Related papers: Multidimensional Terahertz Probes of Quantum Mater…
Coherent continuous wave (CW) terahertz spectroscopy is an extremely valuable technique that allows for the interrogation of systems that exhibit narrow resonances in the terahertz (THz) frequency range, such as high-quality (high-Q) THz…
"Single-shot" ultrafast spectroscopy based on the frequency encoding of transient absorbance kinetics using chirped probe pulses is analyzed theoretically. FDSS has an advantage over pump-probe spectroscopy in a situation where the "noise"…
Quantum phenomena are typically observable at length and time scales smaller than those of our everyday experience, often involving individual particles or excitations. The past few decades have seen a revolution in the ability to structure…
The discovery of graphene and its fascinating capabilities have triggered an unprecedented interest in inorganic two-dimensional (2D) materials. Van der Waals (vdW) layered materials as graphene, hexagonal boron nitride (hBN), transition…
The response of an ungated two-dimensional electron gas(2DEG) to an external electromagnetic excitation is analyzed. The possibility of creating a single-mode resonance detector operating in the terahertz frequency range is demonstrated.
The terahertz spectral regime, ranging from about 0.1 to 15 THz, is one of the least explored yet most technologically transformative spectral regions. One current challenge is to develop efficient and compact terahertz emitters/detectors…
Time-frequency duality, which enables control of optical waveforms by manipulating amplitudes and phases of electromagnetic fields, plays a pivotal role in a wide range of modern optics. The conventional one-dimensional (1D) time-frequency…
The field of quantum sensing explores the use of quantum phenomena to measure a broad range of physical quantities, of both static and time-dependent types. An important figure of merit for sensing time dependent signals is the spectral…
This tutorial aims to provide details on the underlying principles and methodologies of atom-based terahertz imaging techniques. Terahertz imaging is a growing field of research which can provide complementary information to techniques…
We describe methods using frequency combs and optical resonators for recording two-dimensional (2D) ultrafast spectroscopy signals with high sensitivity. By coupling multiple frequency combs to higher-order modes of one or more optical…
Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy…
Quantum devices made from van der Waals (vdW) heterostructures of two dimensional (2D) materials may herald a new frontier in designer materials that exhibit novel electronic properties and unusual electronic phases. However, due to the…
An apporach for the sensing of small amounts of chemical and biochemical material is presented. A frequency selective surface (FSS) made from asymmetric split ring resonators (aDSR) is excited with free space radiation. Due to interference…
Two-dimensional electronic spectroscopy (2DES) has enabled significant discoveries in both biological and synthetic energy-transducing systems. Although deriving chemical information from 2DES is a complex task, machine learning (ML) offers…
Protocols for processing of quantum information are the foundation of quantum technology, enabling to share secrets at a distance, teleport quantum states, and to implement quantum computation. While many protocols were realized, and even…
Recent interest in the role of quantum mechanics in the primary events of photosynthetic energy transfer has led to a convergence of nonlinear optical spectroscopy and quantum optics on the topic of energy-transfer dynamics in…
The anomalous low-temperature properties of glasses arise from intrinsic excitable entities, so-called tunneling Two-Level-Systems (TLS), whose microscopic nature has been baffling solid-state physicists for decades. TLS have become…
Quantum thermodynamics seeks to extend non-equilibrium stochastic thermodynamics to small quantum systems where non-classical features are essential to its description. Such a research area has recently provided meaningful theoretical and…
Triple sum-frequency (TSF) spectroscopy measures multidimensional spectra by resonantly exciting multiple quantum coherences of vibrational and electronic states. In this work we demonstrate pump-TSF-probe spectroscopy in which a pump…
The brightness of a light source defines its applicability to nonlinear phenomena in science. Bright low frequency terahertz (< 5THz) radiation confined to a diffraction-limited spot size is a present hurdle due to the broad bandwidth and…