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Our current understanding of the structure and dynamics of aqueous interfaces at the molecular level has grown substantially in the last few decades due to the continuous development of surface-specific spectroscopies, such as vibrational…

Chemical Physics · Physics 2023-09-27 Yair Litman , Jinggang Lan , Yuki Nagata , David M. Wilkins

Ultrafast lasers have become one of the most powerful tools in coherent nonlinear optical spectroscopy. Short pulses enable direct observation of fast molecular dynamics, whereas broad spectral bandwidth offers ways of controlling nonlinear…

Chemical Physics · Physics 2015-05-13 X. G. Xu , S. O. Konorov , J. W. Hepburn , V. Milner

X-ray spectral fitting in high-energy astrophysics can be reliably accelerated using Machine Learning. In particular, Simulation-based Inference (SBI) produces accurate posterior distributions in the Gaussian and Poisson regime for…

Instrumentation and Methods for Astrophysics · Physics 2025-07-09 Simon Dupourqué , Didier Barret

Fourier-transform infrared spectroscopy (FTIR) is the golden standard of mid-infrared (MIR) molecular spectroscopic analysis through optically-encoded vibrational signatures. Michelson-type FTIR and MIR dual-comb spectrometers allow us to…

Optics · Physics 2025-05-06 Kazuki Hashimoto , Venkata Ramaiah Badarla , Takuro Ideguchi

A spectral mixture (SM) kernel is a flexible kernel used to model any stationary covariance function. Although it is useful in modeling data, the learning of the SM kernel is generally difficult because optimizing a large number of…

Machine Learning · Statistics 2020-06-15 Yohan Jung , Kyungwoo Song , Jinkyoo Park

Quantum computational chemistry holds great promise for simulating molecular systems more efficiently than classical methods by leveraging quantum bits to represent molecular wavefunctions. However, current implementations face significant…

Quantum Physics · Physics 2025-09-10 Weitang Li , Shi-Xin Zhang , Zirui Sheng , Cunxi Gong , Jianpeng Chen , Zhigang Shuai

Presented is a novel way to combine snapshot compressive imaging and lateral shearing interferometry in order to capture the spatio-spectral phase of an ultrashort laser pulse in a single shot. A deep unrolling algorithm is utilised for the…

Tissue oxygenation and perfusion can be an indicator for organ viability during minimally invasive surgery, for example allowing real-time assessment of tissue perfusion and oxygen saturation. Multispectral imaging is an optical modality…

Computer Vision and Pattern Recognition · Computer Science 2017-06-23 Geoffrey Jones , Neil T Clancy , Xiaofei Du , Maria Robu , Simon Arridge , Daniel S Elson , Danail Stoyanov

We propose visual-inertial simultaneous localization and mapping that tightly couples sparse reprojection errors, inertial measurement unit pre-integrals, and relative pose factors with dense volumetric occupancy mapping. Hereby depth…

Robotics · Computer Science 2025-03-10 Jaehyung Jung , Simon Boche , Sebastián Barbas Laina , Stefan Leutenegger

To improve the classification performance in the context of hyperspectral image processing, many works have been developed based on two common strategies, namely the spatial-spectral information integration and the utilization of neural…

Computer Vision and Pattern Recognition · Computer Science 2020-06-24 Yi Liang , Xin Zhao , Alan J. X. Guo , Fei Zhu

Gravitational-wave data from advanced-era interferometric detectors consists of background Gaussian noise, frequent transient artefacts, and rare astrophysical signals. Multiple search algorithms exist to detect the signals from compact…

General Relativity and Quantum Cosmology · Physics 2026-01-13 Gregory Ashton , Ann-Kristin Malz , Nicolo Colombo

Spectral measurements in the infrared (IR) optical range provide unique fingerprints of materials which are useful for material analysis, environmental sensing, and health diagnostics. Current IR spectroscopy techniques require the use of…

Quantum Physics · Physics 2016-02-05 Dmitry A. Kalashnikov , Anna V. Paterova , Sergei P. Kulik , Leonid A. Krivitsky

Numerous experimental and theoretical studies have established that intramolecular vibrational energy redistribution (IVR) in isolated molecules has a heirarchical tier structure. The tier structure implies strong correlations between the…

Chaotic Dynamics · Physics 2009-11-07 Srihari Keshavamurthy , Nicholas R. Cerruti , Steven Tomsovic

We propose an inverse-design approach for computational spectrometers in which the scattering media are topology-optimized to achieve better performance in inference of unknown spectra. Unlike traditional end-to-end approaches, our inverse…

Optics · Physics 2026-03-31 Wenchao Ma , Raphaël Pestourie , Zin Lin , Steven G. Johnson

We develop a strategy that integrates machine learning and first-principles calculations to achieve technical accurate predictions of infrared spectra. Specifically, the methodology allows to predict infrared spectra for complex systems at…

Materials Science · Physics 2024-05-01 Bernhard Schmiedmayer , Georg Kresse

In this work, a simple and efficient dual iterative refinement (DIR) method is proposed for dense correspondence between two nearly isometric shapes. The key idea is to use dual information, such as spatial and spectral, or local and global…

Computer Vision and Pattern Recognition · Computer Science 2020-11-20 Rui Xiang , Rongjie Lai , Hongkai Zhao

Reconfigurable intelligent surface (RIS) is a two-dimensional periodic structure integrated with a large number of reflective elements, which can manipulate electromagnetic waves in a digital way, offering great potentials for wireless…

Machine Learning · Computer Science 2025-01-22 Zhen Zhang , Jun Hui Qiu , Jun Wei Zhang , Hui Dong Li , Dong Tang , Qiang Cheng , Wei Lin

Integrated sensing and communication (ISAC) can reduce beam-training overhead in mmWave vehicle-to-infrastructure (V2I) links by enabling in-band sensing-based beam prediction, while exteroceptive sensors can further enhance the prediction…

Signal Processing · Electrical Eng. & Systems 2026-01-06 Abidemi Orimogunje , Hyunwoo Park , Igbafe Orikumhi , Sunwoo Kim , Dejan Vukobratovic

Hyperspectral imaging provides spatially resolved spectral information. Utilising dual frequency combs as active illumination sources, hyperspectral imaging with ultra-high spectral resolution can be implemented in a scan-free manner when a…

Methyl benzoate (MB) is studied as a model compound for the development of new IR pulse schemes with possible applicability to biomolecules. Anharmonic vibrational modes of MB are calculated on different level (MP2, SCS, CCSD(T) with…

Chemical Physics · Physics 2014-01-03 Kiran Sankar Maiti , Christoph Scheurer
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