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We present an overview of our recent investigations of long-range interactions in an ultracold Cs Rydberg gas. These interactions are studied by high-resolution photoassociation spectroscopy, using excitation close to one-photon transitions…
We present photodissociation of ultracold long-range Rydberg molecules as a tool to characterize their electronic properties. We photoassociate K2 37P molecules with highly entangled electronic and nuclear spins of the two bound atoms and…
Assemblies of interacting Rydberg atoms show promise for the quantum simulation of transport phenomena, quantum chemistry and condensed matter systems. Such schemes are typically limited by the finite lifetime of Rydberg states. Circular…
Rydberg blockade of ultracold atoms is considered now as one of the most promising tools for the implementation of quantum computing, but its fidelity can be substantially compromised by detrimental excitation of the neighbouring atoms.…
We show that an array of polar molecules interacting with Rydberg atoms is a promising hybrid system for scalable quantum computation. Quantum information is stored in long-lived hyperfine or rotational states of molecules which interact…
We propose and study a quantum pump which emulates a traditional paddlewheel, that can be implemented with ultracold atoms in waveguides. We use wavepacket propagation to study its single-mode dynamics, which also determines its multimode…
We observe long-range $^{85}$Rb and $^{87}$Rb (24$D$+5$S_{1/2}$) Rydberg molecules for eight different spin couplings, with binding energies up to 440~MHz and sub-percent relative uncertainty. Isotopic effects of the molecular binding…
Rydberg atoms provide a powerful platform for exploring strongly interacting quantum systems, both in free space and in structured electromagnetic environments, with growing applications in quantum technology. Accurately modeling their…
The Fraunhofer diffraction of quantum particles from materials with sharp electron-density edges or symmetric bond structures is ubiquitous. In contrast, diffraction from atoms with characteristic asymptotically-diffused electron…
A detailed theoretical framework for highly excited Rydberg molecules is developed based on the generalized local frame transformation. Our approach avoids the use of pseudopotentials and yields analytical expressions for the body-frame…
The generation of entanglement produced by a local potential interaction in a bipartite system is investigated. The degree of entanglement is contrasted with the underlying classical dynamics for a Rydberg molecule (a charged particle…
This topical review addresses how Rydberg atoms can serve as building blocks for emerging quantum technologies. Whereas the fabrication of large numbers of artificial quantum systems with the uniformity required for the most attractive…
Rydberg states of atoms are of great current interest for quantum manipulation of mesoscopic samples of atoms. Long-range Rydberg-Rydberg interactions can inhibit multiple excitations of atoms under the appropriate conditions. These…
We explore the fluorescence signals from a pair of atoms driven towards Rydberg states on a three-level ladder transition. The dipole--dipole interactions between Rydberg excited atoms significantly distort the dark state and…
Ultracold atomic gases have been used extensively in recent years to realize textbook examples of condensed matter phenomena. Recently, phase transitions to ordered structures have been predicted for gases of highly excited, 'frozen'…
We report the engineering of molecular potentials at large interatomic distances. The molecular states are generated by off-resonant optical coupling to a highly excited, long-range Rydberg molecular potential. The coupling produces a…
The interaction between a Rydberg electron and a neutral atom situated inside its extended orbit is described via contact interactions for each atom-electron scattering channel. In ultracold environments, these interactions lead to…
Diffusive molecular dynamics is a novel model for materials with atomistic resolution that can reach diffusive time scales. The main ideas of diffusive molecular dynamics are to first minimize an approximate variational Gaussian free energy…
The ability to generate and control strong long-range interactions via highly excited electronic states has been the foundation for recent breakthroughs in a host of areas, from atomic and molecular physics [1, 2] to quantum optics [3, 4]…
Run-and-tumble particles, frequently considered today for modeling bacterial locomotion, naturally appear outside a biological context as well, e.g. for producing waves in the telegraph process. Here, we use a wave function to drive their…