Related papers: Coherent all X-ray four wave mixing at core shell …
In the field of beam physics, two frontier topics have taken center stage due to their potential to enable new approaches to discovery in a wide swath of science. These areas are: advanced, high gradient acceleration techniques, and x-ray…
Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…
Optical-domain Transient Grating (TG) spectroscopy is a versatile background-free four-wave-mixing technique used to probe vibrational, magnetic and electronic degrees of freedom in the time domain. The newly developed coherent X-ray Free…
Vibrational sum- and difference-frequency generation (SFG and DFG) spectroscopy probes the nonlinear response of interfaces at mid-infrared (MIR) wavelengths while detecting upconverted signals in the visible. Recent work has moved from…
Defect engineering is crucial for tuning 2D transition metal dichalcogenide properties for quantum and optoelectronic applications. While conventional photoluminescence (PL) and Raman spectroscopies are important characterization tools,…
We present a combined theoretical and experimental study of X-ray optical wave mixing. This class of nonlinear phenomena combines the strengths of spectroscopic techniques from the optical domain, with the high-resolution capabilities of…
Nonlinear wave-mixing in solids with ultrafast x-rays can provide new insight into complex electronic dynamics of materials. Here, tabletop-based attosecond noncollinear four-wave mixing (FWM) spectroscopy using one extreme ultraviolet…
Multiphoton processes in dense atomic vapors such as four-wave mixing or coherent blue light generation are typically viewed from single-atom perspective. Here we study the surprisingly important effect of phase matching near two-photon…
We demonstrate the correspondence between theoretically calculated K-shell resonances lying below the K-edge in multiple ionization states of an element (Pradhan et al. 2009), and recently observed K-alpha resonances in high-intensity X-ray…
In this work we numerically analyze a photonic unconventional accelerator based on the four-wave mixing effect in highly nonlinear waveguides. The proposed scheme can act as a fully analogue system for nonlinear signal processing directly…
Free-electron lasers have demonstrated their capability of generating intense attosecond X-ray pulses, which are the key to studying electron dynamics at their natural time scale and in specifically targeted electronic states, but come at…
Several nonlinear spectroscopy experiments which employ broadband x-ray pulses to probe the coupling between localized core and delocalized valence excitation are simulated for the amino acid cysteine at the K-edges of oxygen and nitrogen…
Here we experimentally map the dynamics of electron plasma waves in laser solid interaction. We do time resolved measurements of second harmonic and hard X-ray generation from interaction of intense ($10^{16} W cm^{-2}$, 100 fs, 800nm)…
We consider harmonics generation and wave-mixing by two-color multi photon resonant excitation of three-level atoms/molecules in strong laser fields. The coherent part of the spectra corresponding to multicolor harmonics generation is…
The advent of X-ray free-electron lasers (XFELs) has revolutionized fundamental science, from atomic to condensed matter physics, from chemistry to biology, giving researchers access to X-rays with unprecedented brightness, coherence, and…
Coherent nonlinear spectroscopies and imaging in the X-ray domain provide direct insight into the coupled motions of electrons and nuclei with resolution on the electronic length and time scale. The experimental realization of such…
Compact laboratory-scale X-ray sources still rely on the same fundamental principles as in the first X-ray tubes developed more than a century ago. In recent years, significant research and development have focused on large-scale X-ray…
We describe an all-fiber nonlinear interferometer based on four-wave mixing in highly nonlinear fiber. Our configuration realizes phase-sensitive interference with 97% peak visibility and >90% visibility over a broad 554 GHz optical band.…
Four-wave mixing (4WM) is a known source of intense non-classical twin beams. It can be generated when an intense laser beam (the pump) and a weak laser beam (the seed) overlap in a $\chi^{(3)}$ medium (here cesium vapor), with frequencies…
X-ray free electron laser (XFEL) experiments have brought unique capabilities and opened new directions in research, such as creating new states of matter or directly measuring atomic motion. One such area is the ability to use finely…