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Implicit solvation is an effective, highly coarse-grained approach in atomic-scale simulations to account for a surrounding liquid electrolyte on the level of a continuous polarizable medium. Originating in molecular chemistry with finite…

Chemical Physics · Physics 2021-08-06 Stefan Ringe , Nicolas G. Hörmann , Harald Oberhofer , Karsten Reuter

We analytically calculate the correlation potential of a test ion near a \emph{strongly} charged plate inside a dilute $m:-n$ electrolyte. We do this by calculating the electrostatic Green's function in the presence of a nonlinear…

Soft Condensed Matter · Physics 2014-03-19 Bing-Sui Lu , Xiangjun Xing

The standard Maxwell formulation of the problem of polarized dielectrics suffers from a number of difficulties, both conceptual and practical. These difficulties are particularly significant in the case of liquid interfaces, where the…

Soft Condensed Matter · Physics 2015-06-18 Dmitry V. Matyushov

The Budd-Vannimenus theorem is modified to apply to superconductors in the Meissner state. The obtained identity links the surface value of the electrostatic potential to the density of free energy at the surface which allows one to…

Superconductivity · Physics 2009-11-10 P. Lipavsky , K. Morawetz , J. Kolacek , J. J. Mares , E. H. Brandt , M. Schreiber

The uniqueness of a surface density of sources localized inside a spatial region $R$ and producing a given electric potential distribution in its boundary $B_0$ is revisited. The situation in which $R$ is filled with various metallic…

Medical Physics · Physics 2009-11-06 Alejandro Cabo , Carlos Handy , Daniel Bessis

Solid polymer electrolytes for lithium batteries promise improvements in safety and energy density if their conductivity can be increased. Nanostructured block copolymer electrolytes specifically have the potential to provide both good…

There is a large body of literature investigating the static and dynamic properties of polyelectrolytes due both to their widespread application in industrial processes and their ubiquitous presence in biology. Because of their highly…

Soft Condensed Matter · Physics 2016-01-20 Florian Fahrenberger , Owen A. Hickey , Jens Smiatek , Christian Holm

An accurate prediction of the surface potential at the air-water interface is critical to calculating ion hydration free energies and electrochemical half-cell potentials. Using Density Functional Theory (DFT), model interfacial…

Materials Science · Physics 2010-09-22 Kevin Leung

Effect of ionic solute on a near-critical binary aqueous mixture confined between charged walls with different adsorption preferences is considered within a simple density functional theory. For the near-critical system containing small…

Soft Condensed Matter · Physics 2015-05-28 F. Pousaneh , A. Ciach

The structure of dilute electrolyte solutions close to a surface carrying a spatially inhomogeneous surface charge distribution is investigated by means of classical density functional theory (DFT) within the approach of fundamental measure…

Soft Condensed Matter · Physics 2020-06-23 Maximilian Mußotter , Markus Bier , S. Dietrich

Mean-field theory is used to model polyelectrolyte adsorption and the possibility of overcompensation of charged surfaces. For charged surfaces that are also chemically attractive, the overcharging is large in high salt conditions,…

Soft Condensed Matter · Physics 2009-11-10 Adi Shafir , David Andelman

An ideal conductor electrode in contact with a semi-infinite two-dimensional two-component plasma in an external potential is considered. The model is mapped onto an integrable sine-Gordon theory with Dirichlet boundary conditions. The…

Statistical Mechanics · Physics 2011-07-19 L. Šamaj , B. Jancovici

Water-in-Salt-Electrolytes (WiSEs) are a promising class of next-generation electrolytes. Unlike classical dilute electrolytes or more conventional battery electrolytes, WiSEs are characterised by their super-concentrated salt concentration…

We study the low-frequency polarization response of a surface-charged oblate spheroidal particle immersed in an electrolyte solution. Because the charged spheroid attracts counter-ions which form the electric double layer around the…

Classical Physics · Physics 2017-04-12 Chang-Yu Hou , Denise E. Freed , Pabitra N. Sen

Using a continuum description, we account for fluctuations in the ionic solvent surrounding a Gaussian, charged chain and derive an effective short-ranged potential between the charges on the chain. This potential is repulsive at short…

Soft Condensed Matter · Physics 2009-11-10 Shirish M. Chitanvis

A better understanding of interfacial mechanisms is needed to improve the performances of electrochemical devices. Yet, simulating an electrode surface at fixed electrolyte composition remains a challenge. Here we apply a finite electric…

Materials Science · Physics 2019-11-13 Thomas Dufils , Guillaume Jeanmairet , Benjamin Rotenberg , Michiel Sprik , Mathieu Salanne

Recently Deyo et al. [\prb {\bf 106}, 104502 (2022)] suggested that the surface resistance $R_s(H_0)$ of a superconductor under strong electromagnetic field can be affected by field-induced quasiparticle bound states at the surface. This…

Superconductivity · Physics 2022-11-10 A. Gurevich

The structure of polar liquids and electrolytic solutions, such as water and aqueous electrolytes, at interfaces underlies numerous phenomena in physics, chemistry, biology, and engineering. In this work, we develop a continuum theory that…

Soft Condensed Matter · Physics 2022-07-13 J. Pedro de Souza , Alexei A. Kornyshev , Martin Z. Bazant

Monolayers of colloidal particles at oil-water interfaces readily crystalize owing to electrostatic repulsion, which is often mediated through the oil. However, little attempts exist to control it using oil-soluble electrolytes. We probe…

Soft Condensed Matter · Physics 2023-05-04 Carolina van Baalen , Jacopo Vialetto , Lucio Isa

We investigate the possibility that electrically neutral porous spheres electrophorese in electrolyte solutions with asymmetric affinity of ions to spheres on the basis of electrohydrodynamics and the Poisson-Boltzmann and…

Soft Condensed Matter · Physics 2015-06-23 Yuki Uematsu
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