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Optically addressable spins at material surfaces have represented a long-standing ambition in quantum sensing, providing atomic resolution and quantum-limited sensitivity. However, they are constrained by a finite depth at which the quantum…

We report on electron spin resonance (ESR) spectroscopy of boron-vacancy (V$_\text{B}^-$) centers hosted in isotopically-engineered hexagonal boron nitride (hBN) crystals. We first show that isotopic purification of hBN with $^{15}$N yields…

We develop a method for entangling operations on nuclear spins surrounding a negatively charged boron vacancy (VB-center) point defect in hexagonal boron nitride (hBN). To this end, we propose to employ the electron spin of a VB-center as a…

Quantum Physics · Physics 2025-05-22 Fattah Sakuldee , Mehdi Abdi

Quantum sensors based on solid-state defects, in particular nitrogen-vacancy (NV) centers in diamond, enable precise measurement of magnetic fields, temperature, rotation, and electric fields. However, the sensitivity of leading NV spin…

Color centers in hexagonal boron nitride (hBN) have emerged as promising candidates for single-photon emitters (SPEs) due to their bright emission characteristics at room temperature. In contrast to mono- and few-layered hBN, color centers…

Applied Physics · Physics 2021-02-24 Pankaj K. Jha , Hamidreza Akbari , Yonghwi Kim , Souvik Biswas , Harry A. Atwater

Silicon Carbide is a promising host material for spin defect based quantum sensors owing to its commercial availability and established techniques for electrical and optical microfabricated device integration. The negatively charged silicon…

Magnetic resonance detection is one of the most important tools used in life-sciences today. However, as the technique detects the magnetization of large ensembles of spins it is fundamentally limited in spatial resolution to mesoscopic…

The experimental identification of optically addressable spin defects in hexagonal boron nitride has opened new possibilities for quantum sensor technologies in two-dimensional materials and structures. Despite numerous fundamental and…

Hexagonal boron nitride (h-BN) is a promising platform for quantum information processing due to its potential to host optically active defects with attractive optical and spin properties. Recent studies suggest that carbon trimers might be…

The Nitrogen-Vacancy (NV) defect in diamond is a unique quantum system that offers precision sensing of nanoscale physical quantities beyond the current state-of-the-art. Here we present a method to controllably encode the interactions in…

Quantum sensing is a key component of quantum technology, enabling highly sensitive magnetometry. We combined a nickelocene molecule with scanning tunneling microscopy to perform versatile spin sensing of magnetic surfaces, namely of model…

Mesoscale and Nanoscale Physics · Physics 2023-11-27 A. Fétida , O. Bengone , M. Romeo , F. Scheurer , R. Robles , N. Lorente , L. Limot

We present theoretical evidence, based on total-energy first-principles calculations, of the existence of spin-polarized states well localized at and extended along the edges of bare zigzag boron nitride nanoribbons. Our calculations…

Materials Science · Physics 2015-05-13 Veronica Barone , Juan E. Peralta

Measuring spins is the corner stone of a variety of analytical techniques including modern magnetic resonance imaging (MRI). The full potential of spin imaging and sensing across length scales is hindered by the achievable signal-to-noise…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 S. Steinert , F. Ziem , L. Hall , A. Zappe , M. Schweikert , A. Aird , G. Balasubramanian , L. Hollenberg , J. Wrachtrup

Quantum sensors based on individual spins provide unprecedented access to local magnetic fields in condensed matter, chemistry, and biology, with solid-state defect spins emerging as the leading platform. However, their molecular-sensing…

We demonstrate quantitative magnetic field mapping with nanoscale resolution, by applying a lock-in technique on the electron spin resonance frequency of a single nitrogen-vacancy defect placed at the apex of an atomic force microscope tip.…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 L. Rondin , J. -P. Tetienne , P. Spinicelli , C. Dal Savio , K. Karrai , G. Dantelle , A. Thiaville , S. Rohart , J. -F. Roch , V. Jacques

Boron vacancy centre ($V_{\rm B}^-$) ensembles in hexagonal boron nitride (hBN) have attracted recent interest for their potential as two-dimensional solid-state quantum sensors. Irradiation is necessary for $V_{\rm B}^-$ creation, however,…

Nuclear magnetic resonance (NMR) spectroscopy is a powerful technique to study local magnetism in a variety of materials. However, the inherently low sensitivity of conventional inductively detected solid state NMR typically requires a…

Mesoscale and Nanoscale Physics · Physics 2025-12-16 Louis Beaudoin , Aimé Verrier , Youcef A. Bioud , Mathieu Massicotte , Bertrand Reulet , Jeffrey A. Quilliam

Mapping the positions of single electron spins is a highly desired capability for applications such as nanoscale magnetic resonance imaging and quantum network characterization. Here, we demonstrate a method based on rotating an external…

Mesoscale and Nanoscale Physics · Physics 2022-11-11 Dan Yudilevich , Rainer Stöhr , Andrej Denisenko , Amit Finkler

Micron scale imaging of magnetic fields is an important tool for understanding the evolution of magnetism through phase transitions and as a result of interactions inside of heterostructures. However, most imaging platforms, like the…

Single-photon emitters play an essential role in quantum technologies, including quantum computing and quantum communications. Atomic defects in hexagonal boron nitride (h-BN) have recently emerged as new room-temperature single-photon…

Applied Physics · Physics 2018-07-16 Gichang Noh , Daebok Choi , Jin-Hun Kim , Dong-Gil Im , Yoon-Ho Kim , Hosung Seo , Jieun Lee