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We measure the inter-modal phase relation of a quantum cascade laser frequency comb operating at 8 um using a coherent beatnote spectroscopy. We find these phases to be reproducible after cycling the power of the device, and to be smoothly…

Optics · Physics 2018-04-13 Matthew Singleton , Pierre Jouy , Mattias Beck , Jérôme Faist

Dual-comb spectroscopy allows for the rapid, multiplexed acquisition of high-resolution spectra without the need for moving parts or low-resolution dispersive optics. This method of broadband spectroscopy is most often accomplished via…

We report the measurement of sub-Doppler double-resonance transitions in methane using a 3.3 $\mu$m continuous wave optical parametric oscillator to pump transitions in the fundamental $\nu_3$ band and a 1.67 $\mu$m frequency comb to probe…

Low noise and high repetition rate optical frequency combs are desirable for many applications from timekeeping to precision spectroscopy. For example, gigahertz repetition rate sources greatly increase the acquisition speed of spectra in a…

We demonstrate a high-accuracy dual-comb spectrometer centered at 3.4 \mu m. The amplitude and phase spectra of the P, Q, and partial R-branch of the methane {\nu}3 band are measured at 25 MHz to 100 MHz point spacing with ~kHz resolution…

Optical frequency combs provide a phase-coherent interface between optical and microwave domains, underpinning advances in precision metrology, spectroscopy, and time-frequency transfer. Most conventional comb architectures are limited to…

Optical frequency combs [1-8] have resulted in significant advances in optical frequency metrology and found wide application to precise physical measurements [1-4, 9] and molecular fingerprinting [8]. A direct analogue of frequency combs…

Pattern Formation and Solitons · Physics 2017-01-25 Adarsh Ganesan , Cuong Do , Ashwin A. Seshia

Lithium niobate (LN) microring resonators, characterized by an exceptionally high second-order nonlinear coefficient and superior electro-optic tunability, serve as an outstanding platform for the precise control of integrated quantum…

We present detailed studies of the coherence properties of an ultra-broadband super-continuum, enabled by a new approach involving continuous wave laser sources to independently probe both the amplitude and phase noise quadratures across…

In recent years, microresonator-based optical frequency combs have created up opportunities for developing a spectroscopy laboratory on a chip due to its broadband emission and high comb power. However, with mode spacings typically in the…

Instrumentation and Detectors · Physics 2017-11-22 Mengjie Yu , Yoshitomo Okawachi , Austin G. Griffith , Michal Lipson , Alexander L. Gaeta

Magnetostriction, mechanical-to-magnetic or magnetic-to-mechanical response, plays a pivotal role in magneto-mechanical systems. Here, we propose and experimentally demonstrate a magneto-mechanical frequency comb via the three-wave mixing…

Strongly Correlated Electrons · Physics 2025-05-30 Guanqi Ye , Ruitong Sun , Junning Zhao , Fusheng Ma

Spectroscopy has attracted much attention in molecular detection, biomolecular identification, and chemical analysis for providing accurate measurement. However, it is almost unable to distinguish different sources with overlapped…

Instrumentation and Detectors · Physics 2020-05-12 Ting Qing , Shupeng Li , Yijie Fang , Xiaohu Tang , Lihan Wang , Meihui Cao , Xinyu Li , Shilong Pan

Superconductors are characterized by macroscopic phase coherence and have enabled cryogenic electronics and quantum technologies. Recent advances in 3D nanofabrication now offer possibilities for tuning functional properties relevant for…

Superconductivity · Physics 2025-03-26 Axel J. M. Deenen , Dirk Grundler

We demonstrate dual-comb spectroscopy based on difference frequency generation of frequency-agile near-infrared frequency combs, produced with the help of electro-optic modulators. The combs have a remarkably flat intensity distribution and…

Laser frequency combs are coherent light sources that emit a broad spectrum consisting of discrete, evenly spaced narrow lines, each having an absolute frequency measurable within the accuracy of an atomic clock. Their development, a decade…

Optics · Physics 2017-06-13 Albert Schliesser , Nathalie Picqué , Theodor W. Hänsch

Molecular spectroscopy in the mid-infrared portion of the electromagnetic spectrum (3--25 um) has been a cornerstone interdisciplinary analytical technique widely adapted across the biological, chemical, and physical sciences. Applications…

Instrumentation and Detectors · Physics 2018-09-18 Abijith S. Kowligy , Henry Timmers , Alex Lind , Ugaitz Elu , Flavio C. Cruz , Peter G. Schunemann , Jens Biegert , Scott A. Diddams

Chip-based optical frequency combs address the demand for compact, bright, coherent light sources of equidistant phase-locked lines. Traditionally, the Fourier Transform Spectroscopy (FTS) technique has been considered a suboptimal choice…

Optics · Physics 2024-03-05 Lukasz A. Sterczewski , Mahmood Bagheri

We report molecular detection using dual frequency-comb spectroscopy with highly coherent broadband (6.6-11.4 {\m}m) long-wavelength infrared (LWIR) combs. The combs were produced via intra-pulse difference frequency generation (IDFG) in…

We demonstrate mid-infrared (MIR) frequency combs at 10 GHz repetition rate via intra-pulse difference-frequency generation (DFG) in quasi-phase-matched nonlinear media. Few-cycle pump pulses ($\mathbf{\lesssim}$15 fs, 100 pJ) from a…

A number of modern millimeter, sub-millimeter, and far-infrared detectors are read out using superconducting microwave (1-10GHz) resonators. The main detector technologies are Transition Edge Sensors, read out using Microwave SQUID…

Instrumentation and Detectors · Physics 2022-08-08 Max Silva-Feaver , Zeeshan Ahmed , Kam Arnold , Josef C. Frisch , John Groh , Shawn W. Henderson , Jesus Vasquez , Cyndia Yu