Related papers: Ultrafast quantum dynamics in $\mathbf{\mathrm{SrT…
An experimental continuous-wave (cw) pump-probe scheme is demonstrated by investigating the population and photoionization dynamics of an atomic system. Specifically, $^6$Li atoms are initially prepared in optically pumped $2^{2}S_{1/2}$…
Light has a wavelength that is usually longer than the size of the unit cell of crystals. Hence, even intense light pulses are not expected to break the translation symmetry of materials. However, certain materials, including KTaO$_3$,…
We experimentally investigate various processes present in the photoassociative interaction of an ultracold atomic sample with shaped femtosecond laser pulses. We demonstrate the photoassociation of pairs of rubidium atoms into…
We investigate the dynamics of molecular photoexcitation by unchirped femtosecond laser pulses using RbCs as a model system. This study is motivated by a goal of optimizing a two-color scheme of transferring vibrationally-excited ultracold…
Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…
We study the breakup of $\text{H}_2^+$ exposed to super-intense, femtosecond laser pulses with frequencies greater than that corresponding to the ionization potential. By solving the time-dependent Schr\"odinger equation in an extensive…
Transient extreme ultraviolet (XUV) spectroscopy probes core level transitions to unoccupied valence and conduction band states. Uncertainty remains to what degree the core-hole created by the XUV transition modifies the measurement of…
We present an optical pump-THz emission study on non-collinear antiferromagnet Mn$_3$Sn. We show that Mn$_3$Sn acts as a source of THz radiation when irradiated by femtosecond laser pulses. The polarity and amplitude of the emitted THz…
Intense laser pulses have recently emerged as a tool to tune between different orders in complex quantum materials. Among different light-induced phenomena, transient superconductivity far above the equilibrium transition temperature in…
The long lifetimes of magnons and phonons make them attractive for information-processing devices, highlighting the importance of visualizing their spatiotemporal dynamics from generation through relaxation. Ultrafast pump-probe…
Extreme states of matter exist throughout the universe e.g. inside planetary cores, stars or astrophysical jets. Such conditions are generated in the laboratory in the interaction of powerful lasers with solids, and their evolution can be…
We investigate theoretically a nuclear excitation mechanism involving absorption of non-resonant photons leveraged by the coupling to the atomic shell. The nuclear non-resonant photoexcitation is assisted by electron recombination which…
Experiments on superconducting materials have unveiled unique emergent properties when they are driven far from equilibrium. However, a quantitative first-principles treatment that describes experimental observations is lacking. In this…
Intense, few-cycle pulses in the terahertz frequency range have strong potential for schemes of control over vibrational modes in solid-state materials in the electronic ground-state. Here we report an experiment using single cycle…
To clarify the ultrafast temporal interplay of the different photocurrent mechanisms occurring in single InAs-nanowire-based circuits, an on-chip photocurrent pump-probe spectroscopy based on coplanar striplines was utilized. The data are…
A model for THz generation by optical rectification using tilted-pulse-fronts is developed. It simultaneously accounts for (i) the spatio-temporal distortions of the optical pump pulse, (ii) the nonlinear coupled interaction of THz and…
Studies employing nonlinear interactions of THz pulses are nowadays a promising scientific research field. To capture these phenomena, THz pulses with energy ranging from hundreds of \muJ to the mJ level are necessary. However, techniques…
The tunnelling of an electron through a suppressed atomic potential followed by its motion in the continuum, is the fundamental mechanism underlying strong-field laser-atom/molecule interactions. Due to its quantum nature, the interaction…
The study of the fundamental properties of phonons is crucial to understand their role in applica- tions in quantum information science, where the active use of phonons is currently highly debated. A genuine quantum phenomenon associated…
Similar to other perovskites in its family, $\mathrm{SrTiO_{3}}$ exhibits a significant softening of the ferroelectric mode with decreasing temperature, a behavior that typically heralds the onset of a ferroelectric transition. However,…