Related papers: Spin hierarchy in van der Waals molecule formation…
We explore the physical origin and the general validity of a propensity rule for the conservation of the hyperfine spin state in three-body recombination. This rule was recently discovered for the special case of $^{87}$Rb with its nearly…
We theoretically investigate the spin structure of weakly bound diatomic van der Waals molecules formed by two identical bosonic alkali atoms. Our studies were performed using known Born-Oppenheimer potentials while developing a reduced…
Van der Waals layered materials are a focus of materials research as they support strong quantum effects and can easily form heterostructures. Electron spins in van der Waals materials played crucial roles in many recent breakthroughs,…
Based on a theoretical model where the nuclear spins remain unchanged during a collision, we provide an analytical and general expression for the nuclear spin state-to-state distribution of an ultracold chemical reaction in a magnetic…
Three-body recombination is a chemical reaction where the collision of three atoms leads to the formation of a diatomic molecule. In the ultracold regime it is expected that the production rate of a molecule generally decreases with its…
Scalar couplings between covalently bound nuclear spins are a ubiquitous feature in nuclear magnetic resonance (NMR) experiments, imparting valuable information to NMR spectra regarding molecular structure and conformation. Such couplings…
We show that weakly bound He-containing van der Waals molecules can be produced and magnetically trapped in buffer-gas cooling experiments, and provide a general model for the formation and dynamics of these molecules. Our analysis shows…
We investigate interacting spin susceptibilities in lattice models for $\mathcal{T}$-reversal symmetry-broken Weyl semimetals. We employ a random phase approximation (RPA) method for the spin-SU(2)-symmetry-broken case that includes…
We describe a novel type of interaction between open-shell polar molecules at sub-millikelvin temperatures. This hyperfine van der Waals interaction occurs between two molecules in two rotational states that differ by one quantum. Normally,…
We reveal a significant spin-exchange pathway in the three-body recombination process for ultracold lithium-7 atoms near a zero-crossing of the two-body scattering length. This newly discovered recombination pathway involves the exchange of…
Three-body recombination is a prime example of the fundamental interaction between three particles. Due to the complexity of this process it has resisted a comprehensive description. Experimental investigations have mainly focussed on the…
We present a technique for engineering quantum magnets via ultracold polar molecules in optical lattices and explore exotic interplay between its spin superfluidity and solidity. The molecular ground and first excited rotational states are…
Strongly correlated two dimensional electrons are believed to form a spin liquid in some regimes of density and temperature. As the density is varied, one expects a transition from this spin liquid state to a spin density wave…
The advent of two-dimensional (2D) crystals has led to numerous scientific breakthroughs. Conventional 2D systems have in-plane covalent bonds and a weak out-of-plane van-der-Waals bond. Here we report a new type of 2D material composed of…
We demonstrate that it is possible to efficiently control ultracold chemical reactions of alkali-metal atoms colliding with open-shell alkali-metal dimers in their metastable triplet states by choosing the internal hyperfine and…
Many-body spin systems represent a paradigmatic platform for the realization of emergent states of matter in a strongly interacting regime. Spin models are commonly studied in one-dimensional periodic chains, whose lattice constant is on…
The main obstacle to coherent control of two-level quantum systems is their coupling to an uncontrolled environment. For electron spins in III-V quantum dots, the random environment is mostly given by the nuclear spins in the quantum dot…
The long-range electrostatic interactions between molecules depend strongly on their relative orientation, which manifests as a rotational state dependence. Interactions between molecules in the same rotational quantum state are well-known…
We present a practical semiclassical method for computing the electron spin dynamics of a radical in which the electron spin is hyperfine coupled to a large number of nuclear spins. This can be used to calculate the singlet and triplet…
We study the role of pairwise long-range interactions in the formation of van der Waals molecules through direct three-body recombination processes A + B + B $\rightarrow$ AB + B, based on a classical trajectory method in hyperspherical…