Related papers: Photon Antibunching in Single-Molecule Vibrational…
Second harmonic generation (SHG) is forbidden in centrosymmetric molecular materials. However, a signal is frequently observed from interfaces where the symmetry is broken. Whereas the effect can be phenomenologically accommodated, an ab…
Generating correlated photon pairs at the nanoscale is a prerequisite to creating highly integrated optoelectronic circuits that perform quantum computing tasks based on heralded single-photons. Here we demonstrate fulfilling this…
Experimental control and detection of atoms and molecules often rely on optical transitions between different electronic states. In many cases, substructure such as hyperfine or spin-rotation structure leads to the need for multiple optical…
The enhanced electric field at plasmonic resonances in nanoscale antennas can lead to efficient harmonic generation, especially when the plasmonic geometry is asymmetric on either inter-particle or intra-particle levels. The planar…
High harmonic generation traditionally combines ~100 near-infrared laser photons, to generate bright, phase matched, extreme ultraviolet beams when the emission from many atoms adds constructively. Here we show that by guiding a…
We demonstrate frequency-bin entanglement between ultra-narrowband photons generated by cavity enhanced spontaneous parametric down conversion. Our source generates photon pairs in widely non-degenerate discrete frequency modes, with one…
We study second and third harmonic generation in centrosymmetric semiconductors at visible and UV wavelengths in bulk and cavity environments. Second harmonic generation is due to a combination of symmetry breaking, the magnetic portion of…
An optical Second-Harmonic Generation (SHG) allows to probe various structural and symmetry-related properties of materials, since it is sensitive to the inversion symmetry breaking in the system. Here, we investigate the SHG response from…
The generation of photocurrents due to coupling of electrons to both classical and quantized electromagnetic fields in thin semiconductor films is described within the framework of the nonequilibrium Green's function formalism. For the…
For centrosymmetric materials such as monolayer graphene, no optical second harmonic generation (SHG) is generally expected because it is forbidden under the electric-dipole approximation. Yet we observed a strong, doping induced SHG from…
Scaling up a superconducting quantum computer will likely require quantum communication between remote chips, which can be implemented using an itinerant microwave photon in a transmission line. To realize high-fidelity communication, it is…
Since the new millennium coherent extreme ultra-violet and soft x-ray radiation has revolutionized the understanding of dynamical physical, chemical and biological systems at the electron's natural timescale. Unfortunately, coherent…
Nonclassical light sources, such as correlated photon-pairs, play an important role in quantum optics and quantum information processing systems. This study proposes a process to generate antibunched photon-pairs in a nondegenerate optical…
Multi-photon microscopy has played a significant role in biological imaging since it allows to observe living tissues with improved penetration depth and excellent sectioning effect. Multi-photon microscopy relies on multi-photon…
A monochromatic laser pumping a parametric down conversion crystal generates frequency entangled photon pairs. We study this experimentally by addressing such frequency entangled photons at telecommunication wavelengths (around 1550 nm)…
We report on the realization of a solid-state-based vacuum ultraviolet frequency comb, using multi-harmonic generation in an external enhancement cavity. Optical conversions in such arrangements were so-far reported only using gaseous…
Single-photon sources are in high demand for quantum information applications. A paradigmatic way to achieve single-photon emission is through anharmonicity in the energy levels, such that the absorption of a single photon from a coherent…
Adversarial waveform generation has been a popular approach as the backend of singing voice conversion (SVC) to generate high-quality singing audio. However, the instability of GAN also leads to other problems, such as pitch jitters and U/V…
Nonlinear second harmonic optical activity of graphene covering a gold photon sieve was determined for different polarizations. The photon sieve consists of a subwavelength gold nanohole array placed on glass. It combines the benefits of…
We investigate the quantum properties of the well-known process of sum frequency generation, showing that it is potentially a very useful source of non-classical states of the electromagnetic field, some of which are not possible with the…