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The hierarchical equations of motion (HEOM) for a generalized quantum dissipative system is rigorously constructed in the frameworks of two different stochastic dynamical descriptions, i.e., the non-Markovian quantum state diffusion…

Quantum Physics · Physics 2018-07-18 Wei Wu

The hierarchical equations of motion (HEOM) theory is one of the standard methods to rigorously describe open quantum dynamics coupled to harmonic environments. Such a model is used to capture non-Markovian and non-perturbative effects of…

Chemical Physics · Physics 2020-06-02 Tatsushi Ikeda , Gregory D. Scholes

An open quantum system refers to a system that is further coupled to a bath system consisting of surrounding radiation fields, atoms, molecules, or proteins. The bath system is typically modeled by an infinite number of harmonic…

Chemical Physics · Physics 2020-07-10 Yoshitaka Tanimura

For a system strongly coupled to a heat bath, the quantum coherence of the system and the heat bath plays an important role in the system dynamics. This is particularly true in the case of non-Markovian noise. We rigorously investigate the…

Statistical Mechanics · Physics 2015-02-16 Yoshitaka Tanimura

Open quantum systems that feature non-Markovian dynamics are routinely solved using techniques such as the Hierarchical Equations of Motion (HEOM). However, their usage of the entire system density-matrix renders them intractable for…

Quantum Physics · Physics 2025-06-30 Kai Müller , Kimmo Luoma , Christian Schäfer

Quantum computing offers promising new avenues for tackling the long-standing challenge of simulating the quantum dynamics of complex chemical systems, particularly open quantum systems coupled to external baths. However, simulating such…

Quantum Physics · Physics 2025-02-20 Xiaohan Dan , Eitan Geva , Victor S. Batista

Over the last two decades, the hierarchical equations of motion (HEOM) of Tanimura and Kubo have become the equation of motion-based tool for numerically exact calculations of system-bath problems. The HEOM is today generalized to many…

Quantum Physics · Physics 2023-05-15 Robert Fuchs , Marten Richter

We have developed a computer code for the thermodynamic hierarchical equations of motion derived from a spin subsystem coupled to multiple Drude baths at different temperatures, which are connected to or disconnected from the subsystem as a…

Statistical Mechanics · Physics 2024-10-31 Shoki Koyanagi , Yoshitaka Tanimura

The hierarchical equations of motion (HEOM) approach can describe the reduced dynamics of a system simultaneously coupled to multiple bosonic and fermionic environments. The complexity of exactly describing the system-environment…

Studies of quantum thermal effects on molecular excitation dynamics have often relied on oversimplified models, such as energy eigenstates or low-dimensional potentials, which fail to capture the complexity of real chemical systems. In…

Chemical Physics · Physics 2025-12-30 Yankai Zhang , Yoshitaka Tanimura , So Hirata

The theory of hierarchical equations of motion (HEOM) is one of the standard methods to give exact evaluations of the dynamics as coupled to harmonic oscillator environments. However, the theory is numerically demanding due to its…

Chemical Physics · Physics 2022-05-31 Tatsushi Ikeda , Akira Nakayama

We present a theoretical framework to investigate quantum thermodynamic processes under non-Markovian system-bath interactions on the basis of the hierarchical equations of motion (HEOM) approach, which is convenient to carry out…

Quantum Physics · Physics 2019-05-01 Akihito Kato , Yoshitaka Tanimura

The hierarchical equations of motion technique has found widespread success as a tool to generate the numerically exact dynamics of non-Markovian open quantum systems. However, its application to low temperature environments remains a…

Chemical Physics · Physics 2013-10-15 Jeremy M. Moix , Jianshu Cao

Being a numerically exact method for the simulation of dynamics in open quantum systems, the hierarchical equations of motion (HEOM) still suffers from the curse of dimensionality. In this study, we propose a novel MCE-HEOM method, which…

Chemical Physics · Physics 2025-09-08 Zhecun Shi , Huiqiang Zhou , Lei Huang , Rixin Xie , Linjun Wang

The time evolution in open quantum systems, such as a molecular aggregate in contact with a thermal bath, still poses a complex and challenging problem. The influence of the thermal noise can be treated using a plethora of schemes, several…

Chemical Physics · Physics 2019-07-24 Hasan Rahman , Ulrich Kleinekathoefer

This work is a pedagogical survey about the hierarchical equations of motion and their implementation with the tensor-train format. These equations are a great standard in non-perturbative non-Markovian open quantum systems. They are exact…

Quantum Physics · Physics 2023-08-09 Etienne Mangaud , Amine Jaouadi , Alex Chin , Michèle Desouter-Lecomte

We unite two of the most widely used approaches for strongly damped, non-Markovian open quantum dynamics, the Hierarchical Equations of Motion (HEOM) and the pseudomode method by proving two statements: First, every physical bath…

Quantum Physics · Physics 2026-04-09 Kai Müller , Walter T. Strunz

The "hierarchical equations of motion" (HEOM) method is a powerful exact numerical approach to solve the dynamics and find the steady-state of a quantum system coupled to a non-Markovian and non-perturbative environment. Originally…

Optimal control theory is implemented with fully converged hierarchical equations of motion (HEOM) describing the time evolution of an open system density matrix strongly coupled to the bath in a spin-boson model. The populations of the…

Embedding non-Markovian open quantum dynamics into an enlarged Markovian space offers a powerful route to nonperturbative simulations, where the dynamics of the extended space can be governed by multiple distinct Markovian equations. We…

Quantum Physics · Physics 2026-02-26 Meng Xu , J. T. Stockburger , J. Ankerhold
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