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Synchronization of oscillators is ubiquitous in nature. Often, the synchronized oscillators couple directly, yet in some cases synchronization can arise from their parametric interactions. Here, we theoretically predict and experimentally…

With demonstrated applications ranging from metrology to telecommunications, soliton microresonator frequency combs have emerged over the past decade as a remarkable new technology. However, standard implementations only allow for the…

Dual-comb spectroscopy is a powerful technique to measure optical spectra in a wide spectral range with high-frequency resolution. The development of compact systems operating in the long-wave infrared wavelength range is of high interest…

The method of Doppler - free comb - spectroscopy for dipole transitions was proposed. The calculations for susceptibility spectrum for moving two-level atoms driving by strong counter propagating combs have been done. The used theoretical…

Optics · Physics 2014-03-07 S. A. Pulkin , A. Kalinichev , V. Arnautov , S. V. Uvarova , S. Savel'eva

Historically, there has been a trade-off in spectroscopic measurements between high spectral resolution, broadband coverage, and acquisition time. Optical frequency combs, initially envisioned for precision spectroscopy of the hydrogen atom…

Optics · Physics 2020-06-04 A. V. Muraviev , D. Konnov , K. L. Vodopyanov

Chip-scale integration of optical frequency combs, particularly soliton microcombs, enables miniaturized instrumentation for timekeeping, ranging, and spectroscopy. Although soliton microcombs have been demonstrated on various material…

Supercontinuum generation in optical fibers is one of the most dramatic nonlinear effects discovered, allowing short pulses to be converted into multi-octave spanning coherent spectra. However, generating supercontinua that are both…

Hyperspectral imaging provides spatially resolved spectral information. Utilising dual frequency combs as active illumination sources, hyperspectral imaging with ultra-high spectral resolution can be implemented in a scan-free manner when a…

Optical spectroscopy and imaging of microscopic samples have opened up a wide range of applications throughout the physical, chemical, and biological sciences. High chemical specificity may be achieved by directly interrogating the…

This thesis presents the development and characterisation of a polarisation-multiplexing ring-cavity fibre laser for dual-comb generation. It explores the underlying physics, implementation, and potential uses of this innovative laser…

Optics · Physics 2025-08-06 Alberto Rodriguez Cuevas

Optical frequency combs represent a revolutionary technology for high precision spectroscopy due to their narrow linewidths and precise frequency spacing. Generation of such combs in the mid-infrared (IR) spectral region (2-20 um) is of…

In the current study, a quantum-cascade-laser-based dual-comb spectrometer (DCS) was used to paint a detailed picture of a 1.0 ms high-temperature reaction between propyne and oxygen. The DCS interfaced with a shock tube to provide…

Dual-comb spectroscopy enables broadband, high-resolution measurements with microsecond temporal resolution, but extending this capability to the 10~12.5 $\mu$m molecular fingerprint region remains technically challenging, particularly for…

Optics · Physics 2026-04-30 Pei-Ling Luo , I-Yun Chen

The ability to generate efficient and coherent frequency combs using photonic integrated circuits offers tremendous potential for a range of applications. In particular, "microcombs" based on chip-integrated resonators are poised to…

Detector nonlinearity is an important factor limiting the maximal power and hence the signal-to-noise ratio (SNR) in dual-comb interferometry. To increase the SNR without overwhelming averaging time, specific experimental conditions must be…

Soliton microcombs provide compact, broadband, coherent light sources for precision metrology, spectroscopy, communications, and microwave photonics. Extending their spectral span while retaining useful output power remains challenging and…

Laser dynamics underpin a broad range of modern photonic technologies and continue to reveal rich nonlinear behaviors. However, existing spectroscopic tools, most notably time-stretched dispersive Fourier transform spectroscopy (TS-DFT),…

Microresonator frequency combs harness the nonlinear Kerr effect in an integrated optical cavity to generate a multitude of phase-locked frequency lines. The line spacing can reach values in the order of 100 GHz, making it an attractive…

Multi-dimensional coherent spectroscopy (MDCS)1,2 is a powerful method for optical spectroscopy that has become an important tool for studying ultrafast dynamics in a wide range of systems. It is an optical analog of multidimensional…

Optics · Physics 2018-10-24 Bachana Lomsadze , Brad. C. Smith , Steven T. Cundiff

We demonstrate the performance of a dual frequency comb QCL spectrometer for the application of vibrational Stark spectroscopy. Measurements performed on fluorobenzene with the dual-comb spectrometer (DCS) were compared to results obtained…

Chemical Physics · Physics 2019-11-22 Urszula Szczepaniak , Samuel H. Schneider , Raphael Horvath , Jacek Kozuch , Markus Geiser