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Related papers: A DFT+$U$+$V$ study of pristine and oxygen-deficie…

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Density functional theory augmented with a Hubbard correction (DFT+U) is widely used to treat localized electronic states, but its predictions are often sensitive to the choice of the local projection space defining the correlated subspace.…

Strongly Correlated Electrons · Physics 2026-04-13 Manjula Raman , Kenneth Park

We present a systematic density functional theory (DFT) plus Hubbard $U$ study of structural trends and the stability of different magnetically ordered states across the rare-earth nickelate series, $R$NiO$_3$, with $R$ from Lu to La. In…

Materials Science · Physics 2017-10-17 Alexander Hampel , Claude Ederer

Transition-metal centers are the active sites for many biological and inorganic chemical reactions. Notwithstanding this central importance, density-functional theory calculations based on generalized-gradient approximations often fail to…

Soft Condensed Matter · Physics 2009-11-11 Heather J. Kulik , Matteo Cococcioni , Damian A. Scherlis , Nicola Marzari

With the motive of unraveling the origin of native vacancy induced magnetization in ferroelectric perovskite oxide systems, here we explore the consequences of electronic structure modification in magnetic ordering of oxygen deficient…

We develop a generalization of the Kohn-Sham density functional theory (KS-DFT) + Hubbard $U$ (DFT+$U$) method to the excited-state regime. This has the form of Hubbard $U$ corrected linear-response time-dependent DFT, or `TDDFT+$U$'.…

Strongly Correlated Electrons · Physics 2019-04-24 Okan K. Orhan , David D. O'Regan

Ferroelectricity, especially in hafnia-based thin films at nanosizes, has been rejuvenated in the fields of low-power, nonvolatile and Si-compatible modern memory and logic applications. Despite tremendous efforts to explore the formation…

We present and discuss results of a density functional theory (DFT) study of a perfect UO2 crystals and He atoms in octahedral interstitial positions. We have calculated basic bulk crystal properties and He incorporation energies into the…

Materials Science · Physics 2019-03-27 Denis Gryaznov , Eugene Heifets , Eugene Kotomin

A self-consistent calculation scheme for correlated electron systems is created based on the density-functional theory (DFT). Our scheme is a multi-reference DFT (MR-DFT) calculation in which the electron charge density is reproduced by an…

Strongly Correlated Electrons · Physics 2009-11-13 Koichi Kusakabe , Naoshi Suzuki , Shusuke Yamanaka , Kizashi Yamaguchi

Density functional theory augmented with Hubbard-$U$ corrections (DFT+$U$) is currently one of the widely used methods for first-principles electronic structure modeling of insulating transition metal oxides (TMOs). Since $U$ is relatively…

Computational Physics · Physics 2018-05-09 Samara Keshavarz , Johan Schött , Andrew J. Millis , Yaroslav O. Kvashnin

Nanosized hafnia-zirconia HfxZr1-xO2 in the form of thin films, multilayers and heterostructures are indispensable silicon-compatible ferroelectric materials for advanced electronic memories and logic devices. The distinctive feature of…

Materials Science · Physics 2026-05-05 Anna N. Morozovska , Eugene A. Eliseev , Sergei V. Kalinin , Maksym V. Strikha

Thin films of HfO2 doped with 4% La were fabricated on LSMO/STO (100) substrates using pulsed laser deposition. The stability of the ferroelectric orthorhombic phase in the hafnia films was investigated with respect to varying oxygen…

Materials Science · Physics 2023-08-16 Badari Narayana Rao , Shintaro Yasui , Hiroko Yokota

Study of nanoscale hafnia-zirconia physical properties is the key topic in fundamental and applied science. However, charge transport mechanisms and magnetic properties of hafnia-zirconia nanoparticles are very poorly studied both…

We have performed a detailed analysis of the magnetic (collinear and noncollinear) order and atomic and the electron structures of UO2, PuO2 and UN on the basis of density functional theory with the Hubbard electron correlation correction…

Materials Science · Physics 2017-08-23 Denis Gryaznov , Eugene Heifets , David Sedmidubsky

Ab initio density-functional calculations show that orthorhombic Pca21 hafnia HfO2 mixed with vanadium at low concentration is a ferroelectric and ferromagnetic insulator. The multiorbital degeneracy of singly-occupied V states in the…

Materials Science · Physics 2025-10-21 Vincenzo Fiorentini , Paola Alippi , Gianaurelio Cuniberti

The phase behavior and kinetic pathways of Li1+xV3O8 are investigated by means of density functional theory (DFT) and a cluster expansion (CE) methodology that approximates the system Hamiltonian in order to identify the lowest energy…

Materials Science · Physics 2013-05-30 Tonghu Jiang , Michael L. Falk

A family of magnetic halide double perovskites (HDPs) have recently attracted attention due to their potential to broaden application areas of halide double perovskites into e.g. spintronics. Up to date the theoretical modelling of these…

Materials Science · Physics 2022-11-30 Johan Klarbring , Utkarsh Singh , Sergei I. Simak , Igor A. Abrikosov

The electronic structure of selected rare-earth atoms adsorbed on a free-standing graphene was investigated using methods beyond the conventional density functional theory (DFT+U, DFT+HIA and DFT+ED). The influence of the electron…

Strongly Correlated Electrons · Physics 2016-09-12 Agnieszka L. Kozub , Alexander B. Shick , Frantisek Maca , Jindrich Kolorenc , Alexander I. Lichtenstein

We performed density functional theory (DFT)+$U$ and dynamical mean field theory (DMFT) calculations with continuous time quantum Monte Carlo impurity solver to investigate the electronic properties of V$_2$O$_5$ and Li$_x$V$_2$O$_5$ ($x$ =…

Strongly Correlated Electrons · Physics 2023-11-28 Huu T. Do , Alex Taekyung Lee , Hyowon Park , Anh T. Ngo

We conduct a systematic investigation of the role of Hubbard U corrections in electronic structure calculations of two-dimensional (2D) materials containing 3d transition metals. Specifically, we use density functional theory (DFT) with the…

Materials Science · Physics 2024-11-19 Sahar Pakdel , Thomas Olsen , Kristian S. Thygesen

Since the preliminary work of Anisimov and co-workers, the Hubbard corrected DFT+$U$ functional has been used for predicting properties of correlated materials by applying on-site effective Coulomb interactions to specific orbitals.…

Materials Science · Physics 2022-12-20 Stefano Falletta , Alfredo Pasquarello
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