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Two-dimensional Ruddlesden-Popper hybrid lead halide perovskites have become a major topic in perovskite optoelectronics. Here, we aim to unravel the ultrafast dynamics governing the evolution of charge carriers and excitons in these…

Applied Physics · Physics 2020-09-02 Andrés Burgos-Caminal , Etienne Socie , Marine E. F. Bouduban , Jacques-E. Moser

Behaving like atomically-precise two-dimensional quantum wells with non-negligible dielectric contrast, the layered HOIPs have strong electronic interactions leading to tightly bound excitons with binding energies on the order of 500 meV.…

Materials Science · Physics 2021-06-02 Yeongsu Cho , Samuel M. Greene , Timothy C. Berkelbach

While polarons --- charges bound to a lattice deformation induced by electron-phonon coupling --- are primary photoexcitations at room temperature in bulk metal-halide hybrid organic-inorganic perovskites (HOIP), excitons --- Coulomb-bound…

Materials Science · Physics 2020-04-14 Ajay Ram Srimath Kandada , Carlos Silva

Strong Coulomb interactions in low-dimensional quantum materials give rise to emergent bound states such as excitons and trions, which play a central role in correlated electronic phases. In quasi-one-dimensional systems, equilibrium…

Excitonic effects play a particularly important role in the optoelectronic behavior of two-dimensional (2D) semiconductors. To facilitate the interpretation of experimental photoabsorption and photoluminescence spectra we provide…

Mesoscale and Nanoscale Physics · Physics 2018-01-04 M. Szyniszewski , E. Mostaani , N. D. Drummond , V. I. Fal'ko

With strongly bound and stable excitons at room temperature, single-layer, two-dimensional organic-inorganic hybrid perovskites are viable semiconductors for light-emitting quantum optoelectronics applications. In such a technological…

Strong Coulomb interaction in atomically-thin transition metal dichalcogenides makes these systems particularly promising for studies of excitonic physics. Of special interest are the manifestations of the charged excitons, also known as…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 M. M. Glazov

We study the dynamic equilibrium between trions and excitons in monolayers of transition metal dichalcogenides in the presence of resident charge carriers and continuous photogeneration of excitons. We show that heating of the system via…

Mesoscale and Nanoscale Physics · Physics 2026-03-25 A. M. Shentsev

The anisotropic nature of the new two-dimensional (2D) material phosphorene, in contrast to other 2D materials such as graphene and transition metal dichalcogenide (TMD) semiconductors, allows excitons to be confined in a…

The optical spectra of two dimensional (2D) materials exhibit sharp absorption peaks that are commonly identified with exciton and trions (or charged excitons). In this paper, we show that excitons and trions in doped 2D materials can be…

Mesoscale and Nanoscale Physics · Physics 2020-09-02 Farhan Rana , Okan Koksal , Christina Manolatou

Excitons, bound electron-hole pairs, in Two-Dimensional Hybrid Organic Inorganic Perovskites (2D HOIPs) are capable of forming hybrid light-matter states known as exciton-polaritons (E-Ps) when the excitonic medium is confined in an optical…

Layered hybrid perovskites containing larger organic cations have demonstrated superior environmental stability, but the presence of these insulating spacers also strengthens the exciton binding energy, which contributes to reduced carrier…

Excitonic quasi-particles, excitons/trions/bi-excitons, and their coupling with phonons and charge carriers play a crucial role in controlling the optical properties of atomically thin semiconducting 2D materials. In this work, we…

Materials Science · Physics 2021-10-01 Deepu Kumar , Rahul Kumar , Mahesh Kumar , Pradeep Kumar

The optical properties of semiconducting transition metal dichalcogenides are dominated by both neutral excitons (electron-hole pairs) and charged excitons (trions) that are stable even at room temperature. While trions directly influence…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Kai Hao , Lixiang Xu , Philipp Nagler , Akshay Singh , Kha Tran , Chandriker Kavir Dass , Christian Schüller , Tobias Korn , Xiaoqin Li , Galan Moody

So far in the literature the terms "charged exciton" and "trion" are often confused with each other and mostly considered as the same. In this work we show this is not the case in 2D quantum dots with a parabolic confinement. By using the…

Mesoscale and Nanoscale Physics · Physics 2022-03-14 Nguyen Hong Quang , Nguyen Que Huong

An excitonic insulator phase is expected to arise from the spontaneous formation of electron-hole pairs (excitons) in semiconductors where the exciton binding energy exceeds the size of the electronic band gap. At low temperature, these…

Strongly Correlated Electrons · Physics 2022-09-02 Selene Mor , Marc Herzog , Claude Monney , Julia Stähler

Excitons are neutral excitations that are composed of electrons and holes bound together by their attractive Coulomb interaction. The electron and the hole forming the exciton also interact with the underlying atomic lattice, and this…

Materials Science · Physics 2024-01-18 Zhenbang Dai , Chao Lian , Jon Lafuente-Bartolome , Feliciano Giustino

We solve the Schr\"{o}dinger equation for two electrons plus one hole by writing it in the electron-exciton basis. The main advantage of this basis is to eliminate the exciton contribution from the trion energy in a natural way. The…

Strongly Correlated Electrons · Physics 2015-03-20 Shiue-Yuan Shiau , Monique Combescot , Yia-Chung Chang

Charge neutrality and their expected itinerant nature makes excitons potential transmitters of information. However, exciton mobility remains inaccessible to traditional optical experiments that only create and detect excitons with…

Monolayer group VI transition metal dichalcogenides have recently emerged as semiconducting alternatives to graphene in which the true two-dimensionality (2D) is expected to illuminate new semiconducting physics. Here we investigate…

Mesoscale and Nanoscale Physics · Physics 2014-03-05 Jason S Ross , Sanfeng Wu , Hongyi Yu , Nirmal J Ghimire , Aaron M Jones , Grant Aivazian , Jiaqiang Yan , David G. Mandrus , Di Xiao , Wang Yao , Xiaodong Xu
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