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Solid-state platforms provide exceptional opportunities for advancing on-chip quantum technologies by enhancing interaction strengths through coupling, scalability, and robustness. Cuprous oxide ($\text{Cu}_{2}\text{O}$) has recently…

Electrocatalytic water splitting, which produces hydrogen and oxygen through water electrolysis, is a promising method for generating renewable, carbon-free alternative fuels. However, its widespread adoption is hindered by the high costs…

Materials Science · Physics 2024-12-23 Kajjana Boonpalit , Nongnuch Artrith

Here we develop a class off face centred cubic structure of metallic silver nanocrystals, to enable high ORR activity process. Silver nanoparticles deposited within different carbon supports: carboxylated-graphene, SiO2-doted reduced-…

Polycrystalline samples and submillimeter size single crystals of Na-doped Ca2CuO2Cl2 have been synthesized under high pressure. A series of experiments showed that the Na content depends not only on the pressure during the synthesis but…

Superconductivity · Physics 2010-03-03 N. D. Zhigadlo , J. Karpinski , S. Weyeneth , R. Khasanov , S. Katrych , P. Wagli , H. Keller

A high temperature electrochemical oxidation process has been used to produce large single crystals of $La_2CuO_{4 + \delta}$ suitable for neutron scattering experiments. Below room temperature the oxygen-rich phases have structural…

Direct fired supercritical CO2 (sCO2) power cycles allow for the combustion of gaseous fuels under oxyfuel conditions with inherent carbon capture. As the CO2 is captured intrinsically, the efficiency penalty of capture on the overall plant…

Chemical Physics · Physics 2022-03-14 James M. Harman-Thomas , Kevin J. Hughes , Mohamed Pourkashanian

Precious-metal-free spinel oxide electrocatalysts are promising candidates for catalyzing the oxygen reduction reaction (ORR) in alkaline fuel cells. In this theory-driven study, we use joint density-functional theory in tandem with…

Understanding O2 bubble nucleation and growth during the oxygen evolution reaction (OER) is crucial to comprehend their influences on catalytically active sites in the process. To achieve this goal, mapping the spatial variation of…

Mesoscale and Nanoscale Physics · Physics 2025-11-18 Nataraju Bodappa , Gregory Jerkiewicz , Peter Grutter

Innovative synthetic approaches can yield new phases containing novel structural and magnetic motifs. In this work, we show the synthesis and magnetic characterization of three new and one previously reported layered phase in the…

Strongly Correlated Electrons · Physics 2024-03-28 Allana G. Iwanicki , Brandon Wilfong , Eli Zoghlin , Wyatt Bunstine , Maxime A. Siegler , Tyrel M. McQueen

Overlaid self-ordering processes: we form anodic self-organized TiO2 nanostumps and exploit them for self-ordering dewetting of Au-Ag sputtered films. This forms ordered particle configurations at tube top (crown position) or bottom (ground…

Materials Science · Physics 2016-10-17 Nhat Truong Nguyen , Marco Altomare , JeongEun Yoo , Patrik Schmuki

We used quantum chemical ab initio methods to determine the effective parameters of Hubbard and $t-J$ models for the $\rm Na_{x}CoO_2$ compounds (x=0 and 0.5). As for the superconducting compound we found the $a_{1g}$ cobalt orbitals above…

Strongly Correlated Electrons · Physics 2010-07-26 Sylvain Landron , Soret Julien , Marie-Bernadette Lepetit

Hydrogen has emerged as a promising energy source, holding the key to achieve low-carbon and sustainable mobility. However, its applications are still limited by modest conversion efficiency in the electrocatalytic oxygen reduction reaction…

Investigating a reactive chemical system with automated reaction network exploration algorithms provides a more detailed picture of its chemical mechanism than what would be accessible by manual investigation. In general, exploration…

Chemical Physics · Physics 2023-04-14 Moritz Bensberg , Markus Reiher

The rational design of hydrogen evolution reaction (HER) electrocatalysts which are competitive with platinum is an outstanding challenge to make power-to-gas technologies economically viable. Here, we introduce the delafossites PdCrO$_2$,…

Copper-based catalysts play a crucial role in industrial oxidation reactions. Although many theoretical studies consider copper to be metallic, it is well established that copper readily oxides at ambient conditions, forming a passivating…

Materials Science · Physics 2025-05-20 E V Charan Reddy , Abhijit Chatterjee

Electrocatalytic CO2 reduction technology is key to mitigating greenhouse gas emissions and the energy crisis. However, controlling the selectivity of CO2RR products at low overpotential remains a challenge. In this paper, we predicted five…

Materials Science · Physics 2024-03-05 Ran Wang , Chaozheng He , Weixing Chen , Qingquan Kong , Thomas Frauenheimac

We developed a facile and scalable 3-step hydrothermal, electrodeposition, and annealing technique to synthesize a variety of nanowire heterostructures. The heterojunction catalysts of CP-ZnO-MoS2 and CP-ZnO-ZnS-MoS2 both saw an increase in…

Materials Science · Physics 2025-03-10 Lee Kendall , Dawn Ford , Giovanni Zangari , Stephen McDonnell

Composite material was prepared from Bystr\"om-Evers metallic particles Ag5Pb2O6 dispersed in a semiconducting matrix CuO-Cu2O. Partial substitution of CuO by Cu2O increases electric conductivity at 673 K for 2-3 orders of magnitude above…

Superconductivity · Physics 2011-08-31 Danijel Djurek

We have explored the electric field controlled magnetization in the nanodot CoFe2O4/SrRuO3/PMN-PT heterostructures. Ordered ferromagnetic CFO nanodots (~300 nm lateral dimension) are developed on the PMN-PT substrate (ferroelectric as well…

The microscopic doping mechanism behind the superconductor-to-insulator transition of a thin film of YBa2Cu3O7 was recently identified as due to the migration of O atoms from the CuO chains of the film. Here we employ density-functional…

Superconductivity · Physics 2024-06-19 Lorenzo A. Mariano , Roberta Poloni