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We report a comprehensive investigation of the lattice and magnetic structure in van der Waals antiferromagnet VBr3, characterized by a BiI3-type structure at room temperature. Neutron diffraction experiments were performed on both…

Strongly Correlated Electrons · Physics 2024-08-06 Yimeng Gu , Yiqing Hao , Zeyu Kao , Yiqing Gu , Feiyang Liu , Shiyi Zheng , Huibo Cao , Lunhua He , Jun Zhao

We report structural, physical properties and electronic structure of van der Waals (vdW) crystal VI3. Detailed analysis reveals that VI3 exhibits a structural transition from monoclinic C2/m to rhombohedral R-3 at Ts ~ 79 K, similar to…

Materials Science · Physics 2019-06-19 Shangjie Tian , Jian-Feng Zhang , Chenghe Li , Tianping Ying , Shiyan Li , Xiao Zhang , Kai Liu , Hechang Lei

We studied magnetic states and phase transitions in the van der Waals antiferromagnet VBr3 by specific heat and magnetization measurements of single crystals in high magnetic fields and by ab initio density functional theory calculations…

The crystallographic, magnetic, and transport properties of the van der Waals bonded, layered compound CrTe3 have been investigated on single crystal and polycrystalline materials. The crystal structure contains layers made up of lozenge…

Strongly Correlated Electrons · Physics 2017-04-19 Michael A. McGuire , V. Ovidiu Garlea , Santosh KC , Valentino R. Cooper , Jiaqiang Yan , Huibo Cao , Brian C. Sales

Two-dimensional (2D) layered magnetic materials are generating a great amount of interest for the next generation of electronic devices thanks to their remarkable properties associated to spin dynamics. The recently discovered layered…

We present comprehensive measurements of the structural, magnetic and electronic properties of layered van-der-Waals ferromagnet VI$_3$ down to low temperatures. Despite belonging to a well studied family of transition metal trihalides,…

The results of a single-crystal X-ray-diffraction study of the evolution of crystal structures of VI3 with temperature with emphasis on phase transitions are presented. Some related specific-heat and magnetization data are included. The…

The van der Waals ferromagnet (FM), VI$_3$, was studied by muon spin relaxation ($\mu^+$SR) and first principle calculations based on density functional theory (DFT). Temperature dependent zero field muon spin relaxation ($\mu^+$SR)…

Strongly Correlated Electrons · Physics 2022-11-01 Ola Kenji Forslund , Yuqing Ge , Hiroto Ohta , Chennan Wang , Mahmoud Abdel-Hafiez , Jun Sugiyama , Martin Månsson , Yasmine Sassa

Van der Waals magnet VI$_3$ demonstrates intriguing magnetic properties that render it great for use in various applications. However, its microscopic magnetic structure has not been determined yet. Here, we report neutron diffraction and…

Strongly Correlated Electrons · Physics 2021-08-19 Yiqing Hao , Yiqing Gu , Yimeng Gu , Erxi Feng , Huibo Cao , Songxue Chi , Hua Wu , Jun Zhao

We present a combined study of zero-field $^{51}$V and $^{127}$I NMR at ambient pressure and specific heat and magnetization measurements under pressure up to 2.08 GPa on bulk single crystals of the van-der-Waals ferromagnet VI$_3$. At…

Strongly Correlated Electrons · Physics 2019-11-21 Elena Gati , Yuji Inagaki , Tai Kong , Robert J. Cava , Yuji Furukawa , Paul C. Canfield , Sergey L. Bud'ko

The van der Waals (vdW) layered multiferroics, which host simultaneous ferroelectric and magnetic orders, have attracted attention not only for their potentials to be utilized in nanoelectric devices and spintronics, but also offer…

Van der Waals (vdW) heterostructures have attracted great interest because of their rich material combinations.The discovery of two-dimensional magnets has provided a new platform for magnetic vdW heterointerfaces; however, research on…

Van der Waals (vdW) magnet heterostructures have emerged as new platforms to explore exotic magnetic orders and quantum phenomena. Here, we study heterostructures of layered antiferromagnets, CrI3 and CrCl3, with perpendicular and in-plane…

Van der Waals (vdW) Dirac magnon system CrI$_3$, a potential host of topological edge magnons, orders ferromagnetically (FM) (T$_C=61$ K) in the bulk, but antiferromagnetic (AFM) order has been observed in nanometer thick flakes, attributed…

Materials Science · Physics 2024-05-14 John A. Schneeloch , Luke Daemen , Despina Louca

The $R\mathrm{Te}_3$ ($R = \text{rare earth}$) family of layered van der Waals (vdW) compounds hosts coexisting magnetic and charge density wave (CDW) orders, yet the interplay between these degrees of freedom remains little explored.…

The recent discovery of magnetism within the family of exfoliatable van der Waals (vdW) compounds has attracted considerable interest in these materials for both fundamental research and technological applications. However current vdW…

We report the enhancement of N\'eel temperature of Cr2O3 by replacing 50% of Cr by Fe prepared by sol-gel method. The structural analysis by neutron diffraction has revealed that FeCrO3 belongs to a corundum structure (R-3c space group)…

Materials Science · Physics 2019-11-26 Rajesh kumar R , C. Dhanasekhar , N. Vijay Prakash Chaudhary , A. Das , A. Venimadhav

We grew high-quality single crystals of the 5f electron van der Waals compound UI$_3$ and investigated them by measurements of specific heat and magnetization as functions of temperature and magnetic field. UI$_3$ behaves as an…

alpha-UTe3, a van der Waals (vdW) actinide compound with a monoclinic ZrSe3-type structure, is a narrow-gap semiconductor with 5f moments. 125Te NMR reveals strongly anisotropic, layer-confined spin fluctuations below about 20 K, with the…

Strongly Correlated Electrons · Physics 2025-10-14 H. Sakai , C. Tabata , K. Kaneko , Y. Tokiwa , T. Kitazawa , S. Kambe , Y. Tokunaga , Y. Haga

External pressure suppresses the ferromagnetism of localized Cr 3d electron moments in the van der Waals insulator CrBr3, which cannot be explained without considering a dramatic pressure-induced crystal or electronic structure change. We…

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