Related papers: Unveiling the nature of cathodoluminescence from p…
Cathodoluminescence (CL) enables optical-frequency analysis of samples with nanometer resolutions, originating from the interaction of a focused electron beam with radiative electronic states, or directly with the optical modes of the…
Photon bunching in incoherent cathodoluminescence (CL) spectroscopy originates from the fact that a single high-energy electron can generate multiple photons when interacting with a material, thus revealing key properties of electron-matter…
We present a method to separate coherent and incoherent contributions of cathodoluminescence (CL) by using a time-resolved coincidence detection scheme. For a proof-of-concept experiment, we generate CL by irradiating an optical multimode…
Cathodoluminescence (CL) microscopy has emerged as a powerful tool for investigating the optical properties of materials at the nanoscale, offering unique insights into the behavior of photonic and plasmonic materials under electron…
The impulsive excitation of ensembles of excitons or color centers by a high-energy electron beam results in the observation of photon bunching in the second-order correlation function of the cathodoluminescence generated by those emitters.…
We investigate theoretically the quantum-coherence properties of the cathodoluminescence (CL) emission produced by a temporally modulated electron beam. Specifically, we consider the quantum-optical correlations of CL from electrons that…
Recent advancements in time-resolved electron and photon detection enable novel correlative measurements of electrons and their associated cathodoluminescence (CL) photons within a transmission electron microscope. These studies are pivotal…
Following the lifespan of optical excitations from their creation to decay into photons is crucial in understanding materials optical properties. Macroscopically, techniques such as the photoluminescence excitation spectroscopy provide…
Spontaneous processes triggered in a sample by free electrons are commonly regarded as incoherent, and therefore unable to interfere with external light sources. Here, we challenge this concept by showing through first-principles theory…
Photoluminescence (PL) is a fundamental light-matter interaction in which absorbed photons are re-emitted, playing a key role in science and engineering. It is commonly modeled by introducing a non-zero chemical potential into Planck's law…
Electron-photon quantum entanglement in an electron microscope paves the way for a new quantum platform, enabling the integration of quantum functionalities into electron microscopy and opening opportunities for quantum imaging and quantum…
Cathodoluminescence spectroscopy in conjunction with second-order auto-correlation measurements of $g_2(\tau)$ allows to extensively study the synchronization of quantum light sources in low-dimensional structures. Co-existing excitons in…
High-energy (1-100 keV) electrons can coherently couple to plasmonic and dielectric nanostructures creating cathodoluminescence (CL) of which the spectral features reveal details of the material's resonant modes at deep-subwavelength…
Electron-beam-induced luminescence typically relies on direct excitation by high energy primary electrons. Here, we explore properties of an alternative excitation approach where cathodoluminescence (CL) is driven by substrate-generated…
Nonlinear optical phenomena such as parametric amplification and frequency conversion are typically driven by external optical fields. Free electrons can also act as electromagnetic sources, offering unmatched spatial precision. Combining…
We investigate the photon statistics of an ensemble of coherently driven non-interacting two-level atoms in the weak driving regime. As it turns out, the system displays unique emission characteristics that are strongly in contrast to the…
Compton scattering is one of the cornerstones of quantum physics, describing the fundamental interaction of a charged particle with photons. The Compton effect and its inverse are utilized in experiments driving free electrons by high…
Photoluminescence (PL) is a light-matter quantum interaction associated with the chemical potential of light formulated by the Generalized Planck's law. Without knowing the inherent temperature dependence of chemical potential, the…
Controlling electrically-stimulated quantum light sources (QLS) is key for developing integrated and low-scale quantum devices. The mechanisms leading to quantum emission are complex, as a large number of electronic states of the system…
The optical interference constitutes a paramount resource in modern physics. At the scale of individual atoms and photons, it is a diverse concept that causes different coherent phenomena. We present the experimental characterization of…