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We describe instrumentation for a high-frequency electron paramagnetic resonance (EPR) and pulsed electron-electron double resonance (PELDOR) spectroscopy. The instrumentation is operated in the frequency range of 107$-$120 GHz and…

Instrumentation and Detectors · Physics 2015-06-19 Franklin H. Cho , Viktor Stepanov , Susumu Takahashi

The design and performance of an electron spin resonance spectrometer operating at 3 and 9 GHz microwave frequencies combined with a 9 T superconducting magnet is described. The probehead contains a compact two-loop, one gap resonator and…

Other Condensed Matter · Physics 2009-11-10 Ferenc Simon , Ferenc Muranyi

Electron Spin Resonance (ESR) describes a suite of techniques for characterising electronic systems, with applications in physics, materials science, chemistry, and biology. However, the requirement for large electron spin ensembles in…

Quantum Physics · Physics 2015-03-04 L. T. Hall , P. Kehayias , D. A. Simpson , A. Jarmola , A. Stacey , D. Budker , L. C. L. Hollenberg

Coherent spin resonance methods such as nuclear magnetic resonance (NMR) and electron spin resonance (ESR) spectroscopy have led to spectrally highly sensitive, non-invasive quantum imaging techniques with groundbreaking applications in…

We describe a quasi-optical multifrequency ESR spectrometer operating in the 75-225 GHz range and optimized at 210 GHz for general use in condensed matter physics, chemistry and biology. The quasi-optical bridge detects the change of mm…

Materials Science · Physics 2012-10-23 Kalman L Nagy , Dario Quintavalle , Titusz Feher , Andras Janossy

The rapidly rising fields of spintronics and quantum information science have led to a strong interest in developing the ability to coherently manipulate electron spins. Electron spin resonance (ESR) is a powerful technique to manipulate…

Materials Science · Physics 2009-11-13 M. Pioro-Ladriere , T. Obata , Y. Tokura , Y. -S. Shin , T. Kubo , K. Yoshida , T. Taniyama , S. Tarucha

We report the development of a continuous-wave and pulsed X-band electron spin resonance (ESR) spectrometer for the study of spins on ordered surfaces down to cryogenic temperatures. The spectrometer operates in ultra-high vacuum and…

High frequency electron spin resonance (ESR) spectroscopy is an invaluable tool for identification and characterization of spin systems. Nanoscale ESR using the nitrogen-vacancy (NV) center has been demonstrated down to the level of a…

Mesoscale and Nanoscale Physics · Physics 2020-05-05 Benjamin Fortman , Junior Pena , Karoly Holczer , Susumu Takahashi

Magnetically coupling a nano-mechanical resonator to a double quantum dot confining two electrons can enable the manipulation of a single electron spin and the readout of the resonator's natural frequency. When the Larmor frequency matches…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 N. Lambert , I. Mahboob , M. Pioro-Ladrière , Y. Tokura , S. Tarucha , H. Yamaguchi

Electron paramagnetic resonance (EPR) spectroscopy is an important technology in physics, chemistry, materials science, and biology. Sensitive detection with a small sample volume is a key objective in these areas, because it is crucial,…

In this work, we demonstrate the use of frequency-tunable superconducting NbTiN coplanar waveguide microresonators for multi-frequency pulsed electron spin resonance (ESR) experiments. By applying a bias current to the center pin, the…

Quantum Physics · Physics 2017-07-19 A. T. Asfaw , A. J. Sigillito , A. M. Tyryshkin , T. Schenkel , S. A. Lyon

We report on electron spin resonance (ESR) measurements of phosphorus donors localized in a 200 square micron area below the inductive wire of a lumped element superconducting resonator. By combining quantum limited parametric amplification…

Mesoscale and Nanoscale Physics · Physics 2017-02-10 C. Eichler , A. J. Sigillito , S. A. Lyon , J. R. Petta

The integration of scanning tunneling microscopy (STM) and electron spin resonance (ESR) spectroscopy has emerged as a powerful and innovative tool for discerning spin excitations and spin-spin interactions within atoms and molecules…

Mesoscale and Nanoscale Physics · Physics 2024-11-04 Lyuzhou Ye , Xiao Zheng , Xin Xu

Coherent spin resonance methods, such as nuclear magnetic resonance and electron spin resonance spectroscopy, have led to spectrally highly sensitive, non-invasive quantum imaging techniques. Here, we propose a pump-probe spin resonance…

Quantum Physics · Physics 2024-12-02 Philipp Haslinger , Stefan Nimmrichter , Dennis Rätzel

The use of superconducting micro-resonators in combination with quantum-limited Josephson parametric amplifiers has in recent years lead to more than four orders of magnitude improvement in the sensitivity of pulsed Electron Spin Resonance…

Electron spin resonance (ESR) spectroscopy in scanning tunneling microscopy (STM) has enabled probing the electronic structure of single magnetic atoms and molecules on surfaces with unprecedented energy resolution, as well as demonstrating…

In this study, we report a conceptually novel broadband high-frequency electron spin resonance (HFESR) spectroscopic technique. In contrast to the ordinary force-detected ESR technique, which detects the magnetization change due to the…

Applied Physics · Physics 2018-08-02 Hideyuki Takahashi , Tsubasa Okamoto , Kento Ishimura , Shigeo Hara , Eiji Ohmichi , Hitoshi Ohta

The field of research on magnetic van der Waals compounds -- a special subclass of quasi-two-dimensional materials -- is currently rapidly expanding due to the relevance of these compounds to fundamental research where they serve as a…

Strongly Correlated Electrons · Physics 2024-07-25 Vladislav Kataev , Bernd Büchner , Alexey Alfonsov

Coherent spin resonance techniques, such as nuclear and electron spin resonance spectroscopy, have revolutionized non-invasive imaging by providing spectrally resolved information about spin dynamics. Motivated by the recent emergence of…

Quantum Physics · Physics 2026-02-25 Santiago Beltrán-Romero , Stefan Löffler , Dennis Rätzel , Philipp Haslinger

We report the development of the frequency-modulation (FM) method for measuring electron spin resonance (ESR) absorption in the 210-420 GHz frequency range. We demonstrate that using a high-frequency ESR spectrometer without resonating…

Strongly Correlated Electrons · Physics 2010-07-14 Balint Nafradi , Richard Gaal , Titusz Feher , Laszlo Forro
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