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We analyze a model problem representing a multi-electronic molecule sitting on a metal surface. Working with a reduced configuration interaction Hamiltonian, we show that one can extract very accurate ground state wavefunctions as compared…

Chemical Physics · Physics 2020-09-24 Junhan Chen , Zuxin Jin , Wenjie Dou , Joseph Subotnik

Silicon nanospheres are high-quality optical resonators and promising building blocks for Mie-tronic devices. While the Mie resonances of an isolated sphere are well understood, practical implementations require substrates that inevitably…

The morphology and electronic structure of pentacene (Pn) deposited on Cu(111) was studied using scanning tunneling microscopy (STM) and spectroscopy (STS). Deposition of a multilayer followed by annealing to reduce coverage to a monolayer…

Mesoscale and Nanoscale Physics · Physics 2011-10-24 Joseph Smerdon , Matthias Bode , Nathan Guisinger , Jeffrey Guest

By constructing an effective model based on recently calculated \emph{ab }initio bare interaction parameters, we study the phase diagram of alkali doped fullerides as a function of temperature and internal pressure. We use a slave-rotor…

Strongly Correlated Electrons · Physics 2019-10-08 Theja N. De Silva

The interaction of coexisting structural instabilities in multiferroic materials gives rise to intriguing coupling phenomena and extraordinarily rich phase diagrams, both in bulk materials and strained thin films. Here we investigate the…

We study the effects of magnetoelastic coupling on the degenerate ground state of the spin-1/2 antiferromagnetic Heisenberg model for the regular triangular spin cluster. Static displacement of spins spontaneously lifts the degeneracy of…

Other Condensed Matter · Physics 2007-05-23 Ikumi Honda , Kiyosi Terao

Scanning tunneling spectroscopy (STS) allows to image single molecules decoupled from the supporting substrate. The obtained images are routinely interpreted as the square moduli of molecular orbitals, dressed by the mean-field…

Mesoscale and Nanoscale Physics · Physics 2013-01-04 Dimitrios Toroz , Massimo Rontani , Stefano Corni

Ca3CoMnO6 is composed of CoMnO6 chains made up of face-sharing CoO6 trigonal prisms and MnO6 octahedra. The structural, magnetic, and ferroelectric properties of this compound were investigated on the basis of density functional theory…

Materials Science · Physics 2009-11-13 Y. Zhang , H. J. Xiang , M. -H. Whangbo

The atomic doping of open-shell nanographenes enables the precise tuning of their electronic and magnetic state, which is crucial for their promising potential applications in optoelectronics and spintronics. Among this intriguing class of…

It is well-known that the electric field can induce phase transitions between superconducting, metallic and insulating states in thin-film materials due to its control of the charge carrier density. Since a similar effect on the charge…

Superconductivity · Physics 2023-08-14 Liyu Yin , Yunfei Bai , Ming Zhang , A. A. Shanenko , Yajiang Chen

We theoretically investigate charge order and nonlinear conduction in a quasi-two-dimensional organic conductor \beta-(meso-DMBEDT-TTF)2PF6 [DMBEDT-TTF=dimethylbis(ethylenedithio)tetrathiafulvalene]. Within the Hartree-Fock approximation,…

Strongly Correlated Electrons · Physics 2013-10-28 Yasuhiro Tanaka , Kenji Yonemitsu

The physics of an electron solid, held on a cryogenic liquid surface by a pressing electric field, is examined in a low-density regime that has not been explored before. We consider the effect of the pressing field in distorting the surface…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Masudul Haque , Indranil Paul , Sergey Pankov

We study a simple model of the two-channel Kondo effect in a distorted crystal. This model is then used to investigate the interplay of the Kondo and Jahn-Teller effects, and also the Kondo effect in an impure crystal. We find that the…

Strongly Correlated Electrons · Physics 2009-10-31 C. N. Hind , A. O. Gogolin

The quest for molecular structures exhibiting strong quantum interference effects in the transport setting has long been on the forefront of chemical research. Here, we establish theoretically that the unusual geometry of spiro-conjugated…

Mesoscale and Nanoscale Physics · Physics 2018-04-03 Jakub K. Sowa , Jan A. Mol , G. Andrew D. Briggs , Erik M. Gauger

Charge ordering accompanied by lattice distortion in quasi-two dimensional organic conductors \theta-(ET)2X (ET=BEDT-TTF) is studied by using an extended Hubbard model with Peierls-type electron-lattice couplings within the Hartree-Fock…

Strongly Correlated Electrons · Physics 2009-11-13 Yasuhiro Tanaka , Kenji Yonemitsu

We present a theoretical study of a possibility of superconductivity in a three dimensional molecular conductor in which the interaction between electrons in doubly degenerate molecular orbitals and an {\em intra}molecular vibration mode is…

Superconductivity · Physics 2016-08-31 R. Ramakumar , Sudhakar Yarlagadda

We investigate electrostatic stability of charged droplets, modeled as permeable, charged spheres, and their encapsidation in thin, arbitrarily charged nano-shells, immersed in a neutralizing asymmetric electrolyte background. The latter…

Soft Condensed Matter · Physics 2013-11-15 Leili Javidpour , Anže Lošdorfer Božič , Ali Naji , Rudolf Podgornik

The electronic structure and magnetism in the sodium nickelate NaNiO_2 in the low-temperature phase is studied from density-functional calculations using the linear muffin-tin orbitals method. An antiferromagnetic solution with a magnetic…

Strongly Correlated Electrons · Physics 2009-11-10 H. Meskine , S. Satpathy

The self-organization of strongly interacting electrons into superlattice structures underlies the properties of many quantum materials. How these electrons arrange within the superlattice dictates what symmetries are broken and what ground…

Using density functional theory (DFT) with local density approximation (LDA) and generalized gradient approximation (GGA) correlation functionals, the electronic and magnetic structures of cubic BaFeO$_{3}$ in the ferromagnetic (FM) and…

Materials Science · Physics 2013-10-15 Gul Rahman , Juliana M. Morbec , Rubén Ferradás , Víctor M. García-Suárez