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We study a two dimensional, two-band double-exchange model for $e_g$ electrons coupled to Jahn-Teller distortions in the presence of quenched disorder using a recently developed Monte-Carlo technique. In the absence of disorder the…

Strongly Correlated Electrons · Physics 2008-01-29 Sanjeev Kumar , Arno P. Kampf , Pinaki Majumdar

The effect of the Berry phase is included explicitly in the wavefunction describing conduction electrons in a crystal composed of periodically arrayed Jahn-Teller centers that have conically intersecting potential energy surfaces. The Berry…

Condensed Matter · Physics 2009-10-31 H. Koizumi , T. Hotta , Y. Takada

This paper reviews recent experimental and theoretical developments of the dynamic Jahn-Teller effect-driven phenomena in heavy transition metal-based spin-orbit Mott insulators. In cubic $4d/5d$ transition metal compounds, the spin,…

Strongly Correlated Electrons · Physics 2024-11-13 Naoya Iwahara

Based on the magnetoresistance, magnetization, ultrasound, and crystallographic data, we studied the role of the cooperative Jahn-Teller effect in the charge ordered (CO) state for La1-xCaxMnO3. We found that, with increasing the fraction…

Strongly Correlated Electrons · Physics 2009-11-10 R. K. Zheng , G. Li , A. N. Tang , Y. Yang , W. Wang , X. G. Li , Z. D. Wang , H. C. Ku

The Jahn-Teller effect explains distortions and non-degenerate energy levels in molecular and solid-state physics via a coupling of effective spins to collective bosons. Here we propose and theoretically analyze the quantum simulation of a…

Quantum Physics · Physics 2012-01-19 Diego Porras , Peter A. Ivanov , Ferdinand Schmidt-Kaler

With the use of the band structure calculations we demonstrate that previously reported [Nat. Materials {\bf 3}, 48 (2004)] experimental crystal and magnetic structures for NaMn$_7$O$_{12}$ are inconsistent with each other. The optimization…

Strongly Correlated Electrons · Physics 2014-06-06 S. V. Streltsov , D. I. Khomskii

CsCuCl$_3$, chiral and Jahn-Teller distorted at room temperature, takes a more symmetric structure above 423K. Describing this 'simpler' high temperature structure is far from simple and has been the subject of many, sometimes…

Materials Science · Physics 2026-05-28 Emma A. Pappas , Toby Woods , Jue Liu , Daniel P. Shoemaker

Temperature dependences of a magnetic and an orbital Bragg reflection at the Mn L2 and L3 edges of La0.5Sr1.5MnO4 have been collected. The temperature evolution of the orbital reflection depend strongly on the x-ray energy and reflects the…

Strongly Correlated Electrons · Physics 2007-05-23 U. Staub , V. Scagnoli , A. M. Mulders , M. Janousch , Z. Honda , J. M. Tonnerre

The orbital, lattice, and spin ordering phenomena in KCuF3 are investigated by means of LDA+U calculations, based on ab-initio pseudopotentials.We examine the Cu-3d orbital ordering and the associated Jahn-Teller distortion in several…

Strongly Correlated Electrons · Physics 2009-11-10 N. Binggeli , M. Altarelli

First-principles calculations reveal a large cooperative coupling of Jahn-Teller (JT) distortion to oxygen-octahedron rotations in perovskite LaMnO$_3$. The combination of the two distortions is responsible for stabilizing the strongly…

Strongly Correlated Electrons · Physics 2013-12-04 Jun Hee Lee , Kris T. Delaney , Eric Bousquet , Nicola A. Spaldin , Karin M. Rabe

A C$_3$-symmetric crystal-field potential in the Fe(II)Fe(III) bimetallic oxalates splits the L=2 Fe(II) multiplet into two doublets and a singlet. In compounds that exhibit magnetic compensation, one of the doublets was predicted to lie…

Other Condensed Matter · Physics 2009-11-13 Randy S. Fishman , Satoshi Okamoto , Fernando A. Reboredo

We present evidence that the insulator to metal transition in (La,Ca)MnO3 near x~0.2 is driven by the suppression of coherent Jahn-Teller distortions, originating from d type orbital ordering. The orbital ordered state is characterised by…

Materials Science · Physics 2009-11-07 Bas B. Van Aken , Auke Meetsma , Y. Tomioka , Y. Tokura , Thomas T. M. Palstra

In developing physical theories analogical reasoning has been found to be very powerful, as attested by a number of important historical examples. An analogy between two apparently different phenomena, once established, allows one to…

We investigate the $E_g \otimes e_g$ Jahn-Teller system for the purpose to reveal the nature of quantum chaos in crystals. This system simulates the interaction between the nuclear vibrational modes and the electronic motion in non-Kramers…

Materials Science · Physics 2008-12-18 Hisatsugu Yamasaki , Yuhei Natsume , Akira Terai , Katsuhiro Nakamura

Using high resolution X-Ray diffraction (XRD) on high purity powders, we resolved the structure and $ab$ symmetry of the intriguing compound \svo$ $ from room temperature down to 20 K to an unprecedented level of accuracy. Upon cooling,…

Strongly Correlated Electrons · Physics 2016-03-31 J. Teyssier , E. Giannini , A. Stucky , R. Cerný , M. V. Eremin , D. van der Marel

The low-doped magnetic perovskite La_{7/8}Sr_{1/8}MnO_3 undergoes within the paramagnetic-semiconducting phase a first-order structural transition due to antiferrodistorsive ordering of Jahn-Teller deformed MnO_6 octahedra. This allows to…

Strongly Correlated Electrons · Physics 2009-10-31 P. Wagner , I. Gordon , S. Mangin , V. V. Moshchalkov , Y. Bruynseraede , L. Pinsard , A. Revcolevschi

KCrF3 represents another prototypical orbital-ordered perovskite, where Cr2+ possesses the same electronic configuration of 3d4 as that of strongly Jahn-Teller distorted Mn3+ in many CMR manganites. The crystal and magnetic structures of…

Strongly Correlated Electrons · Physics 2013-09-30 Y. Xiao , Y. Su , H. -F. Li , C. M. N. Kumar , R. Mittal , J. Persson , A. Senyshyn , K. Gross , Th. Brueckel

The Jahn-Teller (JT) distortion that can remove electronic degeneracies in partially occupied states and results in systematic atomic displacements is a common underlying feature to many of the intriguing phenomena observed in 3d…

Materials Science · Physics 2019-12-04 Julien Varignon , Manuel Bibes , Alex Zunger

The development of Mn-rich cathodes for Li-ion batteries promises to alleviate supply chain bottlenecks in battery manufacturing. Challenges in Mn-rich cathodes arise from Jahn-Teller (JT) distortions of Mn$^{3+}$, Mn migration, and phase…

Materials Science · Physics 2025-05-26 Ronald L. Kam , Luca Binci , Aaron D. Kaplan , Kristin A. Persson , Nicola Marzari , Gerbrand Ceder

We introduce an effective model for $e_g$ electrons to describe three-dimensional perovskite (La$_{1-x}$Sr$_{x}$MnO$_3$ and La$_{1-x}$Ca$_{x}$MnO$_3$) manganites and study the magnetic and orbital order on $4\times 4\times 4$ cluster using…

Strongly Correlated Electrons · Physics 2010-10-26 Krzysztof Rościszewski , Andrzej M. Oleś