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The duration of isolated attosecond pulses created via high-order harmonic generation is determined by the number of optical cycles in the driving laser. Achieving shorter attosecond soft X-ray pulses requires minimizing the number of…

Optics · Physics 2025-11-03 Kaito Nishimiya , Rambabu Rajpoot , Eiji J Takahashi

High-harmonic upconversion driven by a mid-infrared femtosecond laser can generate coherent soft X-ray beams in a tabletop-scale setup. Here, we report on a compact ytterbium-pumped optical parametric chirped pulse amplifier (OPCPA) laser…

Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element…

Atomic Physics · Physics 2016-06-08 S. M. Teichmann , F. Silva , S. L. Cousin , M. Hemmer , J. Biegert

We report on the generation of 6.1 mJ, 3.8 fs pulses by the compression of a kHz Ti:sapphire laser in a large-aperture long hollow fiber. In order to find optimal conditions for spectral broadening at high pulse energies, we explore…

Optics · Physics 2020-07-15 Tamas Nagy , Martin Kretschmar , Marc J. J. Vrakking , Arnaud Rouzee

Bright, coherent soft X-ray (SXR) radiation is essential to a variety of applications in fundamental research and life sciences. So far, high photon flux in this spectral region can only be delivered by synchrotrons, free electron lasers or…

Attosecond pulse trains (APTs) are indispensable for probing electron dynamics at their intrinsic timescales. High harmonic generation (HHG) has long been a successful and widely used technique in producing extreme ultraviolet APTs. While…

Accelerator Physics · Physics 2025-10-16 Lanpeng Ni , Junhao Liu , Zheng Qi , Chao Feng

High harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, to date the shortest attosecond (as) pulses have been produced only in the extreme ultraviolet…

The field of attosecond physics has expanded significantly in recent years, yet experimental facilities supporting attosecond pump attosecond probe spectroscopy remain rare. Here, we present a newly constructed beamline for the generation…

In the present work we report on the current progress of the recently constructed GW attosecond extreme ultraviolet (XUV) source developed at the Institute of Electronic Structure and Laser of the Foundation for Research and…

Attosecond pulses in the soft-X-ray (SXR) to water-window energy region offer the tools for creating and studying target specific localized inner-shell electrons or holes in materials, enable monitoring or controlling charge and energy…

Atomic and Molecular Clusters · Physics 2020-03-25 Zhao Xi , Wang Su-Ju , Yu Wei-Wei , Wei Hui , Lin C. D

Paraxial light skyrmions are topological configurations that map a spatial domain of the field onto the full Poincar\'e sphere of polarization states. While optical skyrmions have been explored in continuous-wave regimes, their realization…

Optics · Physics 2025-10-17 David Marco , Luis Plaja , Carlos Hernández-García

A stable 50 mJ three-channel optical waveform synthesizer is demonstrated and used to reproducibly generate a high-order harmonics supercontinuum in the soft-x-ray region. This synthesizer is composed of pump pulses from a…

The generation of coherent light pulses in the extreme ultraviolet (XUV) spectral region with attosecond pulse durations constitutes the foundation of the field of attosecond science. Twenty years after the first demonstration of isolated…

High-order harmonic generation (HHG) in simultaneous intense near-infrared (NIR) laser light and brilliant x rays above an inner-shell absorption edge is examined. A tightly bound inner-shell electron is transferred into the continuum.…

The ongoing development of intense high-harmonic generation (HHG) sources has recently enabled highly nonlinear ionization of atoms by the absorption of at least 10 extreme-ultraviolet (XUV) photons within a single atom [Senfftleben…

Generation of ultrabroadband isolated attosecond pulses (IAPs) is essential for time-resolved applications in chemical and material sciences, as they have the potential to access the spectral water window region of chemical elements, which…

Mesoscale and Nanoscale Physics · Physics 2022-04-20 Younes Adnani , Abdelmalek Taoutioui , Abdelkader Makhoute , Károly Tökési , Hicham Agueny

The development of schemes for coherent nonlinear time-domain spectroscopy in the extreme-ultraviolet regime (XUV) has so far been impeded by experimental difficulties that arise at these short wavelengths. In this work we present a novel…

The short wavelength and high peak power of the present generation of free-electron lasers (FELs) opens the possibility of ultra-short pulses even surpassing the present (tens to hundreds of attoseconds) capabilities of other light sources…

Accelerator Physics · Physics 2013-09-03 D. J. Dunning , B. W. J. McNeil , N. R. Thompson

High-order harmonic generation (HHG) has become a standard technique for producing attosecond XUV pulses in the laboratory, yet the high flux necessary for nonlinear XUV photoionization remains accessible to only a few research groups.…

Attosecond light sources based on high-order harmonic generation (HHG) constitute to date the only table-top solution for producing coherent broadband radiation covering the spectral range from the extreme ultraviolet to the soft X-rays.…

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