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A hexagonal structure of solid molecular hydrogen with $P6_122$ symmetry is calculated to be more stable below about 200 GPa than the monoclinic $C2/c$ structure identified previously as the best candidate for phase III. We find that the…

Materials Science · Physics 2016-11-01 Bartomeu Monserrat , Richard J. Needs , Eugene Gregoryanz , Chris J. Pickard

An unambiguous crystallographic structure solution for the observed phases II-VI of high pressure hydrogen does not exist due to the failure of standard structural probes at extreme pressure. In this work we propose that nuclear magnetic…

Materials Science · Physics 2019-04-03 Bartomeu Monserrat , Sharon E. Ashbrook , Chris J. Pickard

Structural changes in REMnO3 (RE= Y, Ho, Lu) under high pressure were examined by synchrotron x-ray diffraction methods at room temperature. Compression occurs more readily in the ab plane than along the c-axis. Under hydrostatic pressure…

Materials Science · Physics 2015-05-20 P. Gao , Z. Chen , T. A. Tyson , T. Wu , K. H. Ahn , Z. Liu , R. Tappero , S. B. Kim , S. -W. Cheong

Understanding high-pressure transitions in prototypical linear diatomic molecules, such as hydrogen, nitrogen, and oxygen, is an important objective in high-pressure physics. Recent ultrahigh-pressure study on hydrogen revealed that there…

Materials Science · Physics 2019-10-31 Shan Liu , Meifang Pu , Qiqi Tang , Feng Zhang , Binbin Wu , Li Lei

Our recent developments in in-situ nuclear magnetic resonance (NMR) spectroscopy under extreme conditions led to the observation of a wide variety of physical phenomena not accessible with standard high pressure experimental probes.…

Ab initio molecular dynamic method within the framework of density functional theory is applied to analyze the structural and electronic properties of crystalline molecular hydrogen at temperature 100\,K. Pressure, pair correlation function…

Materials Science · Physics 2022-01-12 I. Saitov

The structural and magnetic properties of the hexagonal four-layer form of SrMnO$_3$ have been investigated by combining magnetization measurements, electron diffraction and high-resolution synchrotron X-ray and neutron powder diffraction.…

Strongly Correlated Electrons · Physics 2007-05-23 A. Daoud-Aladine , C. Martin , L. C. Chapon , M. Hervieu , K. S. Knight , M. Brunelli , P. G. Radaelli

We reassess the phase diagram of high-pressure solid hydrogen using mean-field and many-body wave function based approaches to determine the nature of phase III of solid hydrogen. To discover the best candidates for phase III, density…

Other Condensed Matter · Physics 2019-10-09 Sam Azadi , T. D. Kuehne

The phase diagram of hydrogen is one of the most important challenges in high-pressure physics and astrophysics. Especially, the melting of dense hydrogen is complicated by dimer dissociation, metallization and nuclear quantum effect of…

Materials Science · Physics 2023-04-25 Hua Y. Geng , Q. Wu

Hydrogen has been the essential element in the development of atomic and molecular physics1). Moving to the properties of dense hydrogen has appeared a good deal more complex than originally thought by Wigner and Hungtinton in their seminal…

Materials Science · Physics 2019-06-14 Paul Loubeyre , Florent Occelli , Paul Dumas

Vanadium sesquioxide, V2O3, is a prototypical metal-to-insulator system where, in temperature-dependent studies, the transition always coincides with a corundum-to-monoclinic structural transition. As a function of pressure, V2O3 follows…

Phase I of hydrogen has several peculiarities. Despite having a close-packed crystal structure, it is less dense than either the low temperature Phase II or the liquid phase. At high pressure, it transforms into either phase III or IV,…

Computational Physics · Physics 2016-05-17 Ioan B Magdau , Floris Balm , Graeme J Ackland

The high-pressure behavior of monoclinic VO$_2$ is revisited by a combination of Raman spectroscopy and X-ray diffraction on a single crystal under hydrostatic conditions at room temperature. A soft mode is observed up to P$_c$ = 13.9(1)…

Strongly Correlated Electrons · Physics 2025-01-14 P. Bouvier , L. Bussmann , D. Machon , I. Breslavetz , G. Garbarino , P. Strobel , V. Dmitriev

A detailed high pressure investigation is carried out using x-ray diffraction, Raman spectroscopy and low temperature resistivity measurements on hexagonal ZrSe$_{2}$ having an excess of 3 at.\% Zr. Structural studies show that the sample…

Strongly Correlated Electrons · Physics 2022-09-21 Bishnupada Ghosh , Mrinmay Sahu , Debabrata Samanta , Pinku Saha , Anshuman Mandal , Goutam Dev Mukherjee

We report high pressure structural phase transformation sequence in a layered Iron-based superconducting compound FeSe0.3Te0.7 to 31 GPa at room temperature. The ambient pressure PbO type tetragonal phase (Space Group - P4/nmm) transforms…

Materials Science · Physics 2011-05-05 Andrew K. Stemshorn , Yogesh K. Vohra , Phillip M. Wu , F. C. Hsu , Y. L. Huang , M. K. Wu , K. W. Yeh

We present a technique for extracting Raman intensities from ab initio molecular dynamics (MD) simulations at high temperature. The method is applied to the highly anharmonic case of dense hydrogen up to 500 K for pressures ranging from 180…

Materials Science · Physics 2013-02-25 Ioan B. Magdau , Graeme J. Ackland

The high-pressure II-III phase transition in solid hydrogen is investigated using the random phase approximation and diffusion Monte Carlo. Good agreement between the methods is found confirming that an accurate treatment of exchange and…

Materials Science · Physics 2024-10-08 Maria Hellgren , Damian Contant , Thomas Pitts , Michele Casula

Being the simplest element with just one electron and proton the electronic structure of the Hydrogen atom is known exactly. However, this does not hold for the complex interplay between them in a solid and in particular not at high…

Materials Science · Physics 2014-06-23 Sam Azadi , Thomas D. Kühne

Layered transition-metal trichalcogenides have become one of the research frontiers as two-dimensional magnets and candidate materials used for phase-change memory devices. Herein we report the high-pressure synchrotron X-ray diffraction…

Strongly Correlated Electrons · Physics 2019-06-03 Zhenhai Yu , Wei Xia , Kailang Xu , Ming Xu , Hongyuan Wang , Xia Wang , Na Yu , Zhiqiang Zou , Jinggeng Zhao , Lin Wang , Xiangshui Miao , Yanfeng Guo

High-pressure synchrotron based angle dispersive x-ray diffraction (ADXRD) studies were carried out on SmGdO3 (SGO) up to 25.7GPa at room temperature. ADXRD results indicated a reversible pressure-induced phase transition from ambient…

Materials Science · Physics 2015-06-22 Yogesh Sharma , Pankaj Misra , Satyaprakash Sahoo , A. K. Mishra , S. M. Sharma , Ram S. Katiyar
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