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We study nonlinear interactions in a strongly driven optomechanical cavity, in regimes where the interactions give rise to resonant scattering between optomechanical polaritons and are thus strongly enhanced. We use a Keldysh formulation…

Quantum Physics · Physics 2015-06-30 Marc-Antoine Lemonde , Aashish A. Clerk

The observation that materials can change their properties when placed inside or near an optical resonator, has sparked a fervid interest in understanding the effects of strong light-matter coupling on molecular dynamics, and several…

Chemical Physics · Physics 2024-03-20 Ilia Sokolovskii , Gerrit Groenhof

We show how to simulate a model of many molecules with both strong coupling to many vibrational modes and collective coupling to a single photon mode. We do this by combining process tensor matrix product operator methods with a mean-field…

Quantum Gases · Physics 2022-10-24 Piper Fowler-Wright , Brendon W. Lovett , Jonathan Keeling

This is a tutorial-style introduction to the field of molecular polaritons. We describe the basic physical principles and consequences of strong light-matter coupling common to molecular ensembles embedded in UV-visible or infrared…

Chemical Physics · Physics 2020-03-18 Felipe Herrera , Jeffrey Owrutsky

We derive the transition rates, dephasing rates, and Lamb shifts for a system consisting of many molecules collectively coupled to a resonant cavity mode. Using a variational polaron master equation, we show that strong vibrational…

Quantum Physics · Physics 2024-07-24 Dominic M Rouse , Erik M Gauger , Brendon W Lovett

Polaritons are quantum mechanical superpositions of photon states with elementary excitations in molecules and solids. The light-matter admixture causes a characteristic frequency-momentum dispersion shared by all polaritons irrespective of…

Third order anharmonic scattering in light-matter systems can drive a wide variety of practical and physically interesting processes from lasing to polariton condensation. Motivated by recent experimental results in the nonlinear optics of…

Mesoscale and Nanoscale Physics · Physics 2017-11-06 Christopher R. Gubbin , Simone De Liberato

We consider the scenario of excitons in a semiconductor bilayer that are strongly coupled to cavity photons, leading to the formation of dipolar exciton polaritons (dipolaritons). Using a realistic pseudopotential for the dipolar…

Mesoscale and Nanoscale Physics · Physics 2026-02-27 Yasufumi Nakano , Olivier Bleu , Brendan C. Mulkerin , Jesper Levinsen , Meera M. Parish

Organic microcavities are photonic nanostructures that strongly confine the electromagnetic field, allowing exotic quantum regimes of light-matter interaction with disordered organic semiconductors. The unambiguous interpretation of the…

Quantum Physics · Physics 2017-06-07 Felipe Herrera , Frank C. Spano

Integrated photonics has been a promising platform for analog quantum simulation of condensed matter phenomena in strongly correlated systems. To that end, we explore the implementation of all-photonic quantum simulators in coupled cavity…

Polaritons are quasiparticles arising from the strong coupling of electromagnetic waves in cavities and dipolar oscillations in a material medium. In this framework, localized surface plasmon in metallic nanoparticles defining optical…

We study a hybrid semiconductor-optomechanical system, which consists of a cavity with an oscillating mirror made by semiconducting materials or with a semiconducting membrane inside. The cavity photons and the excitons in the oscillating…

Quantum Physics · Physics 2018-10-03 Sai-Nan Huai , Yu-Long Liu , Yunbo Zhang , Yu-xi Liu

We study theoretically the quantum dynamics and spectroscopy of rovibrational polaritons formed in a model system composed of a single rovibrating diatomic molecule, which interacts with two degenerate, orthogonally polarized modes of an…

Chemical Physics · Physics 2023-01-11 Eric W. Fischer , Peter Saalfrank

Molecular polaritons have gained considerable attention due to their potential to control nanoscale molecular processes by harnessing electromagnetic coherence. Although recent experiments with liquid-phase vibrational polaritons have shown…

Understanding the vibrational and thermal properties of amorphous solids is one of the most discussed and long-standing issues in condensed matter physics. Recent works have made significant steps towards understanding harmonic vibrational…

Soft Condensed Matter · Physics 2020-02-28 Hideyuki Mizuno , Masanari Shimada , Atsushi Ikeda

We calculate the intensity of the polariton mediated inelastic light scattering in semiconductor microcavities. We treat the exciton-photon coupling nonperturbatively and incorporate lifetime effects in both excitons and photons, and a…

Strongly Correlated Electrons · Physics 2008-05-04 L. M. Leon Hilario , A. Bruchhausen , A. M. Lobos , A. A. Aligia

We introduce a theory of chemical equilibrium in optical microcavities, which allows us to relate equilibrium reaction quotients in different electromagnetic environments. Our theory shows that in planar microcavities under strong coupling…

Chemical Physics · Physics 2023-05-02 Kaihong Sun , Raphael F. Ribeiro

Fabry-Perot microcavities can strongly enhance interactions between light and molecules, leading to the formation of hybrid light-matter states known as polaritons. Polaritons possess much smaller effective masses and much larger group…

Chemical Physics · Physics 2023-10-18 Zeyu Zhou , Hsing-Ta Chen , Maxim Sukharev , Joseph E. Subotnik , Abraham Nitzan

We demonstrate a macro-coherent regime in exciton-polariton systems, where nonequilibrium polariton Bose--Einstein condensation coexists with macroscopically occupied vibrational states. Strong exciton-vibration coupling induces an…

Intramolecular energy transfer driven by near-field effects plays an important role in applications ranging from biophysics and chemistry to nano-optics and quantum communications. Advances in strong light-matter coupling in molecular…

Mesoscale and Nanoscale Physics · Physics 2025-07-14 Kristin B. Arnardottir , Piper Fowler-Wright , Christos Tserkezis , Brendon W. Lovett , Jonathan Keeling