importance for controlling a large variety of molecular-based devices such as organic light emitting diodes, nanoscale organic spin-valves…

Mesoscale and Nanoscale Physics · Physics 2016-02-03 T. Yelin , R. Korytar , N. Sukenik , R. Vardimon , B. Kumar , C. Nuckolls , F. Evers , O. Tal

In most electronic devices, electric current of both types (electrons and holes) flows through a junction. Usually the boundary conditions have been formulated exclusively for open circuit. The boundary conditions proposed here bypass this…

Materials Science · Physics 2009-11-07 O. Yu. Titov , J. Giraldo , Yu. G. Gurevich

How dissipation affects transport is an important theme in quantum science. Here we theoretically investigate an impact of a single-particle loss in mesoscopic transport, which has been an issue in experiments of ultracold atomic gases. By…

Quantum Gases · Physics 2023-07-07 Shun Uchino

We study heat conduction in a one-dimensional chain of particles with longitudinal as well as transverse motions. The particles are connected by two-dimensional harmonic springs together with bending angle interactions. The problem is…

Statistical Mechanics · Physics 2009-11-10 Jian-Sheng Wang , Baowen Li

We measure the low bias conductance of a series of substituted benzene diamine molecules while breaking a gold point contact in a solution of the molecules. Transport through these substituted benzenes is by means of nonresonant tunneling…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Latha Venkataraman , Young S. Park , Adam C. Whalley Colin Nuckolls , Mark S. Hybertsen , Michael L. Steigerwald

Various causes for negative differential conductance in transport through an interacting double quantum dot are investigated. Particular focus is given to the interplay between the renormalization of the energy levels due to the coupling to…

Mesoscale and Nanoscale Physics · Physics 2011-11-09 Jonas Nyvold Pedersen , Benny Lassen , Andreas Wacker , Matthias H. Hettler

A 1D model study of charge transport in nano-devices is made by comparing multi-configuration time dependent Hartree-Fock and frozen core calculations. The influence of exchange and Coulomb correlation on the tunneling current is…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Zhongxi Zhang , C. F. Destefani , Chris McDonald , Thomas Brabec

For defining the conductance of single molecule junctions with a redox functionality in an electrochemical cell, two conceptually different electron transport mechanisms, namely coherent tunnelling and vibrationally induced hopping compete…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Georg Kastlunger , Robert Stadler

We review data analysis techniques that can be used to study temporal correlations among conductance traces in break junction measurements. We show that temporal histograms are a simple but efficient tool to check the temporal homogeneity…

Mesoscale and Nanoscale Physics · Physics 2017-03-08 A. Magyarkuti , K. P. Lauritzen , Z. Balogh , A. Nyáry , G. Mészáros , P. Makk , G. C. Solomon , A. Halbritter

We demonstrate that a simple phenomenological approach can be used to simulate electronic conduction in molecular wires under thermal effects induced by the surrounding environment. This "Landauer-B\"uttiker's probe technique" can properly…

Chemical Physics · Physics 2015-08-25 Michael Kilgour , Dvira Segal

Scanning tunneling miscoscopy is one of the most powerful spectroscopic tools for single-electron excitations. We show that the conductance fluctuations, or noise in the conductance, of a tunneling current into an interacting electron…

Strongly Correlated Electrons · Physics 2009-02-03 Kelly R. Patton , Hartmut Hafermann , Sergej Brener , Alexander I. Lichtenstein , Mikhail I. Katsnelson

Transport through molecular contacts with a sluggish intramolecular vibrational mode strongly coupled to excess charges is studied far from equilibrium. A Born-Oppenheimer approximation in steady state reveals voltage dependent energy…

Mesoscale and Nanoscale Physics · Physics 2012-06-27 Lars Kecke , Joachim Ankerhold