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We present a theoretical study of the time-dependent laser alignment of molecules taking into account the hyperfine coupling due to nuclear-quadrupole interactions. The coupling of nuclear spins to the overall angular momentum of molecules…

Chemical Physics · Physics 2020-06-18 Linda V. Thesing , Andrey Yachmenev , Rosario González-Férez , Jochen Küpper

We present a general variational approach for computing the laser-induced rovibrational dynamics of molecules taking into account the hyperfine effects of the nuclear quadrupole coupling. The method combines the general variational approach…

Atomic and Molecular Clusters · Physics 2020-06-18 Andrey Yachmenev , Linda V. Thesing , Jochen Küpper

Among the possible types of magnetic dipole interactions in molecular systems, couplings between nuclear motion and the nuclear spin have probably received the least attention in molecular spectroscopy. Although very small in comparison to…

Chemical Physics · Physics 2026-04-22 Matthias Diez , Johannes K. Krondorfer , Albert Hirtenfelder , Andreas W. Hauser

Lanthanide-based single-ion magnetic molecules can have large magnetic hyperfine interactions as well as large magnetic anisotropy. Recent experimental studies reported tunability of these properties by changes of chemical environments or…

Materials Science · Physics 2019-10-29 Aleksander L. Wysocki , Kyungwha Park

This study employs the isospin-dependent Boltzmann-Uehling-Uhlenbeck model to simulate intermediate-energy heavy-ion collisions between prolate nuclei $^{24}$Mg. The emphasis is on investigating the influence of centrality and orientation…

Nuclear Theory · Physics 2023-09-12 Xiao-Hua Fan , Zu-Xing Yang , Peng-Hui Chen , Shunji Nishimura , Zhi-Pan Li

Nuclear quadrupole interaction extends the limits imposed by hyperfine interaction on the spin coherence of the electron and nuclei in a quantum dot. The strain-induced nuclear quadrupole interaction suppresses the nuclear spin flip and…

Mesoscale and Nanoscale Physics · Physics 2008-04-01 R. I. Dzhioev , V. L. Korenev

We study the mechanism of dynamical nuclear spin polarization by hyperfine interaction in spin-blocked double quantum dot system. We calculate the hyperfine transition rates and solve the master equations for the nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Changxue Deng , Xuedong Hu

The interplay of optical driving and hyperfine interaction between an electron confined in a quantum dot and its surrounding nuclear spin environment produces a range of interesting physics such as mode-locking. In this work, we go beyond…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Arian Vezvaee , Gargee Sharma , Sophia E. Economou , Edwin Barnes

We have studied nuclear quadrupole deformation effects in deeply bound pionic atoms theoretically. We have evaluated the level shifts and widths of the hyperfine components using the first order perturbation theory and compared them with…

Nuclear Theory · Physics 2009-10-30 N. Nose-Togawa , S. Hirenzaki , K. Kume

The nuclear spins of ionized donors in silicon have become an interesting quantum resource due to their very long coherence times. Their perfect isolation, however, comes at a price, since the absence of the donor electron makes the nuclear…

We present electrically detected electron nuclear double resonance measurements of the nuclear spins of ionized and neutral arsenic donors in strained silicon. In addition to a reduction of the hyperfine coupling, we find significant…

The shape of atomic nuclei is often interpreted to possess a quadrupole deformation that fluctuates around some average profile. We investigate the impact of nuclear shape fluctuations on the initial state geometry in heavy ion collisions,…

Nuclear Theory · Physics 2023-06-27 Aman Dimri , Somadutta Bhatta , Jiangyong Jia

Strain-induced gradients of local electric fields in semiconductor quantum dots can couple to the quadrupole moments of nuclear spins. We develop a theory describing the influence of this quadrupolar coupling (QC) on the spin correlators of…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 N. A. Sinitsyn , Yan Li , S. A. Crooker , A. Saxena , D. L. Smith

Nuclear spin levels play an important role in understanding magnetization dynamics and implementation and control of quantum bits in lanthanide-based single-molecule magnets. We investigate the hyperfine and nuclear quadrupole interactions…

Materials Science · Physics 2020-06-24 Aleksander L. Wysocki , Kyungwha Park

A series expansion of the interaction between a nucleus and its surrounding electron distribution provides terms that are well-known in the study of hyperfine interactions: the familiar quadrupole interaction and the less familiar…

Atomic and Molecular Clusters · Physics 2015-05-14 Katrin Koch , Klaus Koepernik , Dimitri Van Neck , Helge Rosner , Stefaan Cottenier

Nuclear magnetic resonance gyroscopes that detect rotation as a shift in the precession frequency of nuclear spins, have attracted a lot of attentions. Under a feedback-generated drive, the precession frequency is supposed to be dependent…

Quantum Physics · Physics 2020-07-15 Yue Chang , Shuang-ai Wan , Jie Qin

A moderately intense $450$ fs laser pulse is used to create rotational wave packets in gas phase $\rm{I_2}$ molecules. The ensuing time-dependent alignment, measured by Coulomb explosion imaging with a delayed probe pulse, exhibits the…

We investigate interactions between the proton spin, the deuteron spin, and the orbital angular momentum in the electronic ground state of the HD molecule. These interactions lead to hyperfine splittings of molecular energy levels. Our…

Chemical Physics · Physics 2020-07-29 Jacek Komasa , Mariusz Puchalski , Krzysztof Pachucki

We studied the influence of a momentum dependent interaction in the context of isopspin effects on fragmentation and dissipation in intermediate energy heavy ion collisions by using an isospin dependent quantum molecular dynamics model. It…

Nuclear Theory · Physics 2009-11-10 Jian-Ye Liu , Wen-Jun Guo , Yong Zhong Xing , Wei Zou , Xi-Guo Lee

It is well known that non-central nuclear forces, such as the spin-orbital coupling and the tensor force, play important roles in understanding many interesting features of nuclear structures. However, their dynamical effects in nuclear…

Nuclear Theory · Physics 2015-11-17 Jun Xu , Bao-An Li , Wen-Qing Shen , Yin Xia
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