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A mean field rate theory description of the homo- and co-polymerization of $f$-functional molecules is developed, which contains the formation of short cyclic structures inside the network. The predictions of this model are compared with…

Soft Condensed Matter · Physics 2021-03-31 Michael Lang , Konrad Schwenke , Jens-Uwe Sommer

We study swelling and structural properties of ionic microgel suspensions within a comprehensive coarse-grained model that combines the polymeric and colloidal natures of microgels as permeable, compressible, charged spheres governed by…

Soft Condensed Matter · Physics 2018-06-07 Tyler J. Weyer , Alan R. Denton

We use 2H NMR stimulated-echo spectroscopy to measure two-time correlation functions characterizing the polymer segmental motion in polymer electrolytes PPO-LiClO4 near the glass transition temperature Tg. To investigate effects of the salt…

Materials Science · Physics 2009-11-11 Michael Vogel , Thorsten Torbruegge

The response of a suspension under a variety of static or alternating external fields strongly depends on the equilibrium electric double layer that surrounds the colloidal particles in the suspension. The theoretical models for salt-free…

Soft Condensed Matter · Physics 2022-02-11 Jun-Sik Sin , Kwang-Il Kim , Kuk-Chol Ri , Dok-Yong Ju , Nam-Hyok Kim , Chung-Sik Sin

We simulate model systems of charged spherical particles in their counterion solution and measure the thermodynamic pressure and the pair distribution function from which we derive effective potentials of mean force. For a system with only…

Soft Condensed Matter · Physics 2007-05-23 Niels Gronbech-Jensen , Keith M Beardmore , Philip Pincus

A charged Yukawa liquid confined in a slit nanopore is studied in order to understand excluded volume effects in the interaction force between the pore walls. A previously developed self-consistent scheme (S. Buyukdagli el al., J. Stat.…

Soft Condensed Matter · Physics 2015-06-03 Sahin Buyukdagli , T. Ala-Nissila

A simple model is presented to calculate the potential of mean force between a polyion and a multivalent counterion inside a polyelectrolite solution. We find that under certain conditions the electrostatic interactions can lead to a strong…

Statistical Mechanics · Physics 2009-11-11 Jürgen F. Stilck , Yan Levin

Ideal MHD provides an accurate description of low-frequency Alfv\'en waves in fully ionized plasmas. However, higher frequency waves in many plasmas of the solar atmosphere cannot be correctly described by ideal MHD and a more accurate…

Solar and Stellar Astrophysics · Physics 2016-12-07 David Martínez-Gómez , Roberto Soler , Jaume Terradas

Adsorption on a boundary line confining a monolayer of particles self-assembling into clusters is studied by MC simulations. We focus on a system of particles interacting via competing interaction potential in which effectively short-range…

Soft Condensed Matter · Physics 2020-01-22 E. Bildanau , J. Pȩkalski , V. Vikhrenko , A. Ciach

We investigate spherical macroions in the strong Coulomb coupling regime within the primitive model in salt-free environment. We first show that the ground state of an isolated colloid is naturally overcharged by simple electrostatic…

Soft Condensed Matter · Physics 2016-08-16 René Messina , Christian Holm , Kurt Kremer

An analytical model of the electrostatic force between the tip of a non-contact Atomic Force Microscope (nc-AFM) and the (001) surface of an ionic crystal is reported. The model is able to account for the atomic contrast of the local…

Atomic and Molecular Clusters · Physics 2008-07-10 Franck Bocquet , Laurent Nony , Christian Loppacher , Thilo Glatzel

Surface force apparatus (SFA) and atomic force microscopy (AFM) can measure a force curve between a substrate and a probe in liquid. However, the force curve had not been transformed to the number density distribution of solvent molecules…

Statistical Mechanics · Physics 2017-02-10 Kota Hashimoto , Ken-ichi Amano

Ions in ionic liquids and concentrated electrolytes reside in a crowded, strongly-interacting environment, leading to the formation of discrete layers of charges at interfaces. Here, we propose a continuum theory that captures the…

Accumulation of particles while flowing past constrictions is a ubiquitous phenomenon observed in diverse systems. Some of the common examples are jamming of salt crystals near the orifice of salt shakers, clogging of filter systems,…

Soft Condensed Matter · Physics 2020-05-28 P. Prakash , A. Z. Abdulla , M. Varma

The relative energies of different phases or polymorphs of molecular solids can be small, less than a kiloJoule/mol. Reliable description of such energy differences requires high quality treatment of electron correlations, typically beyond…

Chemical Physics · Physics 2024-02-19 Khanh Ngoc Pham , Marcin Modrzejewski , Jiří Klimeš

We construct a coarse-grained molecular dynamics model based on poly(ethylene oxide) and lithium bis-(trifluoromethane)sulfonimide salt to examine the combined effects of temperature and salt concentration on the transport properties. Salt…

Soft Condensed Matter · Physics 2023-12-27 Alexandros J. Tsamopoulos , Zhen-Gang Wang

Computer simulations and theory are used to systematically investigate how the effective force between two big colloidal spheres in a sea of small spheres depends on the basic (big-small and small-small) interactions. The latter are modeled…

Soft Condensed Matter · Physics 2009-11-07 A. A. Louis , E. Allahyarov , H. Lowen , R. Roth

We propose the realization of linear crystals of cold ions which contain different atomic species for investigating quantum phase transitions and frustration effects in spin system beyond the commonly discussed case of $s=1/2$. Mutual…

Quantum Physics · Physics 2015-05-28 Peter A. Ivanov , Ferdinand Schmidt-Kaler

We study the effective interaction between differently charged polyelectrolyte-colloid complexes in electrolyte solutions via Monte Carlo simulations. These complexes are formed when short and flexible polyelectrolyte chains adsorb onto…

Soft Condensed Matter · Physics 2010-05-05 D. Truzzolillo , F. Bordi , F. Sciortino , S. Sennato

Acid ionization in aprotic media is studied using Molecular Dynamics techniques. In particular, models for HCl ionization in acetonitrile and dimethylsulfoxide are investigated. The proton is treated quantum mechanically using Feynman path…

chem-ph · Physics 2009-10-28 Daniel Laria , Raymond Kapral , Dario Estrin , Giovanni Ciccotti
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