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We develop a theoretical framework for probing moir\'e phonon modes using Raman spectroscopy, and illustrate it with the example of twisted bilayer graphene (TBG). These moir\'e phonons arise from interlayer sliding motion in twisted 2D…

Strongly Correlated Electrons · Physics 2025-06-24 Vitor Dantas , Héctor Ochoa , Rafael M. Fernandes , Natalia B. Perkins

We investigate the vibrational and magnetic properties of thin layers of chromium tribromide (CrBr$_3$) with a thickness ranging from three to twenty layers (3~L to 20~L) revealed by the Raman scattering (RS) technique. Systematic…

Using resonant Raman scattering spectroscopy with 25 different laser lines, we describe the Raman scattering spectra of mono- and multi-layers 2H-molybdenum diselenide (MoSe$_2$) as well as the different resonances affecting the most…

Mesoscale and Nanoscale Physics · Physics 2016-04-19 P. Soubelet , A. E. Bruchhausen , A. Fainstein , K. Nogajewski , C. Faugeras

Multipolar order, such as octupolar order, is a key concept in condensed matter physics, particularly in light of elusive hidden orders. However, its experimental identification remains challenging due to the absence of direct coupling to…

Optics · Physics 2026-03-25 Hikaru Watanabe , Rikuto Oiwa , Hitoshi Mori , Ryotaro Arita

We report temporal changes in Raman-scattering spectra of detwinned YBa$_2$Cu$_3$O$_{6+x}$ single crystals under exposure to red laser light polarized along the crystallographic $a$-axis. A recent publication by Bakr et al. (Phys. Rev. B 88…

Superconductivity · Physics 2018-08-22 H. Gretarsson , S. M. Souliou , S. Jeong , J. Porras , T. Loew , M. Bluschke , M. Minola , B. Keimer , M. Le Tacon

We study the scattering of guided light from a multilevel cesium atom with the transitions between the hyperfine levels $6S_{1/2}F=4$ and $6P_{3/2}F'=5$ of the $D_2$ line into the guided modes of a nanofiber. We show that the rate of…

Quantum Physics · Physics 2014-08-13 Fam Le Kien , A. Rauschenbeutel

The Raman coupling coefficients of site- and bond-percolators at concentration higher than percolation threshold are computed for two scattering mechanisms: Bond Polarizability (BPOL) and Dipole-Induced-Dipole (DID). The results show that…

Disordered Systems and Neural Networks · Physics 2015-06-25 O. Pilla , G. Viliani , R. DellAnna , G. Ruocco

Lattice structure and symmetry of two-dimensional (2D) layered materials are of key importance to their fundamental mechanical, thermal, electronic and optical properties. Raman spectroscopy, as a convenient and nondestructive tool, however…

Mesoscale and Nanoscale Physics · Physics 2015-08-28 Yanqing Feng , Wei Zhou , Yaojia Wang , Jian Zhou , Erfu Liu , Yajun Fu , Zhenhua Ni , Xinglong Wu , Hongtao Yuan , Feng Miao , Baigeng Wang , Xiangang Wan , Dingyu Xing

Natural van der Waals (vdW) crystals with hyperbolic dispersion challenge artificial metamaterials but remain confined to the mid-infrared spectrum. The emergence of MoOCl2, a quasi-one-dimensional metal with in-plane hyperbolicity,…

We present a Raman study of ZrAs_{2} single crystals, a nodal line semimetal with symmetry-enforced Dirac-like band crossings. We identified the symmetry of phonon modes by polarized light measurements and comparison with calculated phonon…

Materials Science · Physics 2024-05-16 R. Bacewicz , C. Jastrzębski , K. Zberecki , A. S. Wadge , D. Jastrzębski , A. Wiśniewski

Understanding the stability limitations and defect formation mechanisms in 2D magnets is essential for their utilization in spintronic and memory technologies. Here, we correlate defects in mono- to multilayer CrSBr with their structural,…

Mesoscale and Nanoscale Physics · Physics 2023-01-16 Kierstin Torres , Agnieszka Kuc , Lorenzo Maschio , Thang Pham , Kate Reidy , Lukas Dekanovsky , Zdenek Sofer , Frances M. Ross , Julian Klein

The analysis of the Raman scattering cross section of the radial breathing modes of double-wall carbon nanotubes allowed to determine the optical transitions of the inner tubes. The Raman lines are found to cluster into species with similar…

Soft Condensed Matter · Physics 2007-05-23 R. Pfeiffer , F. Simon , H. Kuzmany , V. N. Popov

We have revisited the still unresolved puzzle of the dispersion of the Raman disordered-induced D band as a function of laser excitation photon energy E$_L$ in graphite-like materials. We propose that the D-mode is a combination of an optic…

Disordered Systems and Neural Networks · Physics 2009-11-07 A. K. Sood , Rajeev Gupta , S. A. Asher

By computing the double-resonant Raman scattering cross-section completely from first principles and including electron-electron interaction at the $GW$ level, we unravel the dominant contributions for the double-resonant 2D-mode in bilayer…

Mesoscale and Nanoscale Physics · Physics 2014-11-04 Felix Herziger , Matteo Calandra , Paola Gava , Patrick May , Michele Lazzeri , Francesco Mauri , Janina Maultzsch

An experimental study of Raman scattering in N-layer graphene as a function of the top layer doping is reported. At high doping level, achieved by a CHF_3 plasma treatment, we observe a splitting of the $G$ band in the spectra of bilayer…

Mesoscale and Nanoscale Physics · Physics 2010-03-23 M. Bruna , S. Borini

We report generation of cascaded rotational Raman scattering up to 58th orders in coherently excited CO_2 molecules. The high-order Raman scattering, which produces a quasiperiodic frequency comb with more than 600 sidebands, is obtained…

We present a Raman spectroscopy study of iodine-intercalated (p-type-doped) double-walled carbon nanotubes. Double-walled carbon nanotubes (DWCNTs) are synthesized by catalytic chemical vapor deposition and characterized by Raman…

Few-layer tungsten diselenide (WSe2) is investigated using circularly polarized Raman spectroscopy with up to eight excitation energies. The main E2g1 and A1g modes near 250 cm-1 appear as a single peak in the Raman spectrum taken without…

Mesoscale and Nanoscale Physics · Physics 2019-06-11 Sanghun Kim , Kangwon Kim , Jae-Ung Lee , Hyeonsik Cheong

As the silicon industry continues to push the limits of device dimensions, tools such as Raman spectroscopy are ideal to analyze and characterize the doped silicon channels. The effect of inter-valence band transitions on the zone center…

Materials Science · Physics 2015-05-14 Brian G. Burke , Jack Chan , Keith A. Williams , Zili Wu , Alexander A. Puretzky , David B. Geohegan

Structural modifications in InP(111) due to 1.5 MeV implantation of Sb have been characterized using first order and second order Raman spectroscopy. With both Longitudinal Optical (LO) and Transverse Optical (TO) modes allowed for…

Materials Science · Physics 2007-08-21 D. Paramanik , S. Varma